WO2019027347A1 - Коррозионностойкий сплав - Google Patents
Коррозионностойкий сплав Download PDFInfo
- Publication number
- WO2019027347A1 WO2019027347A1 PCT/RU2017/001014 RU2017001014W WO2019027347A1 WO 2019027347 A1 WO2019027347 A1 WO 2019027347A1 RU 2017001014 W RU2017001014 W RU 2017001014W WO 2019027347 A1 WO2019027347 A1 WO 2019027347A1
- Authority
- WO
- WIPO (PCT)
- Prior art keywords
- corrosion
- alloy
- nickel
- niobium
- carbon
- Prior art date
Links
- 229910045601 alloy Inorganic materials 0.000 title claims abstract description 35
- 239000000956 alloy Substances 0.000 title claims abstract description 35
- 230000007797 corrosion Effects 0.000 title claims abstract description 20
- 238000005260 corrosion Methods 0.000 title claims abstract description 20
- PXHVJJICTQNCMI-UHFFFAOYSA-N Nickel Chemical compound [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 claims abstract description 22
- XEEYBQQBJWHFJM-UHFFFAOYSA-N Iron Chemical compound [Fe] XEEYBQQBJWHFJM-UHFFFAOYSA-N 0.000 claims abstract description 10
- 229910052759 nickel Inorganic materials 0.000 claims abstract description 10
- 239000010936 titanium Substances 0.000 claims abstract description 9
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 claims abstract description 8
- 229910052799 carbon Inorganic materials 0.000 claims abstract description 8
- 229910052758 niobium Inorganic materials 0.000 claims abstract description 8
- 239000010955 niobium Substances 0.000 claims abstract description 8
- GUCVJGMIXFAOAE-UHFFFAOYSA-N niobium atom Chemical compound [Nb] GUCVJGMIXFAOAE-UHFFFAOYSA-N 0.000 claims abstract description 8
- RTAQQCXQSZGOHL-UHFFFAOYSA-N Titanium Chemical compound [Ti] RTAQQCXQSZGOHL-UHFFFAOYSA-N 0.000 claims abstract description 7
- 229910052719 titanium Inorganic materials 0.000 claims abstract description 7
- 229910052782 aluminium Inorganic materials 0.000 claims abstract description 5
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 claims abstract description 5
- 229910052710 silicon Inorganic materials 0.000 claims abstract description 5
- 239000010703 silicon Substances 0.000 claims abstract description 5
- 239000012535 impurity Substances 0.000 claims abstract description 4
- 229910052742 iron Inorganic materials 0.000 claims abstract description 4
- FYYHWMGAXLPEAU-UHFFFAOYSA-N Magnesium Chemical compound [Mg] FYYHWMGAXLPEAU-UHFFFAOYSA-N 0.000 claims abstract description 3
- 229910052804 chromium Inorganic materials 0.000 claims abstract description 3
- 239000011651 chromium Substances 0.000 claims abstract description 3
- 239000011777 magnesium Substances 0.000 claims abstract description 3
- 229910052749 magnesium Inorganic materials 0.000 claims abstract description 3
- VYZAMTAEIAYCRO-UHFFFAOYSA-N Chromium Chemical compound [Cr] VYZAMTAEIAYCRO-UHFFFAOYSA-N 0.000 claims abstract 3
- ZOKXTWBITQBERF-UHFFFAOYSA-N Molybdenum Chemical compound [Mo] ZOKXTWBITQBERF-UHFFFAOYSA-N 0.000 claims abstract 3
- 229910052750 molybdenum Inorganic materials 0.000 claims abstract 3
- 239000011733 molybdenum Substances 0.000 claims abstract 3
- OAICVXFJPJFONN-UHFFFAOYSA-N Phosphorus Chemical compound [P] OAICVXFJPJFONN-UHFFFAOYSA-N 0.000 claims abstract 2
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical compound [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 claims abstract 2
- WPBNNNQJVZRUHP-UHFFFAOYSA-L manganese(2+);methyl n-[[2-(methoxycarbonylcarbamothioylamino)phenyl]carbamothioyl]carbamate;n-[2-(sulfidocarbothioylamino)ethyl]carbamodithioate Chemical compound [Mn+2].[S-]C(=S)NCCNC([S-])=S.COC(=O)NC(=S)NC1=CC=CC=C1NC(=S)NC(=O)OC WPBNNNQJVZRUHP-UHFFFAOYSA-L 0.000 claims abstract 2
- 229910052698 phosphorus Inorganic materials 0.000 claims abstract 2
- 239000011574 phosphorus Substances 0.000 claims abstract 2
- XUIMIQQOPSSXEZ-UHFFFAOYSA-N Silicon Chemical compound [Si] XUIMIQQOPSSXEZ-UHFFFAOYSA-N 0.000 claims description 3
- 239000011572 manganese Substances 0.000 claims description 3
- PWHULOQIROXLJO-UHFFFAOYSA-N Manganese Chemical compound [Mn] PWHULOQIROXLJO-UHFFFAOYSA-N 0.000 claims description 2
- 229910052748 manganese Inorganic materials 0.000 claims description 2
- 229910052717 sulfur Inorganic materials 0.000 claims 1
- 239000011593 sulfur Substances 0.000 claims 1
- 238000005272 metallurgy Methods 0.000 abstract description 2
- 239000005864 Sulphur Substances 0.000 abstract 1
- 239000004411 aluminium Substances 0.000 abstract 1
- QTBSBXVTEAMEQO-UHFFFAOYSA-N Acetic acid Chemical compound CC(O)=O QTBSBXVTEAMEQO-UHFFFAOYSA-N 0.000 description 6
- 230000015572 biosynthetic process Effects 0.000 description 5
- -1 chromium carbides Chemical class 0.000 description 3
- 230000007423 decrease Effects 0.000 description 3
- 238000004519 manufacturing process Methods 0.000 description 3
- 239000000203 mixture Substances 0.000 description 3
- 239000000126 substance Substances 0.000 description 3
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 2
- 150000001805 chlorine compounds Chemical class 0.000 description 2
- 238000005336 cracking Methods 0.000 description 2
- 230000006378 damage Effects 0.000 description 2
- 229910052751 metal Inorganic materials 0.000 description 2
- 239000002184 metal Substances 0.000 description 2
- 150000001247 metal acetylides Chemical class 0.000 description 2
- 239000001301 oxygen Substances 0.000 description 2
- 229910052760 oxygen Inorganic materials 0.000 description 2
- 239000004033 plastic Substances 0.000 description 2
- 229920003023 plastic Polymers 0.000 description 2
- 238000011179 visual inspection Methods 0.000 description 2
- UGFAIRIUMAVXCW-UHFFFAOYSA-N Carbon monoxide Chemical compound [O+]#[C-] UGFAIRIUMAVXCW-UHFFFAOYSA-N 0.000 description 1
- VEXZGXHMUGYJMC-UHFFFAOYSA-M Chloride anion Chemical compound [Cl-] VEXZGXHMUGYJMC-UHFFFAOYSA-M 0.000 description 1
- 229920000877 Melamine resin Polymers 0.000 description 1
- 229910001182 Mo alloy Inorganic materials 0.000 description 1
- 229910018487 Ni—Cr Inorganic materials 0.000 description 1
- 229910000831 Steel Inorganic materials 0.000 description 1
- XTXRWKRVRITETP-UHFFFAOYSA-N Vinyl acetate Chemical compound CC(=O)OC=C XTXRWKRVRITETP-UHFFFAOYSA-N 0.000 description 1
- QCWXUUIWCKQGHC-UHFFFAOYSA-N Zirconium Chemical compound [Zr] QCWXUUIWCKQGHC-UHFFFAOYSA-N 0.000 description 1
- 239000002253 acid Substances 0.000 description 1
- 230000002411 adverse Effects 0.000 description 1
- 239000003905 agrochemical Substances 0.000 description 1
- 238000005452 bending Methods 0.000 description 1
- 238000009835 boiling Methods 0.000 description 1
- VNNRSPGTAMTISX-UHFFFAOYSA-N chromium nickel Chemical compound [Cr].[Ni] VNNRSPGTAMTISX-UHFFFAOYSA-N 0.000 description 1
- 238000006477 desulfuration reaction Methods 0.000 description 1
- 230000023556 desulfurization Effects 0.000 description 1
- 230000006866 deterioration Effects 0.000 description 1
- 238000005516 engineering process Methods 0.000 description 1
- 239000003822 epoxy resin Substances 0.000 description 1
- 230000005496 eutectics Effects 0.000 description 1
- 239000003546 flue gas Substances 0.000 description 1
- 150000002362 hafnium Chemical class 0.000 description 1
- LNEPOXFFQSENCJ-UHFFFAOYSA-N haloperidol Chemical compound C1CC(O)(C=2C=CC(Cl)=CC=2)CCN1CCCC(=O)C1=CC=C(F)C=C1 LNEPOXFFQSENCJ-UHFFFAOYSA-N 0.000 description 1
- 238000009434 installation Methods 0.000 description 1
- 230000003993 interaction Effects 0.000 description 1
- JDSHMPZPIAZGSV-UHFFFAOYSA-N melamine Chemical compound NC1=NC(N)=NC(N)=N1 JDSHMPZPIAZGSV-UHFFFAOYSA-N 0.000 description 1
- 238000002844 melting Methods 0.000 description 1
- 150000004767 nitrides Chemical class 0.000 description 1
- 229910052757 nitrogen Inorganic materials 0.000 description 1
- 150000002894 organic compounds Chemical class 0.000 description 1
- 239000007800 oxidant agent Substances 0.000 description 1
- 230000001590 oxidative effect Effects 0.000 description 1
- 238000005554 pickling Methods 0.000 description 1
- 229920000647 polyepoxide Polymers 0.000 description 1
- 230000008092 positive effect Effects 0.000 description 1
- 230000009257 reactivity Effects 0.000 description 1
- 230000008929 regeneration Effects 0.000 description 1
- 238000011069 regeneration method Methods 0.000 description 1
- 239000010959 steel Substances 0.000 description 1
- 229910052726 zirconium Inorganic materials 0.000 description 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C22—METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
- C22C—ALLOYS
- C22C19/00—Alloys based on nickel or cobalt
- C22C19/03—Alloys based on nickel or cobalt based on nickel
- C22C19/05—Alloys based on nickel or cobalt based on nickel with chromium
- C22C19/051—Alloys based on nickel or cobalt based on nickel with chromium and Mo or W
- C22C19/055—Alloys based on nickel or cobalt based on nickel with chromium and Mo or W with the maximum Cr content being at least 20% but less than 30%
-
- C—CHEMISTRY; METALLURGY
- C22—METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
- C22F—CHANGING THE PHYSICAL STRUCTURE OF NON-FERROUS METALS AND NON-FERROUS ALLOYS
- C22F1/00—Changing the physical structure of non-ferrous metals or alloys by heat treatment or by hot or cold working
- C22F1/10—Changing the physical structure of non-ferrous metals or alloys by heat treatment or by hot or cold working of nickel or cobalt or alloys based thereon
Definitions
- the invention relates to metallurgy, to nickel-based alloys, intended for operation in aggressive oxidizing environments.
- Nicrofer 6616 hMo alloy C-4 (N ° 2.4610), containing wt.%: 14.5-17.5 Cg, 14.0-17.0 Mo, ⁇ 3.0 Fe, ⁇ 0.009 ⁇ , ⁇ 1.0 Mn, ⁇ 0.05 Si, ⁇ 2.0 Co, ⁇ 0.7 Ti, ⁇ 0.020 P, ⁇ 0.010 S, nickel and inevitable impurities are the rest (Reference book “Corrosion-resistant, heat-resistant and high-strength steels and Alloys, M., Prometheus-Splav, 2008, p. 304 - 306).
- the alloy is used to manufacture equipment operated in a wide range of chemical environments, at room and elevated temperatures. In particular - for adsorbers during flue gas desulfurization; pickling baths and acid regeneration plants; Acetic acid and agrochemical plants.
- the closest analogue of the present invention is an alloy HN65MVU (EP760) containing, wt.%: ⁇ 0.02 C, ⁇ 0.1 Si, ⁇ 1.0 Mp, 14.5-16.5 Cg, 15.0-17, 0 Mo, 3.0-4.5 W, ⁇ 0.5 Fe, ⁇ 0.012 S, ⁇ 0.015 P, nickel and inevitable impurities else (GOST 5632-2014 is a prototype).
- the alloy is used for the manufacture of welded structures (columns, heat exchangers, reactors) operating at elevated temperatures in corrosive redox environments, in the chemical, petrochemical industry (production of acetic acid, epoxy resins, vinyl acetate, melamine) complex organic compounds) and other industries in the temperature range from -70 to 500 ° C.
- the KhN65MVU brand alloy and its welded joints can be used in KCl-AlCb-ZrCU environments only up to 500 ° C, since at temperatures above the specified value, in addition to intergranular corrosion and corrosion cracking, the alloy sharply decreases the relative elongation from 48% to 7.3-13% at 550 ° C and to 2.5% at 625 ° C and metal embrittlement when deformation is applied.
- the technical result of the invention consists in obtaining an alloy with an increased level of plastic properties during operation in the temperature range from 550 ° C to steadiness and, accordingly, the deterioration of the processability of the alloy during metallurgical processing.
- Niobium in an amount of 0.01–0.03% binds residual carbon and nitrogen into carbides, nitrides, and carbonitrides, prevents the formation of chromium carbides and carbonitrides at grain boundaries.
- the addition of niobium in an amount 6–10 times higher than the carbon content in the alloy eliminates intergranular corrosion of the alloys and protects the welds from damage.
- the niobium content is less than 0.01%, its interaction with residual carbon is ineffective, and the niobium content above 0.03% is not rational for carbide formation.
- An increase in the manganese content of more than 1.0% leads to the appearance of a low-melting eutectic, which leads to the destruction of the ingot during pressure treatment and reduces the heat resistance of the alloy, and also leads to a decrease in resistance to local corrosion.
- Nickel is stable in HC1 even at boiling point. However, in the presence of chlorides, Fe (III) ions and other oxidizing agents, corrosion of nickel and nickel chromium of molybdenum alloys is enhanced, and the associated iron content is not more than 0.75%.
- titanium in an amount of 0.01–0.06% increases the corrosion resistance in molten zirconium and hafnium salts, binds residual carbon to carbides and leads to the formation of a sufficient amount of intermetallic Ni 3 Ti, which, at an operating temperature of 500–700 ° C positive effect on the heat resistance of the alloy.
- the content of titanium is less than 0.01%, the requirements for corrosion resistance are not met, and an excess of titanium content above 0.06% leads to a decrease in the processability of the alloy and the formation of undesirable phases due to the reactivity of titanium.
- Aluminum and magnesium in the amount of 0.1-0.2% and 0.005-0.01% are introduced into the alloy for the removal of residual oxygen, and also, as for aluminum, for the formation of intermetallic metal Ni 3 Al, which positively affects on the heat resistance of the alloy. With the introduction of these elements in quantities less than those indicated, the necessary removal of residual oxygen is not achieved. If the content of these elements is exceeded, coarse non-metallic inclusions are formed.
- the corrosion rate of alloys (alloys 1, 2), satisfying the claimed composition, is lower than the corrosion rate of the prototype alloy, visual inspection did not reveal cracks, unlike the prototype alloy.
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Mechanical Engineering (AREA)
- Metallurgy (AREA)
- Organic Chemistry (AREA)
- Physics & Mathematics (AREA)
- Thermal Sciences (AREA)
- Crystallography & Structural Chemistry (AREA)
- Powder Metallurgy (AREA)
- Preventing Corrosion Or Incrustation Of Metals (AREA)
- Treatment Of Steel In Its Molten State (AREA)
- Manufacture And Refinement Of Metals (AREA)
Abstract
Description
Claims
Priority Applications (9)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
MYPI2019007591A MY192470A (en) | 2017-08-01 | 2017-12-29 | Corrosion resistant alloy |
CA3093022A CA3093022C (en) | 2017-08-01 | 2017-12-29 | Corrosion resistant alloy |
EA201992733A EA201992733A1 (ru) | 2017-08-01 | 2017-12-29 | Коррозионно-стойкий сплав |
KR1020197038839A KR20200060694A (ko) | 2017-08-01 | 2017-12-29 | 내식합금 |
JP2019572506A JP6974507B2 (ja) | 2017-08-01 | 2017-12-29 | 耐食性合金 |
EP17919968.2A EP3663422A4 (en) | 2017-08-01 | 2017-12-29 | CORROSION RESISTANT ALLOY |
BR112019028257-2A BR112019028257B1 (pt) | 2017-08-01 | 2017-12-29 | Liga resistente à corrosão |
CN201780092598.3A CN111094603B (zh) | 2017-08-01 | 2017-12-29 | 耐腐蚀合金 |
US16/627,736 US20210164075A1 (en) | 2017-08-01 | 2017-12-29 | Corrosion-resistant alloy |
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
RU2017127607 | 2017-08-01 | ||
RU2017127607A RU2672647C1 (ru) | 2017-08-01 | 2017-08-01 | Коррозионностойкий сплав |
Publications (2)
Publication Number | Publication Date |
---|---|
WO2019027347A1 true WO2019027347A1 (ru) | 2019-02-07 |
WO2019027347A8 WO2019027347A8 (ru) | 2020-09-10 |
Family
ID=64328060
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
PCT/RU2017/001014 WO2019027347A1 (ru) | 2017-08-01 | 2017-12-29 | Коррозионностойкий сплав |
Country Status (11)
Country | Link |
---|---|
US (1) | US20210164075A1 (ru) |
EP (1) | EP3663422A4 (ru) |
JP (1) | JP6974507B2 (ru) |
KR (1) | KR20200060694A (ru) |
CN (1) | CN111094603B (ru) |
CA (1) | CA3093022C (ru) |
EA (1) | EA201992733A1 (ru) |
JO (1) | JOP20190301A1 (ru) |
MY (1) | MY192470A (ru) |
RU (1) | RU2672647C1 (ru) |
WO (1) | WO2019027347A1 (ru) |
Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4906437A (en) * | 1988-03-03 | 1990-03-06 | Vdm Nickel-Technologie Aktiengesellschaft | Corrosion resistant hot and cold forming parts of Ni-Cr-Mo alloy and method of making same |
US5855699A (en) * | 1994-10-03 | 1999-01-05 | Daido Tokushuko Kabushiki Kaisha | Method for manufacturing welded clad steel tube |
US20030049155A1 (en) * | 2001-06-28 | 2003-03-13 | Pike Lee M. | Two step aging treatment for Ni-Cr-Mo alloys |
GB2405643A (en) * | 2003-09-05 | 2005-03-09 | Haynes Internat Inc | A nickel-chromium-molybdenum alloy |
RU2440876C1 (ru) * | 2010-08-23 | 2012-01-27 | Евгений Григорьевич Старченко | Сварочная проволока для сварки корпусных деталей из разнородных сталей |
Family Cites Families (11)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
IL82587A0 (en) * | 1986-05-27 | 1987-11-30 | Carpenter Technology Corp | Nickel-base alloy and method for preparation thereof |
JPH028337A (ja) * | 1988-06-24 | 1990-01-11 | Nippon Stainless Steel Co Ltd | 電気めっき用通電ロールおよびその製造方法 |
JPH05255784A (ja) * | 1992-03-11 | 1993-10-05 | Sumitomo Metal Ind Ltd | 耐食性に優れた油井用Ni基合金 |
JPH0617173A (ja) * | 1992-07-03 | 1994-01-25 | Mitsubishi Steel Mfg Co Ltd | 電気メッキ用通電ロール |
DE19723491C1 (de) * | 1997-06-05 | 1998-12-03 | Krupp Vdm Gmbh | Verwendung einer Nickel-Chrom-Molybdän-Legierung |
KR20030003017A (ko) * | 2001-06-28 | 2003-01-09 | 하이네스인터내셔널인코포레이티드 | Ni-Cr-Mo합금의 2-단계 에이징 처리방법 및 결과의합금 |
DE10302989B4 (de) * | 2003-01-25 | 2005-03-03 | Schmidt + Clemens Gmbh & Co. Kg | Verwendung einer Hitze- und korrosionsbeständigen Nickel-Chrom-Stahllegierung |
JP4519520B2 (ja) * | 2003-09-24 | 2010-08-04 | 新日鐵住金ステンレス株式会社 | 高Ni基合金溶接ワイヤ |
EP1777313B1 (en) * | 2004-06-30 | 2012-08-01 | Sumitomo Metal Industries, Ltd. | Ni BASE ALLOY MATERIAL TUBE AND METHOD FOR PRODUCTION THEREOF |
JP6259336B2 (ja) * | 2014-03-26 | 2018-01-10 | 日本冶金工業株式会社 | Ni基合金およびその製造方法 |
JP6323188B2 (ja) * | 2014-06-11 | 2018-05-16 | 新日鐵住金株式会社 | Ni基耐熱合金溶接継手の製造方法 |
-
2017
- 2017-08-01 RU RU2017127607A patent/RU2672647C1/ru active
- 2017-12-29 EA EA201992733A patent/EA201992733A1/ru unknown
- 2017-12-29 JP JP2019572506A patent/JP6974507B2/ja active Active
- 2017-12-29 US US16/627,736 patent/US20210164075A1/en not_active Abandoned
- 2017-12-29 EP EP17919968.2A patent/EP3663422A4/en not_active Withdrawn
- 2017-12-29 KR KR1020197038839A patent/KR20200060694A/ko not_active Application Discontinuation
- 2017-12-29 CN CN201780092598.3A patent/CN111094603B/zh active Active
- 2017-12-29 WO PCT/RU2017/001014 patent/WO2019027347A1/ru unknown
- 2017-12-29 CA CA3093022A patent/CA3093022C/en active Active
- 2017-12-29 MY MYPI2019007591A patent/MY192470A/en unknown
-
2019
- 2019-02-01 JO JOP/2019/0301A patent/JOP20190301A1/ar unknown
Patent Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4906437A (en) * | 1988-03-03 | 1990-03-06 | Vdm Nickel-Technologie Aktiengesellschaft | Corrosion resistant hot and cold forming parts of Ni-Cr-Mo alloy and method of making same |
US5855699A (en) * | 1994-10-03 | 1999-01-05 | Daido Tokushuko Kabushiki Kaisha | Method for manufacturing welded clad steel tube |
US20030049155A1 (en) * | 2001-06-28 | 2003-03-13 | Pike Lee M. | Two step aging treatment for Ni-Cr-Mo alloys |
GB2405643A (en) * | 2003-09-05 | 2005-03-09 | Haynes Internat Inc | A nickel-chromium-molybdenum alloy |
RU2440876C1 (ru) * | 2010-08-23 | 2012-01-27 | Евгений Григорьевич Старченко | Сварочная проволока для сварки корпусных деталей из разнородных сталей |
Also Published As
Publication number | Publication date |
---|---|
CA3093022C (en) | 2023-08-08 |
EP3663422A4 (en) | 2021-01-20 |
JOP20190301A1 (ar) | 2019-12-30 |
JP2020530064A (ja) | 2020-10-15 |
US20210164075A1 (en) | 2021-06-03 |
CN111094603B (zh) | 2021-12-07 |
CN111094603A (zh) | 2020-05-01 |
EP3663422A1 (en) | 2020-06-10 |
CA3093022A1 (en) | 2019-02-07 |
JP6974507B2 (ja) | 2021-12-01 |
KR20200060694A (ko) | 2020-06-01 |
BR112019028257A2 (pt) | 2020-08-04 |
WO2019027347A8 (ru) | 2020-09-10 |
RU2672647C1 (ru) | 2018-11-16 |
MY192470A (en) | 2022-08-22 |
EA201992733A1 (ru) | 2021-04-20 |
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