WO2011128760A3 - Method of manufacturing a fuel cell - Google Patents

Method of manufacturing a fuel cell Download PDF

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Publication number
WO2011128760A3
WO2011128760A3 PCT/IB2011/000813 IB2011000813W WO2011128760A3 WO 2011128760 A3 WO2011128760 A3 WO 2011128760A3 IB 2011000813 W IB2011000813 W IB 2011000813W WO 2011128760 A3 WO2011128760 A3 WO 2011128760A3
Authority
WO
WIPO (PCT)
Prior art keywords
substrate
manufacturing
fuel cell
carbon nanotubes
polymer electrolyte
Prior art date
Application number
PCT/IB2011/000813
Other languages
French (fr)
Other versions
WO2011128760A2 (en
Inventor
Shigeki Hasegawa
Yoshihiro Shinozaki
Masahiro Imanishi
Seiji Sano
Original Assignee
Toyota Jidosha Kabushiki Kaisha
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Toyota Jidosha Kabushiki Kaisha filed Critical Toyota Jidosha Kabushiki Kaisha
Priority to US13/637,996 priority Critical patent/US9203101B2/en
Priority to EP11726489.5A priority patent/EP2559086B1/en
Publication of WO2011128760A2 publication Critical patent/WO2011128760A2/en
Publication of WO2011128760A3 publication Critical patent/WO2011128760A3/en

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1007Fuel cells with solid electrolytes with both reactants being gaseous or vaporised
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8605Porous electrodes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8657Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites layered
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8663Selection of inactive substances as ingredients for catalytic active masses, e.g. binders, fillers
    • H01M4/8673Electrically conductive fillers
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8803Supports for the deposition of the catalytic active composition
    • H01M4/8814Temporary supports, e.g. decal
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8817Treatment of supports before application of the catalytic active composition
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8875Methods for shaping the electrode into free-standing bodies, like sheets, films or grids, e.g. moulding, hot-pressing, casting without support, extrusion without support
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8878Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M2008/1095Fuel cells with polymeric electrolytes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8825Methods for deposition of the catalytic active composition
    • H01M4/8846Impregnation
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8825Methods for deposition of the catalytic active composition
    • H01M4/886Powder spraying, e.g. wet or dry powder spraying, plasma spraying
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8878Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8892Impregnation or coating of the catalyst layer, e.g. by an ionomer
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product

Abstract

A method of manufacturing a fuel cell (10) includes: growing carbon nanotubes (161) substantially perpendicular to a substrate formed by loading a growth catalyst on a base material; arranging the substrate and a polymer electrolyte membrane (12) so as to oppose to each other and combining the carbon nanotubes (161) with the polymer electrolyte membrane (12); and dissolving and removing part of the substrate by immersing the substrate in a solution which dissolves the substrate, after the carbon nanotubes (161) and the polymer electrolyte (12) membrane are combined..
PCT/IB2011/000813 2010-04-13 2011-04-12 Method of manufacturing fuel cell WO2011128760A2 (en)

Priority Applications (2)

Application Number Priority Date Filing Date Title
US13/637,996 US9203101B2 (en) 2010-04-13 2011-04-12 Method of manufacturing fuel cell
EP11726489.5A EP2559086B1 (en) 2010-04-13 2011-04-12 Method of manufacturing a fuel cell

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2010091928A JP5093288B2 (en) 2010-04-13 2010-04-13 Manufacturing method of fuel cell
JP2010-091928 2010-04-13

Publications (2)

Publication Number Publication Date
WO2011128760A2 WO2011128760A2 (en) 2011-10-20
WO2011128760A3 true WO2011128760A3 (en) 2012-02-02

Family

ID=44280657

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/IB2011/000813 WO2011128760A2 (en) 2010-04-13 2011-04-12 Method of manufacturing fuel cell

Country Status (4)

Country Link
US (1) US9203101B2 (en)
EP (1) EP2559086B1 (en)
JP (1) JP5093288B2 (en)
WO (1) WO2011128760A2 (en)

Families Citing this family (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP5240348B2 (en) 2011-11-07 2013-07-17 トヨタ自動車株式会社 Manufacturing method of membrane electrode assembly
JP5655802B2 (en) * 2012-03-01 2015-01-21 トヨタ自動車株式会社 Membrane electrode assembly manufacturing method, membrane electrode assembly, and fuel cell
WO2019101517A1 (en) * 2017-11-21 2019-05-31 Asml Netherlands B.V. Porous graphitic pellicle

Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20040224217A1 (en) * 2003-05-08 2004-11-11 Toops Todd Jefferson Integrated membrane electrode assembly using aligned carbon nanotubules
WO2005035841A2 (en) * 2003-10-10 2005-04-21 Board Of Regents, The University Of Texas System Carbon nanostructure-based electrocatalytic electrodes
US6890506B1 (en) * 2001-04-12 2005-05-10 Penn State Research Foundation Method of forming carbon fibers
US20060269827A1 (en) * 2005-05-26 2006-11-30 The University Of Chicago Method of fabricating electrode catalyst layers with directionally oriented carbon support for proton exchange membrane fuel cell
WO2008115753A2 (en) * 2007-03-16 2008-09-25 Honda Motor Co., Ltd. Method of preparing carbon nanotube containing electrodes
US20100075201A1 (en) * 2006-03-20 2010-03-25 Haruyuki Nakanishi Fuel cell with electrode having an electrically conductive nano-column and production method thereof

Family Cites Families (17)

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Publication number Priority date Publication date Assignee Title
JP3655208B2 (en) 2001-03-29 2005-06-02 株式会社東芝 FUEL CELL, ELECTRODE FOR FUEL CELL AND METHOD FOR PRODUCING THE SAME
KR20040093665A (en) * 2001-11-28 2004-11-06 고쿠리츠 다이가쿠 호우징 나고야 다이가쿠 Method for preparing hollow nanofiber, hollow nanofiber and catalyst composition for preparing hollow nanofiber
US6793738B2 (en) * 2002-03-28 2004-09-21 General Electric Company Method for processing acid treatment solution, solution processed thereby, and method for treating articles therewith
US7531158B2 (en) * 2003-03-20 2009-05-12 Cheol Jin Lee Vapor phase synthesis of double-walled carbon nanotubes
JP2004352605A (en) * 2003-05-01 2004-12-16 Toray Ind Inc Method for refining composition comprising carbon nanotube
JP2005004967A (en) 2003-06-09 2005-01-06 Toyota Motor Corp Electrode for fuel cell, its manufacturing method, and solid polymer type fuel cell equipped with it
EP1652815A1 (en) * 2003-07-18 2006-05-03 Norio Akamatsu Carbon nanotube manufacturing apparatus and method for manufacturing carbon nanotube
JP4977945B2 (en) 2003-12-18 2012-07-18 トヨタ自動車株式会社 Membrane electrode assembly, method for producing the same, and fuel cell
US20100062229A1 (en) * 2004-07-27 2010-03-11 Kenji Hata Aligned single-walled carbon nanotube aggregate, bulk aligned single-walled carbon nanotube aggregate, powdered aligned single-walled carbon nanotube aggregate, and production method thereof
JP2006196413A (en) * 2005-01-17 2006-07-27 Canon Inc Membrane electrode junction for fuel cell, its manufacturing method, and fuel cell
JP2006228502A (en) * 2005-02-16 2006-08-31 Mitsui Chemicals Inc Electrode catalyst for fuel cell, its manufacturing method, and electrode and fuel cell using the same
JP4702735B2 (en) * 2005-02-16 2011-06-15 国立大学法人山梨大学 Manufacturing method of gas diffusion layer for fuel cell
WO2006090464A1 (en) * 2005-02-24 2006-08-31 Octec, Inc. Solid polymer fuel cell and method for producing same
JP2007173109A (en) * 2005-12-22 2007-07-05 Canon Inc Membrane-electrode conjugate for fuel cell, its manufacturing method, and fuel cell
JP5019905B2 (en) * 2007-02-22 2012-09-05 旭化成株式会社 Fuel cell electrode and fuel cell using the electrode
JP2009129853A (en) * 2007-11-27 2009-06-11 Toyota Central R&D Labs Inc Membrane electrode assembly, manufacturing method thereof, and solid polymer fuel cell
EP2098484A1 (en) * 2008-02-15 2009-09-09 Imec Synthesis of zeolite crystals and formation of carbon nanostructures in patterned structures

Patent Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6890506B1 (en) * 2001-04-12 2005-05-10 Penn State Research Foundation Method of forming carbon fibers
US20040224217A1 (en) * 2003-05-08 2004-11-11 Toops Todd Jefferson Integrated membrane electrode assembly using aligned carbon nanotubules
WO2005035841A2 (en) * 2003-10-10 2005-04-21 Board Of Regents, The University Of Texas System Carbon nanostructure-based electrocatalytic electrodes
US20060269827A1 (en) * 2005-05-26 2006-11-30 The University Of Chicago Method of fabricating electrode catalyst layers with directionally oriented carbon support for proton exchange membrane fuel cell
US20100075201A1 (en) * 2006-03-20 2010-03-25 Haruyuki Nakanishi Fuel cell with electrode having an electrically conductive nano-column and production method thereof
WO2008115753A2 (en) * 2007-03-16 2008-09-25 Honda Motor Co., Ltd. Method of preparing carbon nanotube containing electrodes

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
ELIZABETH J BIDDINGER ET AL: "Nitrogen-Containing Carbon Nanostructures as Oxygen-Reduction Catalysts", TOPICS IN CATALYSIS, KLUWER ACADEMIC PUBLISHERS-PLENUM PUBLISHERS, NE, vol. 52, no. 11, 28 April 2009 (2009-04-28), pages 1566 - 1574, XP019734224, ISSN: 1572-9028, DOI: 10.1007/S11244-009-9289-Y *

Also Published As

Publication number Publication date
WO2011128760A2 (en) 2011-10-20
US9203101B2 (en) 2015-12-01
EP2559086B1 (en) 2014-08-20
EP2559086A2 (en) 2013-02-20
JP2011222378A (en) 2011-11-04
JP5093288B2 (en) 2012-12-12
US20130020280A1 (en) 2013-01-24

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