JP6255222B2 - 金属酸化物−ポリマー積層体およびその製造方法 - Google Patents
金属酸化物−ポリマー積層体およびその製造方法 Download PDFInfo
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- JP6255222B2 JP6255222B2 JP2013244625A JP2013244625A JP6255222B2 JP 6255222 B2 JP6255222 B2 JP 6255222B2 JP 2013244625 A JP2013244625 A JP 2013244625A JP 2013244625 A JP2013244625 A JP 2013244625A JP 6255222 B2 JP6255222 B2 JP 6255222B2
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- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C24/00—Coating starting from inorganic powder
- C23C24/02—Coating starting from inorganic powder by application of pressure only
- C23C24/04—Impact or kinetic deposition of particles
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- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C14/00—Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
- C23C14/22—Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material characterised by the process of coating
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D1/00—Processes for applying liquids or other fluent materials
- B05D1/02—Processes for applying liquids or other fluent materials performed by spraying
- B05D1/08—Flame spraying
- B05D1/10—Applying particulate materials
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D1/00—Processes for applying liquids or other fluent materials
- B05D1/02—Processes for applying liquids or other fluent materials performed by spraying
- B05D1/12—Applying particulate materials
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C14/00—Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
- C23C14/06—Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material characterised by the coating material
- C23C14/08—Oxides
- C23C14/083—Oxides of refractory metals or yttrium
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C14/00—Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
- C23C14/58—After-treatment
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D2201/00—Polymeric substrate or laminate
- B05D2201/02—Polymeric substrate
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D2201/00—Polymeric substrate or laminate
- B05D2201/04—Laminate
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D2201/00—Polymeric substrate or laminate
- B05D2201/04—Laminate
- B05D2201/06—Laminate of which the last layer is not a polymer
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T428/00—Stock material or miscellaneous articles
- Y10T428/249921—Web or sheet containing structurally defined element or component
- Y10T428/249953—Composite having voids in a component [e.g., porous, cellular, etc.]
- Y10T428/249986—Void-containing component contains also a solid fiber or solid particle
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T428/00—Stock material or miscellaneous articles
- Y10T428/249921—Web or sheet containing structurally defined element or component
- Y10T428/249953—Composite having voids in a component [e.g., porous, cellular, etc.]
- Y10T428/249987—With nonvoid component of specified composition
- Y10T428/24999—Inorganic
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T428/00—Stock material or miscellaneous articles
- Y10T428/25—Web or sheet containing structurally defined element or component and including a second component containing structurally defined particles
- Y10T428/256—Heavy metal or aluminum or compound thereof
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- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Mechanical Engineering (AREA)
- Metallurgy (AREA)
- Organic Chemistry (AREA)
- Laminated Bodies (AREA)
- Other Surface Treatments For Metallic Materials (AREA)
- Physical Vapour Deposition (AREA)
Description
ポリマー層2aとして、4フッ化エチレン樹脂多孔質膜(PTFE:「TEMISH」、7cm×7cm、厚み80μm、日東電工社製)を用意した。
ジルコニア粉末の凝集体の平均粒子径(メジアン径)を表1のように変更した以外は、実施例1と同様にして、金属酸化物−ポリマー積層体1を得た。結果を表1に示す。
ポリマー層2として、ポリプロピレン不織布(PP:商品名「HOP60HCF」、日東電工社製、7cm×7cm、厚み200μm、熱ラミネート法)を用意した以外は、実施例1と同様にして、金属酸化物層3(5cm×5cm、厚み20.6μm)がポリマー層2aの表面(平面視略中央部)に金属酸化物層3の厚み方向の一部が埋設された金属酸化物−ポリマー積層体1を得た。結果を表2に示す。
ジルコニア粉末の凝集体の平均粒子径(メジアン径)を表2のように変更した以外は、実施例1と同様にして、金属酸化物−ポリマー積層体1を得た。結果を表2に示す。
セリア粉末(一次粒子の平均粒子径50nm)を800℃、3時間加熱して、セリア粉末の凝集体(メジアン径3μm)を作製し、この凝集体を使用した以外は、実施例5と同様にして、金属酸化物層3(5cm×5cm、厚み17μm)がポリマー層2aの表面(平面視略中央部)に金属酸化物層3の厚み方向の一部が埋設された金属酸化物−ポリマー積層体1を得た。結果を表3に示す。
セリア粉末の凝集体の平均粒子径(メジアン径)を表3のように変更した以外は、実施例9と同様にして、金属酸化物−ポリマー積層体1を得た。結果を表3に示す。なお、実施例10では、セリア粉末を1050℃で0.5時間加熱することにより、セリア粉末の凝集体の平均粒子径を調整した。
ジルコニア粉末の1次粒子粉末(平均粒子径0.2μm)10gを溶媒(1−メチル−2−ピロリドン)44gに分散させ、さらにバインダーとしてポリフッ化ビニリデンを2.5質量%となるように配合して、ジルコニア分散液を調製した。
ジルコニア粉末の1次粒子粉末を、実施例1で使用したジルコニア粉末の凝集体(メジアン径2μm)に変更した以外は、比較例1と同様にして、ジルコニア分散液を、フッ化エチレン樹脂多孔質膜の表面に、スピンコート法により積層させ、乾燥させた。
各実施例および各比較例の金属酸化物−ポリマー積層体1を、超音波洗浄器の浴槽に配置し、室温(25℃)の水中において、3分間、超音波洗浄器を作動させた。
2 ポリマー層
3 金属酸化物層
Claims (4)
- 多孔質層であるポリマー層と、
前記ポリマー層の表面に積層され、金属酸化物粒子の凝集体を用いてエアロゾルデポジション法により形成される金属酸化物層とを備え、
前記金属酸化物層の少なくとも一部が、厚み方向において、前記ポリマー層に埋設されていることを特徴とする、金属酸化物−ポリマー積層体。 - 前記ポリマー層が、4フッ化エチレン樹脂多孔質膜であることを特徴とする、請求項1に記載の金属酸化物−ポリマー積層体。
- 前記金属酸化物粒子の凝集体のメジアン径が、0.5μm以上10μm以下であることを特徴とする、請求項1または2に記載の金属酸化物−ポリマー積層体。
- 多孔質層であるポリマー層を用意する工程、および、
前記ポリマー層の表面に、少なくとも一部が厚み方向において前記ポリマー層に埋設されるように、金属酸化物層を金属酸化物粒子の凝集体を用いてエアロゾルデポジション法により形成する工程
を備えることを特徴とする、金属酸化物−ポリマー積層体の製造方法。
Priority Applications (6)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
JP2013244625A JP6255222B2 (ja) | 2013-11-27 | 2013-11-27 | 金属酸化物−ポリマー積層体およびその製造方法 |
CN201410674343.6A CN104669733A (zh) | 2013-11-27 | 2014-11-21 | 金属氧化物-聚合物层叠体和其制造方法 |
EP14194470.2A EP2878703A1 (en) | 2013-11-27 | 2014-11-24 | Metal oxide-polymer laminate and production method thereof |
US14/553,286 US20150147565A1 (en) | 2013-11-27 | 2014-11-25 | Metal oxide-polymer laminate and production method thereof |
KR1020140166056A KR20150061589A (ko) | 2013-11-27 | 2014-11-26 | 금속 산화물-폴리머 적층체 및 그의 제조 방법 |
US15/209,944 US10415132B2 (en) | 2013-11-27 | 2016-07-14 | Metal oxide-polymer laminate and production method thereof |
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JP2013244625A JP6255222B2 (ja) | 2013-11-27 | 2013-11-27 | 金属酸化物−ポリマー積層体およびその製造方法 |
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JP2015101042A JP2015101042A (ja) | 2015-06-04 |
JP6255222B2 true JP6255222B2 (ja) | 2017-12-27 |
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US (2) | US20150147565A1 (ja) |
EP (1) | EP2878703A1 (ja) |
JP (1) | JP6255222B2 (ja) |
KR (1) | KR20150061589A (ja) |
CN (1) | CN104669733A (ja) |
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CN109153226B (zh) * | 2016-05-16 | 2021-04-20 | 国立研究开发法人产业技术综合研究所 | 层叠结构体及其制作方法 |
US9872399B1 (en) * | 2016-07-22 | 2018-01-16 | International Business Machines Corporation | Implementing backdrilling elimination utilizing anti-electroplate coating |
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Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JPS59145219A (ja) * | 1983-02-04 | 1984-08-20 | Nippon Pillar Packing Co Ltd | 四弗化エチレン樹脂の表面処理方法 |
US6004667A (en) * | 1994-06-30 | 1999-12-21 | Shinshu Ceramics Company, Ltd. | Low temperature melt injected anti-microbial films, articles containing such films and methods of manufacture and use thereof |
US6531187B2 (en) | 1999-04-23 | 2003-03-11 | Agency Of Industrial Science And Technology | Method of forming a shaped body of brittle ultra fine particles with mechanical impact force and without heating |
JP3265481B2 (ja) * | 1999-04-23 | 2002-03-11 | 独立行政法人産業技術総合研究所 | 脆性材料超微粒子成形体の低温成形法 |
US20020110682A1 (en) * | 2000-12-12 | 2002-08-15 | Brogan Jeffrey A. | Non-skid coating and method of forming the same |
KR100531295B1 (ko) * | 2003-07-16 | 2005-11-28 | 엘지전자 주식회사 | 단판식 프로젝션 디바이스 |
JP2005274260A (ja) * | 2004-03-24 | 2005-10-06 | Fuji Photo Film Co Ltd | 放射線撮像パネルを構成する光導電層の製造方法 |
DE102004038795B4 (de) * | 2004-08-09 | 2007-07-19 | Atg- Advanced Technology Group S.R.O. | Verfahren zur Herstellung photokatalytisch aktiver Polymere |
JP2006128229A (ja) | 2004-10-26 | 2006-05-18 | Murata Mfg Co Ltd | 複合多層基板 |
US20070110919A1 (en) * | 2005-11-15 | 2007-05-17 | ATG Advanced Technology Group s.r.o. | Method for producing photocatalytically active polymers |
US7547393B2 (en) | 2005-12-07 | 2009-06-16 | General Electric Company | Membrane structure and method of making |
JP5401805B2 (ja) * | 2008-02-29 | 2014-01-29 | 富士通株式会社 | 成膜方法 |
JP2009301825A (ja) * | 2008-06-12 | 2009-12-24 | Panasonic Corp | 非水電解質二次電池およびそれに用いられる電極、ならびにこれらの製造方法 |
JP5252380B2 (ja) * | 2008-07-14 | 2013-07-31 | Toto株式会社 | 複合構造物及びその作製方法 |
US8247050B2 (en) * | 2009-06-02 | 2012-08-21 | Integran Technologies, Inc. | Metal-coated polymer article of high durability and vacuum and/or pressure integrity |
EP2501466A4 (en) * | 2009-11-11 | 2016-08-17 | Nano Nouvelle Pty Ltd | POROUS MATERIALS |
KR101497854B1 (ko) * | 2010-12-15 | 2015-03-04 | 유겐가이샤 후치타 나노 기켄 | 성막 방법 |
US20120237789A1 (en) * | 2011-02-15 | 2012-09-20 | Integran Technologies Inc. | High yield strength lightweight polymer-metal hybrid articles |
JP2012216684A (ja) | 2011-03-31 | 2012-11-08 | Nippon Zeon Co Ltd | 複合多層基板 |
CN103551171A (zh) * | 2013-10-23 | 2014-02-05 | 三棵树涂料股份有限公司 | 磷酸铝包裹的光催化纳米二氧化钛粉末及其应用 |
-
2013
- 2013-11-27 JP JP2013244625A patent/JP6255222B2/ja not_active Expired - Fee Related
-
2014
- 2014-11-21 CN CN201410674343.6A patent/CN104669733A/zh active Pending
- 2014-11-24 EP EP14194470.2A patent/EP2878703A1/en not_active Withdrawn
- 2014-11-25 US US14/553,286 patent/US20150147565A1/en not_active Abandoned
- 2014-11-26 KR KR1020140166056A patent/KR20150061589A/ko not_active Application Discontinuation
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2016
- 2016-07-14 US US15/209,944 patent/US10415132B2/en not_active Expired - Fee Related
Also Published As
Publication number | Publication date |
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EP2878703A1 (en) | 2015-06-03 |
US20160319420A1 (en) | 2016-11-03 |
CN104669733A (zh) | 2015-06-03 |
US10415132B2 (en) | 2019-09-17 |
US20150147565A1 (en) | 2015-05-28 |
JP2015101042A (ja) | 2015-06-04 |
KR20150061589A (ko) | 2015-06-04 |
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