HRP20150081T1 - Nove smjese za premaz radi kontrole obraštanja - Google Patents

Nove smjese za premaz radi kontrole obraštanja Download PDF

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Publication number
HRP20150081T1
HRP20150081T1 HRP20150081TT HRP20150081T HRP20150081T1 HR P20150081 T1 HRP20150081 T1 HR P20150081T1 HR P20150081T T HRP20150081T T HR P20150081TT HR P20150081 T HRP20150081 T HR P20150081T HR P20150081 T1 HRP20150081 T1 HR P20150081T1
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coating mixture
mixture according
polysiloxane
biocides
coating
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HRP20150081TT
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English (en)
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Peter Christian Weinrich Thorlaksen
Anders Blom
Ulrik Bork
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Hempel A/S
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Publication of HRP20150081T1 publication Critical patent/HRP20150081T1/hr
Publication of HRP20150081T8 publication Critical patent/HRP20150081T8/hr

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    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
    • C09D5/16—Antifouling paints; Underwater paints
    • C09D5/1656—Antifouling paints; Underwater paints characterised by the film-forming substance
    • C09D5/1662—Synthetic film-forming substance
    • C09D5/1675—Polyorganosiloxane-containing compositions
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04—Polysiloxanes
    • C08G77/14—Polysiloxanes containing silicon bound to oxygen-containing groups
    • C08G77/16—Polysiloxanes containing silicon bound to oxygen-containing groups to hydroxyl groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/42—Block-or graft-polymers containing polysiloxane sequences
    • C08G77/46—Block-or graft-polymers containing polysiloxane sequences containing polyether sequences
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D183/00—Coating compositions based on macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon, with or without sulfur, nitrogen, oxygen, or carbon only; Coating compositions based on derivatives of such polymers
    • C09D183/04—Polysiloxanes
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
    • C09D5/14—Paints containing biocides, e.g. fungicides, insecticides or pesticides
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
    • C09D5/16—Antifouling paints; Underwater paints
    • C09D5/1606—Antifouling paints; Underwater paints characterised by the anti-fouling agent
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D7/00—Features of coating compositions, not provided for in group C09D5/00; Processes for incorporating ingredients in coating compositions
    • C09D7/40—Additives
    • C09D7/65—Additives macromolecular
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/02—Polysilicates
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/56—Organo-metallic compounds, i.e. organic compounds containing a metal-to-carbon bond
    • C08K5/57—Organo-tin compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L51/00—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
    • C08L51/08—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to macromolecular compounds obtained otherwise than by reactions only involving unsaturated carbon-to-carbon bonds
    • C08L51/085—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to macromolecular compounds obtained otherwise than by reactions only involving unsaturated carbon-to-carbon bonds on to polysiloxanes

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Engineering & Computer Science (AREA)
  • Wood Science & Technology (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Polymers & Plastics (AREA)
  • Medicinal Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Plant Pathology (AREA)
  • Paints Or Removers (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)
  • Application Of Or Painting With Fluid Materials (AREA)
  • Polymers With Sulfur, Phosphorus Or Metals In The Main Chain (AREA)

Claims (33)

1. Smjesa za premaz radi kontrole obraštanja naznačena time da sadrži sustav veziva na bazi polisiloksana, 0,01-20% suhe mase jednog ili više hidrofilno modificiranih polisiloksana, te jednog ili više biocida, pri čemu je maseni omjer između jednog ili više hidrofilno modificiranih polisiloksana i jednog ili više biocida u rasponu od 1:0,2 do 1:6, i pri čemu jedan ili više hidrofilno modificiranih polisiloksana ne sadrže skupine koje mogu reagirati s vezivom ili bilo kojim sredstvom za poprečno povezivanje.
2. Smjesa za premaz prema patentnom zahtjevu 1, naznačena time da je relativni maseni omjer između jednog ili više hidrofilno modificiranih polisiloksana i jednog ili više biocida od 1:0,2 do 1:4.
3. Smjesa za premaz prema patentnom zahtjevu 2, naznačena time da je relativni maseni omjer između jednog ili više hidrofilno modificiranih polisiloksana i jednog ili više biocida 1:0,25 do 1:4.
4. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da jedan ili više hidrofilno modificiranih polisiloksana čine 0,05-10% suhe mase smjese za premaz.
5. Smjesa za premaz prema patentnom zahtjevu 4, naznačena time da jedan ili više hidrofilno modificiranih polisiloksana čine 2-7% suhe mase smjese za premaz.
6. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da jedan ili više biocida čine 0.1-10% suhe mase smjese za premaz.
7. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da je najmanje jedan biocid organski biocid.
8. Smjesa za premaz prema patentnom zahtjevu 7, naznačena time da je jedan ili više biocida odabrano iz 3-(3,4-diklorfenil)-1,1-dimetilureje (diurona), N2-terc-butil-N4-ciklopropil-6-metiltio-1,3,5-triazin-2,4-diamina (cibutrina), 4,5-dikloro-2-n-oktil-4-izotiazolin-3-ona (DCOIT, Sea-Nine® 211N), bis(1-hidroksi-2(1H)-piridinetionato-O,S)-(T-4) cinka (cinkovog piridinetionata, cinkovog piritiona), bis(1-hidroksi-2(1H)- piridinetionata-O, S)-T-4) bakra (bakrovog piridinetiona, bakrovog piritiona) i cinkovog etilen-1,2-bis-ditiokarbamata (cink-etilen-N-N'-ditiokarbamata, zineba).
9. Smjesa za premaz prema patentnom zahtjevu 8, naznačena time da je jedan ili više biocida odabrano iz cinkovog piritiona, bakrovog piritiona i 4,5-diklor-2-n-oktil-4-izotiazolin-3-ona (DCOIT, Sea-Nine® 211N).
10. Smjesa za premaz prema bilo kojem od patentnih zahtjeva 7-9, naznačena time da je barem jedan biocid pirition kompleks.
11. Smjesa za premaz prema bilo kojem od patentnih zahtjeva 7-10, naznačena time da je jedan ili više biocida pirition kompleks.
12. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da hidrofilne skupine imaju prosječnu brojčanu molekulsku masu (Mn) u rasponu od 400-10.000 g/mol.
13. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da hidrofilno modificirani polisiloksan ima prosječnu brojčanu molekulsku masu (Mn) u rasponu od 500-50.000 g/mol.
14. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da je relativna masa hidrofilnih dijelova iz jednog ili više hidrofilno modificiranih polisiloksana 10-70% ukupne mase hidrofilno modificiranog polisiloksana.
15. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da sustav veziva na bazi polisiloksana čini najmanje 40% suhe mase smjese za premaz.
16. Smjesa za premaz prema patentnom zahtjevu 15, naznačena time da sustav veziva na bazi polisiloksana čini 50-90% suhe mase smjese za premaz.
17. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da sustav veziva na bazi polisiloksana čini najmanje 40% suhe mase smjese za premaz, pri čemu hidrofilno modificirani polisiloksani čine 0,05-10% suhe mase smjese za premaz pri čemu je navedeni hidrofilno modificirani polisiloksan poli(oksialkilen)-modificirani polisiloksan i pri čemu jedan ili više biocida čine 0.1-10% suhe mase smjese za premaz, pri čemu navedena smjesa za premaz ima viskoznost u rasponu od 200-4.000 mPa·s mjereno na 25 °C u skladu s normom ISO 2555:1989, te pri čemu navedena smjesa za premaz sadrži i pigmente i/ili punila u količini od 0-35% suhe mase smjese za premaz.
18. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da sadrži: (i) 40-70% mokre mase ukupne smjese za vanjski premaz polidiorganosiloksana koji završava sa silanol skupinama i sredstva za poprečno povezivanje; (ii) 0.1-10 % mokre mase ukupne smjese za vanjski premaz jednog ili više biocida, poželjno odabranih iz organskih biocida; i (iii) 0.1-10 % mokre mase ukupne smjese za vanjski premaz jednog ili više hidrofilno modificiranih polisiloksana odabranih iz poli(oksialkilen)-modificiranih polisiloksana.
19. Smjesa za premaz prema jednom od prethodno navedenih zahtjeva, naznačena time da je vezivo na bazi polisiloksana funkcionalni organopolisiloksan s terminalnom i/ili postojećom funkcionalnošću, pri čemu je navedena funkcionalnost hidrolizirajuća skupina ili silanolna skupina.
20. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da vezivni sustav na bazi polisiloksana sadrži (i), vezivo te (ii) sredstvo za poprečno povezivanje, pri čemu vezivo (i) čini 20-90% suhe mase smjese za premaz, te je diorganopolisiloksan koji se upotrebljava u liječenju i koji je predstavljen općom formulom (1): [image] pri čemu je svaki A1 nezavisno odabran iz hidroksilne skupine, hidrolizirajuće skupine, amino skupine i epoksi skupine; svaki A2 nezavisno odabran između alkilne, arilne, alkenilne i hidrolizirajuće skupine; svaki A3 i A4 nezavisno odabran između alkilnog i arilnog alkenila; i pri čemu je a= 1-25.000, b = 1-2.500, te je a + b najmanje 30.
21. Smjesa za premaz prema bilo kojem od patentnih zahtjeva 19-20, naznačena time da organopolisiloksan ima terminalne ili epoksi ili amino skupine, kao i postojeće hidrolizirajuće skupine s alkoksi funkcionalnošću.
22. Smjesa za premaz prema bilo kojem od patentnih zahtjeva 19-21, naznačena time da je navedena hidrolizirajuća skupina odabrana iz alkoksi skupine ili ketoksim skupine.
23. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da vezivo na bazi polisiloksana sadrži vezivo na bazi polidimetilsiloksana.
24. Smjesa za premaz prema jednom od prethodno navedenih patentnih zahtjeva, naznačena time da sustav veziva sadrži sredstvo za poprečno povezivanje odabrano iz tetraetoksisilana; viniltris(metiletiloksimo)silana; metiltris(metiletiloksimo)silana; viniltrimetoksisilana; metiltrimetoksisilana i viniltriizopropenoksisilana; te njihovih proizvoda nastalih hidrolizom i kondenzacijom.
25. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da se hidrofilni karakter jednog ili više hidrofilno modificiranih polisiloksana dobiva dodavanjem oligomernih ili polimernih skupina odabranih iz amida, kiselina, alkohola, ketona, aldehida, amina, estera, etera i imida, uključujući njihove kopolimere.
26. Smjesa za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva, naznačena time da je hidrofilno modificirani polisiloksan zapravo poli(oksialkilen)-modificirani polisiloksan.
27. Smjesa za premaz prema patentnom zahtjevu 26, naznačena time da je poli(oksialkilen)-modificirani polisiloksan zapravo polisiloksan koji sadrži poli(oksialkilenske) lance.
28. Smjesa za premaz prema patentnom zahtjevu 26, naznačena time da je poli(oksialkilen)-modificirani polisiloksan zapravo polisiloksan koji u svojoj srži ima ugrađene poli(oksialkilenske) lance.
29. Smjesa za premaz prema patentnom zahtjevu 26, naznačena time da je poli(oksialkilen)-modificiarni polisiloksan zapravo polisiloksan koji u svojoj srži ima ugrađene poli(oksialkilenske) lance i koji sadrži poli(oksialkilenske) lance.
30. Smjesa za premaz prema bilo kojem od patentnih zahtjeva 17-18 i 25-29, naznačena time da je poli(oksialkilen) odabran između polioksietilena, polioksipropilena i poli(oksietilen-ko-oksipropilena).
31. Morska struktura naznačena time da sadrži barem dio vanjske površine i krajnji vanjski sloj dobiven iz smjese za premaz prema bilo kojem od prethodno navedenih patentnih zahtjeva.
32. Struktura prema patentnom zahtjevu 31, naznačena time da je barem dio vanjske površine koja nosi krajnji vanjski sloj uronjeni dio spomenute strukture.
33. Upotreba kombinacije jednog ili više nereaktivnih hidrofilno modificiranih polisiloksana i jednog ili više biocida, naznačena time da je omjer mase između jednog ili više hidrofilno modificiranih polisiloksana i jednog ili više biocida u rasponu od 1:0,2 do 1:6, pri čemu jedan ili više hidrofilno modificiranih polisiloksana ne sadrži skupine koje mogu reagirati s vezivom ili bilo kojim sredstvom za poprečno povezivanje, radi poboljšanja antivegetativnih svojstava smjese za premaz na bazi polisiloksana.
HRP20150081TT 2009-12-22 2015-01-22 Nove smjese za premaz radi kontrole obraštanja HRP20150081T8 (hr)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
EP09180360 2009-12-22
EP10792948.1A EP2516559B1 (en) 2009-12-22 2010-12-22 Novel fouling control coating compositions
PCT/EP2010/070509 WO2011076856A1 (en) 2009-12-22 2010-12-22 Novel fouling control coating compositions

Publications (2)

Publication Number Publication Date
HRP20150081T1 true HRP20150081T1 (hr) 2015-05-08
HRP20150081T8 HRP20150081T8 (hr) 2015-07-03

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US (1) US9534121B2 (hr)
EP (1) EP2516559B1 (hr)
JP (2) JP5990462B2 (hr)
KR (2) KR101798604B1 (hr)
CN (2) CN105368311B (hr)
BR (1) BR112012015153A2 (hr)
DK (1) DK2516559T3 (hr)
ES (1) ES2528606T3 (hr)
HR (1) HRP20150081T8 (hr)
PL (1) PL2516559T3 (hr)
PT (1) PT2516559E (hr)
SG (1) SG181914A1 (hr)
WO (1) WO2011076856A1 (hr)

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