JP5263928B2 - Square battery - Google Patents
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- JP5263928B2 JP5263928B2 JP2007326003A JP2007326003A JP5263928B2 JP 5263928 B2 JP5263928 B2 JP 5263928B2 JP 2007326003 A JP2007326003 A JP 2007326003A JP 2007326003 A JP2007326003 A JP 2007326003A JP 5263928 B2 JP5263928 B2 JP 5263928B2
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/10—Energy storage using batteries
Description
本発明は、主として、リチウムイオン二次電池などの高エネルギー密度を有する二次電池の大電流充放電用電源としての用途に適した角型電池に関するものである。 The present invention mainly relates to a prismatic battery suitable for use as a power source for charging and discharging a large current of a secondary battery having a high energy density such as a lithium ion secondary battery.
リチウムイオン二次電池などの、正極集電体の両面に正極活物質を塗布した正極板と、負極集電体の両面に負極活物質を塗布した負極板とが、セパレータを介して積層されてなる極板群には、正極板と負極板とをセパレータを介して交互に積層させ極板群を形成する積層型と、正極板と負極板とをセパレータを介して渦巻き状に積層し極板群を形成する巻回型とがある。一般にはこれら極板群を電解液と共に電池缶に収納し、正極板、負極板の適所に、集電タブや集電リードの片端を接続し、他端を正極端子、負極端子に接続して電気を取り出す構造として電池が構成されている。 A positive electrode plate in which a positive electrode active material is applied to both surfaces of a positive electrode current collector, such as a lithium ion secondary battery, and a negative electrode plate in which a negative electrode active material is applied to both surfaces of a negative electrode current collector are stacked via a separator. In the electrode plate group, a positive electrode plate and a negative electrode plate are alternately stacked via a separator to form a stacked plate, and a positive electrode plate and a negative electrode plate are spirally stacked via a separator. There are winding types that form groups. Generally, these electrode plate groups are housed in a battery can together with an electrolyte, and one end of a current collecting tab or current collecting lead is connected to an appropriate position of the positive electrode plate and the negative electrode plate, and the other end is connected to a positive electrode terminal and a negative electrode terminal. A battery is configured as a structure for extracting electricity.
上記の構造では、正極板、負極板の一箇所から集電タブや集電リードを介して電気を取り出しているので、大電流で充放電を行う場合でも、面積の小さい集電タブや集電リードに電流が流れるだけであるため、電気抵抗が大きくなり発熱することや、電極反応が不均一に発生することが懸念される。その結果、電池の充放電特性が低下することから、長期間に亘る信頼性の向上が要望されている。 In the above structure, electricity is taken out from one place of the positive electrode plate and the negative electrode plate via the current collecting tab or current collecting lead. Therefore, even when charging / discharging with a large current, the current collecting tab or current collecting device with a small area is used. Since only the current flows through the lead, there is a concern that the electrical resistance increases and heat is generated, and the electrode reaction occurs unevenly. As a result, the charge / discharge characteristics of the battery are lowered, and thus there is a demand for improvement in reliability over a long period of time.
また、集電タブや集電リードを電池缶内に納めるにあたり、極性の異なる集電タブや集電リード相互の接触、あるいは集電タブや集電リードと極性の異なる極板との接触等によって、内部短絡が起こる可能性がある。これらの内部短絡を防ぐためには、絶縁板を組み込む等の構造が必要となり、体積容積密度を向上させることが困難となっている。 Also, when the current collecting tab or current collecting lead is placed in the battery can, the current collecting tabs or current collecting leads with different polarities, or the current collecting tab or current collecting lead with the electrode plate with different polarity, etc. Internal short circuit may occur. In order to prevent these internal short circuits, a structure such as an insulating plate is required, and it is difficult to improve the volumetric volume density.
一方、例えば特許文献1に開示されているように、集電タブや集電リードを用いず、極板群の両側面から集電体を突出させ、直接集電板に接続するタブレス方式が提案されている。この方式は、正極板、負極板それぞれの極板全体から均一に集電でき、大電流の充放電に適しているという特徴がある。また、集電タブや集電リードの折りたたみや絶縁板を組み込むなどの工程が不要となり、構造を単純化できるという利点がある。
On the other hand, as disclosed in
タブレス方式は、極性群の両側面から突出した集電体同士がそれぞれ集電板に直接接続されている構造であるが、側面に極性の異なる集電体が露出したままの状態では、その露出部分が異極の集電体に接触することで内部短絡が発生する可能性がある。また、集電体と集電板とを密着させ接続する場合に、集電体と集電板の接触面積が小さいと接続箇所の強度が不十分となり、弱い衝撃でも接続が壊れる恐れがある。集電体と集電板とを確実に接続するためには、集電体と集電板との接触面積を大きくする必要がある。 The tabless system is a structure in which current collectors protruding from both sides of the polar group are directly connected to the current collector plates, but if the current collectors of different polarity are left exposed, There is a possibility that an internal short circuit may occur when the part contacts a current collector with a different polarity. Further, when the current collector and the current collector plate are connected in close contact with each other, if the contact area between the current collector and the current collector plate is small, the strength of the connection portion becomes insufficient, and the connection may be broken even with a weak impact. In order to reliably connect the current collector and the current collector plate, it is necessary to increase the contact area between the current collector and the current collector plate.
本発明は、上述の問題を解決すべくなされたもので、その技術的課題は、内部短絡の発生を防止でき、且つ極板群の両側面から突出させた集電体と集電板を確実に接続し、安全性、信頼性の高い角型電池を提供することである。 The present invention has been made to solve the above-mentioned problems, and its technical problem is that it is possible to prevent the occurrence of an internal short circuit and to ensure the current collector and the current collector plate protruding from both side surfaces of the electrode plate group. To provide a prismatic battery with high safety and reliability.
本発明の角型電池は、正極集電体の両面に正極活物質を塗布した正極板と、負極集電体の両面に負極活物質を塗布した負極板とがセパレータを介して積層構造を形成した極板群を、電解液と共に電池缶に収納されてなる角型電池であって、前記極板群の両側面に接するように設けられた絶縁体と、前記正極集電体の端部と前記負極集電体の端部とが前記両側面から前記絶縁体を通して互いに逆方向に突出し、該突出した端部が同極同士で接合されて輪状に形成された集電体接合部と、前記集電体接合部にそれぞれ密着して接続された正極集電板および負極集電板であって、外部端子との導通を確保するための正極集電板および負極集電板と、を有することを特徴とする角型電池が得られる。この構造を採用することによって、異極の集電体相互の接触による内部短絡を防止でき、また、集電体と集電板との接触面積が大きくなり、確実な接合が得られる。 In the prismatic battery of the present invention, a positive electrode plate in which a positive electrode active material is applied to both surfaces of a positive electrode current collector and a negative electrode plate in which a negative electrode active material is applied to both surfaces of a negative electrode current collector form a laminated structure via a separator. the the electrode plate group, a prismatic cell comprising housed in a battery can together with an electrolyte, an insulator provided in contact with both sides of the electrode plate assembly, an end portion of the positive electrode current collector the negative electrode current collector and the end protruding in opposite directions to each other through the insulator from the both sides, the collector junction end issued projecting are formed on the ring are joined with the same poles, a positive electrode current collector plate and the negative electrode current collector plate that is connected in close contact to each of the current collector junction, having a positive electrode and negative electrode terminal plates to ensure conduction between the external terminal A square battery characterized by the above can be obtained. By adopting this structure, it is possible to prevent an internal short circuit due to contact between current collectors of different polarities, and the contact area between the current collector and the current collector plate is increased, so that reliable bonding can be obtained.
また、前記極板群両側面に設けた絶縁体に、前期集電板に向けて絶縁突起部を形成し、前記集電体接合部は、前記絶縁突起部を覆うように当接させることで、集電体と集電板との接続を保持することを特徴とする角型電池が得られる。 Further, an insulating protrusion is formed on the insulator provided on both side surfaces of the electrode plate group toward the current collector plate, and the current collector joint is brought into contact so as to cover the insulating protrusion. A prismatic battery characterized in that the connection between the current collector and the current collector plate is maintained.
また、前記集電板に前記集電体接合部を挟み込む手段を有する挟持部材を設置し、前記狭持部材に前記集電体接合部を挿入し挟み込んで固定することにより、集電体と集電板との接続を保持することを特徴とする角型電池が得られる。 In addition, a clamping member having means for sandwiching the current collector joint portion between the current collector plates is installed, and the current collector joint portion is inserted into the sandwiching member and sandwiched and fixed, thereby fixing the current collector and the current collector. A prismatic battery characterized by maintaining connection with the electric plate can be obtained.
また、前記集電板を櫛歯形状とし、前記集電体接合部と前記集電板とを交差させ、集電体と集電板との接続を保持することを特徴とする角型電池が得られる。 A rectangular battery characterized in that the current collector plate has a comb shape, the current collector junction and the current collector plate are crossed, and the connection between the current collector and the current collector plate is maintained. can get.
また、前記集電体接合部と前記集電板とを溶接にて接続したことを特徴とする角型電池が得られる。 Moreover, the square battery characterized by connecting the said collector collector part and the said current collector plate by welding is obtained.
本発明によれば、体積容積効率が高く大電流充放電に適したタブレス方式の角型電池において、内部短絡発生を防止できる構造で、かつ集電板と集電体とを確実に接続する、安全性、信頼性の高い角型電池を提供することができる。 According to the present invention, in a tabless type prismatic battery that is high in volumetric volume efficiency and suitable for large current charge / discharge, it has a structure that can prevent the occurrence of an internal short circuit, and reliably connects the current collector and the current collector, A prismatic battery with high safety and reliability can be provided.
以下、本発明の角型電池の一実施の形態のリチウムイオン二次電池について、図面を参照しながら詳細に説明するが、本発明はこれらの実施の形態に限定されるものではない。 Hereinafter, a lithium ion secondary battery according to an embodiment of the square battery of the present invention will be described in detail with reference to the drawings, but the present invention is not limited to these embodiments.
図1は、本発明の第1の実施の形態に関わる角型電池の縦断面図である。この図では電池缶と電解液は省略されている。 FIG. 1 is a longitudinal sectional view of a prismatic battery according to the first embodiment of the present invention. In this figure, the battery can and the electrolyte are omitted.
正極板3は、アルミニウム製の正極集電体1の両面にリチウム含有遷移金属酸化物などの正極活物質2が塗布されたシートであり、負極板6は、銅製の負極集電体4の両面に黒鉛などの負極活物質5が塗布されたシートである。各極板の片端部には一定幅で両面に活物質を塗布せず、各極の集電体が露出した部分を設ける。
The
積層型電池の場合は、上記正極板3と負極板6をセパレータ9を介して所定の数量になるように積層し極板群を形成する。また、巻回型電池の場合は、上記正極板3と負極板6をセパレータ9を介して渦巻状に所定の巻き数になるように巻きつけ極板群を形成する。このとき各極板の集電体が露出した端部は、正極、負極で互いに逆方向になるように配置する。セパレータ9の材質としては、例えばポリエチレン、ポリプロピレンなどのオレフィン系ポリマーや、ガラス繊維などからなる織布や不織布などを用いることができる。
In the case of a stacked battery, the
次いで、上記極板群の各極板の集電体が露出した端部を除く両側面に、絶縁体10を形成し、各極板の集電体が露出した端部は、絶縁体10から突出させるような構造とする。この構造により、絶縁体10から突出した集電体突出部は、異極の極板と接触することが無く、内部短絡の発生を防止でき、より安全性、信頼性の高い電池を提供することが可能となる。絶縁体の材質としては、加熱やUV照射により重合固化して得られるポリマー等が好適に用いられる。
Next, the
前述の集電体突出部は、同極同士で接合して輪状を形成し、この輪状の集電体接合部と正極集電板7、負極集電板8とをそれぞれ接続させる。このとき、集電体突出部の全面を輪状に接合し、集電体接合部を形成しても良いが、予め集電体突出部の一箇所または複数箇所を矩形状に切断加工しておき、この部分を同極同士で輪状に接合し、所定幅の集電体接合部を形成しても良い。
The current collector projections described above are joined at the same polarity to form a ring shape, and the ring-shaped current collector joint portion is connected to the positive electrode
集電体接合部と集電板との接続は、抵抗溶接またはレーザ溶接などを施すことができるが、この際、接合部分の面積を大きくできるので、接合を強固、確実に保つことが可能である。 The connection between the current collector joint and the current collector plate can be performed by resistance welding or laser welding, but at this time, the area of the joint can be increased, so that the joint can be maintained firmly and securely. is there.
図2は、本発明の第2の実施の形態に関わる角型電池の要部の縦断面図である。この図は、正極集電板側の集電体接合部と極板群の一部を示したもので、その他の部分は省略しているが、正極側と負極側は同様の形態とすることができる。極板群側面の絶縁体に絶縁突起部11を形成して、輪状に接合された集電体接合部を、その絶縁突起部11を覆うように当接させる。この集電体接合部を正極集電板7に押し当て接続させる。この場合に、絶縁突起部11が集電体接合部を支持する構造となるので、正極集電板7と正極集電体1とを容易に接続することが可能となる。なお、絶縁突起部11の形状は図2に示したものに限定はせず、集電体接合部と集電板との接続を支持するものであれば、他の形状でも同様の効果が得られる。
FIG. 2 is a longitudinal cross-sectional view of the main part of the prismatic battery according to the second embodiment of the present invention. This figure shows the current collector joint on the positive electrode current collector plate side and a part of the electrode plate group, and other parts are omitted, but the positive electrode side and the negative electrode side have the same configuration. Can do. An
図3は、本発明の第3の実施の形態に関わる角型電池の集電板に設けた狭持部材の形状の一例を示す図で、図3(a)は狭持部材と集電体との接続形態を示す説明図で、図3(b)は図3(a)を矢印13の方向から見た説明図である。この図は、正極集電板側の極板群の一部を示したもので、その他の部分は省略しているが、正極側と負極側は同様の形態とすることができる。正極集電板7に狭持部材12を設置し、この狭持部材12に集電体同士の接合部分を挿入することにより、正極集電板7と正極集電体1とを接続、固定するものである。これによって、集電体接合部と正極集電板7との接続を強固かつ容易に行うことが可能となる。
FIG. 3 is a view showing an example of the shape of the holding member provided on the current collector plate of the prismatic battery according to the third embodiment of the present invention, and FIG. 3 (a) shows the holding member and the current collector. FIG. 3B is an explanatory view of FIG. 3A viewed from the direction of the
図4は、本発明の第3の実施の形態に関わる角型電池の集電板に設けた狭持部材の別の形状を示す説明図である。また狭持部材12の形状は、これらに限定されるものではなく、集電体接合部の挟み込みが可能な機能を有する形状の狭持部材を集電板に設置することで、同様の効果が得られるものである。
FIG. 4 is an explanatory view showing another shape of the holding member provided on the current collector plate of the prismatic battery according to the third embodiment of the present invention. Further, the shape of the holding
図5は、本発明の第4の実施の形態に関わる角型電池の要部を示す図で、図5(a)は、櫛歯形状集電板と集電体との接続形態を示す説明図で、図5(b)は図5(a)の集電体を矢印14の方向から見た説明図である。この図は、正極集電板側の極板群の一部を示したもので、その他の部分は省略しているが、正極側と負極側は同様の形態とすることができる。
FIG. 5 is a diagram showing a main part of a prismatic battery according to the fourth embodiment of the present invention, and FIG. 5 (a) is a diagram showing a connection configuration between a comb-shaped current collector plate and a current collector. FIG. 5B is an explanatory view of the current collector of FIG. 5A viewed from the direction of the
図6は、本発明の第4の実施の形態に関わる角型電池の集電板の形状を示す図で、図6(a)は櫛歯状の集電板を示す図、図6(b)は長方形状の孔を設けた集電板を示す図、図6(c)は櫛歯状に対向するように配置された集電板を示す図、図6(d)は角孔が形成された集電板を示す図である。 FIG. 6 is a diagram showing the shape of a current collecting plate of a prismatic battery according to the fourth embodiment of the present invention, FIG. 6 (a) is a diagram showing a comb-shaped current collecting plate, and FIG. ) Is a diagram showing a current collector plate provided with a rectangular hole, FIG. 6C is a diagram showing a current collector plate arranged so as to be opposed in a comb-tooth shape, and FIG. 6D is a diagram showing a square hole formed. It is a figure which shows the made current collecting plate.
図5において、図6(a)の櫛歯形状の集電体を使用した場合を例にとって説明をする。正極集電板7aを櫛歯形状とし、集電体接合部と正極集電板7aとが交差した構造をとっている。このとき、正極集電体1は予め櫛歯形状の正極集電板7aに交差させておき、その後、正極集電体1を輪状に接合し、集電体接合部を正極集電板7aを覆うように密接させる。この構造により、集電板と集電体との接触面積を十分確保して接続することが可能であることに加え、正極集電板7aは隙間が開いた形状であるので、電解液注入をより容易に行うことができる。
In FIG. 5, the case where the comb-shaped current collector of FIG. 6A is used will be described as an example. The positive electrode
集電板の形状は、図6(b)、図6(c)、図6(d)に示すものでもよく、正極集電体1を正極集電板7b、正極集電板7c、正極集電板7dに交差させ、上記と同様に作製することで、同等の効果を得られる。また、図6(a)や図6(b)の形状の集電板の場合は、先に集電体接合部を形成してから、正極集電板7a、正極集電板7bと交差させることも可能である。なお、集電板の櫛歯の形状や孔の形状は、図6に示したものに限定されるものではなく、正極集電体1と交差する形状であれば、同等の効果が得られる。
The shape of the current collector plate may be as shown in FIGS. 6 (b), 6 (c), and 6 (d). The positive electrode
1 正極集電体
2 正極活物質
3 正極板
4 負極集電体
5 負極活物質
6 負極板
7、7a、7b、7c、7d 正極集電板
8 負極集電板
9 セパレータ
10 絶縁体
11 絶縁突起部
12 狭持部材
13、14 矢印
DESCRIPTION OF
Claims (5)
前記極板群の両側面に接するように設けられた絶縁体と、
前記正極集電体の端部と前記負極集電体の端部とが前記両側面から前記絶縁体を通して互いに逆方向に突出し、該突出した端部が同極同士で接合されて輪状に形成された集電体接合部と、
前記集電体接合部にそれぞれ密着して接続された正極集電板および負極集電板であって、外部端子との導通を確保するための正極集電板および負極集電板と、
を有することを特徴とする角型電池。 An electrode plate group in which a positive electrode plate in which a positive electrode active material is applied on both surfaces of a positive electrode current collector and a negative electrode plate in which a negative electrode active material is applied on both surfaces of a negative electrode current collector forms a laminated structure with a separator interposed therebetween. A prismatic battery housed in a battery can,
An insulator provided in contact with both sides of the electrode plate assembly,
Forming the the end of the end portion of the positive electrode current collector and the negative electrode current collector projecting in opposite directions to each other through the insulator from the both sides, annular end issued projecting is joined with same poles and the collector junction is,
A positive electrode current collector plate and the negative electrode current collector plate that is connected in close contact to each of the current collector junction, the positive electrode and negative electrode terminal plates to ensure conduction between the external terminal,
Prismatic battery characterized by having a.
By a clamping member having means for sandwiching the collector junction the collector plate is placed and fixed by sandwiching inserting the current collector junction to said clamping member, the current collector and the current collector plate The prismatic battery according to claim 1, wherein the connection with the battery is maintained.
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