CN104087422B - A kind of preparation method of hollyhock rhizome Aqueous extracts and application thereof - Google Patents
A kind of preparation method of hollyhock rhizome Aqueous extracts and application thereof Download PDFInfo
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Abstract
A preparation method for hollyhock rhizome Aqueous extracts, is characterized in that: comprise following processing step: dry Root of Hollyhock and/or stem → removal of impurities, pulverizing → soak → enzyme digestion reaction → heating lixiviate → solid-liquid separation → concentrating under reduced pressure → hollyhock rhizome Aqueous extracts.The hollyhock rhizome Aqueous extracts of gained is yellowish brown liquid, is applied on cigarette shreds after water dilution with feed liquid, and when burning and sucking cigarette, flue gas free from extraneous odour, can enrich note, improve aroma quality, increases sweet sense, reduce dry sensation, improve oral cavity comfortableness.Maximum feature of the present invention is: provide one " hollyhock rhizome Aqueous extracts " Novel tobacco flavor, the application of this spices does not change original performance and the complete processing of cigarette, improve the flavouring essence quality of cigarette, improve sense organ comfort level when cigarette burns and sucks, without any side effects; And hollyhock is widely distributed in China, aboundresources, production technique is simple to operation, and production cost is lower, therefore has more the meaning and value of actual production.
Description
Technical field
The present invention relates to essence spice for cigarette field, specifically a kind of hollyhock rhizome Aqueous extracts preparation method and as the application of tobacco aromatics using in cigarette.
Background technology
Certain deficiency is still there is in current domestic cigarette product in physics humid keeping performance and sense organ comfort level etc.For improving the overall quality of cigarette product, the research and discovery relating to the fields such as raw tobacco material, complete processing and essence and flavoring agent launches in succession.Developing distinctive Novel tobacco flavor is one of them main solution route.Natural perfume is because of its note enriches, the advantage such as fragrance is true to nature, safety and environmental protection becomes recent researches exploitation emphasis.
Vast territory and abundant resources in China, and floristics is various, and the composition of contained effective constituent also respectively has feature, for the exploitation of natural perfume provides rich in natural resources.By different modes method, extraction and isolation is carried out to effective ingredients in plant, and for the feature of cigarette product, extract is applied in cigarette in different forms, to improving the overall quality of cigarette.
Hollyhock [
althaearosea(Linn.) Cavan.] have another name called one zhang of red, waste of flax flower, checkerbloom, cape flower, Dragon Boat Festival flower etc., English name hollyhock, the biennial upright herbaceous plant (Feng Guomei of Malvaceae (Malvaceae) Althaea, Chinese Plants will (the 49th volume second fascicle), the Chinese Academy of Sciences's " Chinese Plants will " editorial board, Science Press: Beijing, 1984, p11).Hollyhock originates in Southwestern China area, is the plant various value such as a kind ofly having ecology, view and admire, eat, be medicinal, extensively cultivation in all parts of the country at present.Hollyhock is used as medicine with root, leaf, flower, seed, clearing heat and detoxicating, for oral administration to treat constipation, separates tetrodotoxin, diuresis; The disease such as sore, scald is controlled in external application.The root of hollyhock and stem contain abundant xylogen and lymphatic temperament, and its mucilagenous main component is acidic polysaccharose, in addition containing monose, oligose, protein, pectin, hemicellulose and trace element etc.In Root of Hollyhock and stem, contained lymphatic temperament can be used as lubricant, for mucosal inflammation, plays protection, alleviates stimulation.The pharmacological research of system confirms that the aqueous extract of Root of Hollyhock, stem can be used as the medicine for the treatment of inflammation; as upper respiratory tract mucosa inflammation, bronchial asthma etc.; and Root of Hollyhock extract is used as Apophlegmatisant; hollyhock stem extract is as anti-ulcer medicament; also preclinical pharmacology research has been entered; be used for the treatment of stomach and enteron aisle ulcer { Azizov, U.M.; Mirakilova, D.B.; Umarova, N.T.; Etal.Chemicalcompositionofdryextractsfrom
alcearosea[J] .ChemistryofNaturalCompounds, 2007,43 (5): 508-511.}.
In hollyhock rhizome, the composition A wide selection of colours and designs of polysaccharide, has semi-lactosi, glucose, wood sugar, pectinose, rhamnosyl and glucuronic acid, galacturonic acid etc.; Its protein composition has analyzed 17 seed amino acids.Polysaccharide and protein in the processing of cigarette and can burn and suck the fragrance matter that in process, reaction generation is abundant after degraded.Glucide itself has the physical properties of moisture absorption and moisturizing simultaneously, can keep the moisture content of pipe tobacco, thus improves the processing characteristics of pipe tobacco.But, have not yet to see the application of hollyhock extract in tobacco.
Summary of the invention
The present invention is studied the extracting method of hollyhock rhizome based on above-mentioned present Research just, the new type natural spices that the suitable cigarette products of exploitation adds, and object is suction quality and the sense organ comfort level of improving cigarette product.
The object of the invention is to be achieved through the following technical solutions:
A kind of cigarette hollyhock rhizome Aqueous extracts is prepared from by the following method: dry Root of Hollyhock and/or stem → removal of impurities, pulverizing → soak → enzyme digestion reaction → heating lixiviate → solid-liquid separation → concentrating under reduced pressure → hollyhock rhizome Aqueous extracts.
Soaking in step, feed liquid mass ratio is 1:8 ~ 1:15, soaking at room temperature 2 ~ 4h.
In enzyme digestion reaction step, the zymin added is cellulase and proteolytic enzyme, addition be respectively Root of Hollyhock, stem dry powder quality 0.5 ~ 2% and 0.2 ~ 0.5%, hydrolysis temperature 40 ~ 60 DEG C, enzymolysis time 1 ~ 3h.Macromole fibrous matter in its cellulase degradable cell walls, contributes to the stripping of the effective constituent in born of the same parents; The macromolecular protein of proteolytic enzyme degradable, reduces protein to the impact of cigarette odor-absorbing.In addition, the small molecular sugar compounds produced in enzymolysis process and micromolecular nitrogenous compound can generate nitrogen heterocyclic or oxa-lopps material further by Maillard reaction again in heat-processed, thus the content of fragrance matter in increase Aqueous extracts, and enrich the note of Aqueous extracts, to the organoleptic quality of cigarette, there is better improvement result.
In heating lixiviate step, extraction temperature 70 ~ 100 DEG C, extraction time 3 ~ 5h.Heating lixiviate can reach three objects simultaneously: (1) make zymin deactivation; (2) improve extracting efficiency; (3) thermal response produces fragrance matter.
In solid-liquid separation step, adopt vacuum filtration, vacuum degree control at-0.05 ~-0.1MPa, or adopts centrifugation, centrifugal rotational speed 1000 ~ 4000rpm, centrifugation time 20 ~ 40min.
Solid-liquid separation gained clear liquid is 10 ~ 30% through being evaporated to paste containing amount.
The hollyhock rhizome Aqueous extracts of the inventive method gained is yellowish brown liquid, be applied on cigarette shreds with feed liquid after water dilution, technique makes cigarette routinely, when burning and sucking cigarette, flue gas free from extraneous odour, note can be enriched, improve aroma quality, increase sweet sense, reduce dry sensation, improve oral cavity comfortableness.Concrete usage ratio is: hollyhock rhizome Aqueous extracts consumption is 0.01 ‰ ~ 0.5 ‰ of tobacco quality.Essence can be deployed into according to cigarette style and other spices to use.
Maximum feature of the present invention is: provide one " hollyhock rhizome Aqueous extracts " Novel tobacco flavor, containing multiple fragrance material or flavor precursors such as multiple monose, oligose, water-soluble polysaccharide and maillard reaction products in this spices.Do not changing on the original performance of cigarette and complete processing basis, the hollyhock rhizome Aqueous extracts of interpolation can enrich cigarette perfume (or spice), improves the water-holding power of pipe tobacco, improves sense organ comfort level when cigarette burns and sucks, without any side effects; And hollyhock is widely distributed in China, aboundresources, production technique is simple to operation, and production cost is lower, therefore has more the meaning and value of actual production.
Embodiment
Below in conjunction with embodiment, the present invention is described further, but does not limit the present invention.
embodiment 1
Get dry hollyhock rhizome, weigh after removal of impurities, pulverizing; Add the water (distilled water, pure water or deionized water all can) of its 12 times of quality, soak at room temperature 3h, after being heated to 50 DEG C, adds the cellulase of Root of Hollyhock stem dry powder quality 1% and the proteolytic enzyme of 0.3%, 50 DEG C of constant temperature 3h; Reheat and be warming up to 90 DEG C of backflow 3h, after stopping heating, treat that feed liquid is cooled to room temperature, the centrifugal 40min of 2000rmp; Namely supernatant liquor obtains hollyhock rhizome Aqueous extracts through being evaporated to paste containing amount 10%.
Take 0.005g above-mentioned hollyhock rhizome Aqueous extracts, add distilled water to 5.000g, spray equably with micro sprayer after mixing and be added on the blank pipe tobacco of 100g (feeding quantity is 0.05 ‰).Loaded by pipe tobacco in sealing bag, place 80 DEG C of constant temperature 30min in baking oven, then shake pipe tobacco rapidly, moisture in cut tobacco controls, about 12%, to roll into cigarette, puts into constant temperature (22 ± 1 DEG C) constant humidity (relative humidity 60 ± 2%) more than case inner equilibrium 48h.Reference cigarette is under similarity condition, adds identical deal distilled water, roll into contrast cigarette with same pipe tobacco spray.Smoke panel test through the above judging panel of 7 people, result shows: cigarette flavor matter and the perfume quantity of adding hollyhock rhizome Aqueous extracts all have lifting, and note is abundant, flue gas is full, and pleasant impression is sweet comfortable, and xerostomia sense reduces, and cigarette smoking quality is improved.
embodiment 2
Root of Hollyhock obtains Root of Hollyhock dry powder after removal of impurities, oven dry, pulverizing, adds the water of its 15 times of quality, soak at room temperature 2h, after being heated to 45 DEG C, adds the cellulase of Root of Hollyhock dry powder quality 0.5% and the proteolytic enzyme of 0.4%, 45 DEG C of constant temperature 2h; Reheat and be warming up to 75 DEG C of backflow 5h, after stopping heating, treat that feed liquid is cooled to room temperature, the centrifugal 30min of 4000rmp; Namely clear liquid obtains Root of Hollyhock Aqueous extracts through being evaporated to paste containing amount 20%.
Take 0.020g Root of Hollyhock Aqueous extracts, add distilled water diluting to 1.000g, mixing, to inject 4 μ L(perfuming amounts be 0.1 ‰ to often propping up in blank cigarette to adopt perfuming cigarette injector); Separately get partial blank cigarette, often prop up injection 4 μ L distilled water cigarette in contrast.Cigarette after perfuming and contrast cigarette are put into constant temperature (22 ± 1 DEG C) constant humidity (relative humidity 60 ± 2%) more than case inner equilibrium 48h respectively.Smoking result shows: the cigarette flavor matter after perfuming and perfume quantity promote, and note enriches, and have Hui Tian to promote the production of body fluid sense, pleasant impression is comfortable.
embodiment 3
Hollyhock stem is weighed after removal of impurities, oven dry, pulverizing, adds the water of its 10 times of quality, soak at room temperature 4h; After being heated to 55 DEG C, add the cellulase of hollyhock stem dry powder quality 1.5% and the proteolytic enzyme of 0.2%, 55 DEG C of constant temperature 1.5h; Reheat and be warming up to 80 DEG C of backflow 4h, after stopping heating, treat that feed liquid is cooled to room temperature, decompress filter, vacuum tightness-0.08MPa, namely clear liquid obtains hollyhock stem Aqueous extracts through being evaporated to paste containing amount 30%.
Take 0.100g above-mentioned hollyhock stem Aqueous extracts, with distilled water diluting to 10.000g, mixing.Get the pipe tobacco of two parts of even equivalent, a diluting soln (perfuming amount is 0.5 ‰) evenly spraying Flower of Hollyhock Aqueous extracts by 5% of pipe tobacco weight on pipe tobacco; Another part of even distilled water pipe tobacco in contrast spraying pipe tobacco weight 5%.Cigarette is rolled into respectively after baking.Test cigarette and contrast cigarette are put into constant temperature (22 ± 1 DEG C), constant humidity (relative humidity 60 ± 2%) more than case inner equilibrium 48h respectively.Smoking result shows: after applying hollyhock stem Aqueous extracts, cigarette smoke free from extraneous odour, can enrich note, improve aroma quality, increases sweet sense, reduce dry sensation, improve oral cavity comfortableness.
Claims (7)
1. the application of a hollyhock rhizome Aqueous extracts in cigarette shreds, it is characterized in that: hollyhock rhizome Aqueous extracts is applied on cigarette shreds with feed liquid after water dilution, technique makes cigarette routinely, when burning and sucking cigarette, flue gas free from extraneous odour, note can be enriched, improve aroma quality, increase sweet sense, reduce dry sensation, improve oral cavity comfortableness; Described hollyhock rhizome Aqueous extracts is prepared from by following processing step: dry Root of Hollyhock and/or stem → removal of impurities, pulverizing → soak → enzyme digestion reaction → heating lixiviate → solid-liquid separation → concentrating under reduced pressure → hollyhock rhizome Aqueous extracts.
2. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, is characterized in that: soaking in step, and feed liquid mass ratio is 1:8 ~ 1:15, soaking at room temperature 2 ~ 4h.
3. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, it is characterized in that: in enzyme digestion reaction step, the zymin added is cellulase and proteolytic enzyme, the addition of cellulase be Root of Hollyhock, stem dry powder quality 0.5 ~ 2%, the addition of proteolytic enzyme be Root of Hollyhock, stem dry powder quality 0.2 ~ 0.5%, hydrolysis temperature 40 ~ 60 DEG C, enzymolysis time 1 ~ 3h.
4. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, is characterized in that: in heating lixiviate step, extraction temperature 70 ~ 100 DEG C, extraction time 3 ~ 5h.
5. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, is characterized in that: in solid-liquid separation step, and adopt vacuum filtration, vacuum degree control is at-0.05 ~-0.1Mpa; Or employing centrifugation, centrifugal rotational speed 1000 ~ 4000rpm, centrifugation time 20 ~ 40min.
6. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, is characterized in that: in concentrating under reduced pressure step, and solid-liquid separation gained clear liquid is 10 ~ 30% through being evaporated to paste containing amount.
7. the application of hollyhock rhizome Aqueous extracts according to claim 1 in cigarette shreds, is characterized in that: hollyhock rhizome Aqueous extracts consumption is 0.01 ‰ ~ 0.5 ‰ of tobacco quality.
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| CN104862075A (en) * | 2015-06-03 | 2015-08-26 | 湖北中烟工业有限责任公司 | Preparation method of mullein extract for cigarette |
| CN106701325A (en) * | 2017-03-08 | 2017-05-24 | 湖北中烟工业有限责任公司 | Apricot extract for tobaccos and preparation method of apricot extract |
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