JP7387451B2 - 筆記具 - Google Patents
筆記具 Download PDFInfo
- Publication number
- JP7387451B2 JP7387451B2 JP2020002466A JP2020002466A JP7387451B2 JP 7387451 B2 JP7387451 B2 JP 7387451B2 JP 2020002466 A JP2020002466 A JP 2020002466A JP 2020002466 A JP2020002466 A JP 2020002466A JP 7387451 B2 JP7387451 B2 JP 7387451B2
- Authority
- JP
- Japan
- Prior art keywords
- bis
- pyridine
- barrel
- dimethylaminophenyl
- writing
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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- 230000000149 penetrating effect Effects 0.000 claims description 2
- 239000000049 pigment Substances 0.000 description 45
- -1 lactone compounds Chemical class 0.000 description 37
- 239000000976 ink Substances 0.000 description 36
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- 230000002441 reversible effect Effects 0.000 description 28
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- YBPFWNXHTBDOQJ-UHFFFAOYSA-N 3,5,5-trimethylhexyl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OCCC(C)CC(C)(C)C YBPFWNXHTBDOQJ-UHFFFAOYSA-N 0.000 description 2
- KBWOAGGPYKQCAO-UHFFFAOYSA-N 4-[2-(4-hydroxyphenyl)nonan-2-yl]phenol Chemical compound C=1C=C(O)C=CC=1C(C)(CCCCCCC)C1=CC=C(O)C=C1 KBWOAGGPYKQCAO-UHFFFAOYSA-N 0.000 description 2
- ZXYXCLKASBAWBE-UHFFFAOYSA-N 4-[6-[4-(dimethylamino)phenyl]-4-(4-methylphenyl)pyridin-2-yl]-n,n-dimethylaniline Chemical compound C1=CC(N(C)C)=CC=C1C1=CC(C=2C=CC(C)=CC=2)=CC(C=2C=CC(=CC=2)N(C)C)=N1 ZXYXCLKASBAWBE-UHFFFAOYSA-N 0.000 description 2
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- CDBYLPFSWZWCQE-UHFFFAOYSA-L Sodium Carbonate Chemical compound [Na+].[Na+].[O-]C([O-])=O CDBYLPFSWZWCQE-UHFFFAOYSA-L 0.000 description 2
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- 125000000217 alkyl group Chemical group 0.000 description 2
- 229910000147 aluminium phosphate Inorganic materials 0.000 description 2
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- LLEMOWNGBBNAJR-UHFFFAOYSA-N biphenyl-2-ol Chemical compound OC1=CC=CC=C1C1=CC=CC=C1 LLEMOWNGBBNAJR-UHFFFAOYSA-N 0.000 description 2
- IISBACLAFKSPIT-UHFFFAOYSA-N bisphenol A Chemical compound C=1C=C(O)C=CC=1C(C)(C)C1=CC=C(O)C=C1 IISBACLAFKSPIT-UHFFFAOYSA-N 0.000 description 2
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- LQZZUXJYWNFBMV-UHFFFAOYSA-N dodecan-1-ol Chemical compound CCCCCCCCCCCCO LQZZUXJYWNFBMV-UHFFFAOYSA-N 0.000 description 2
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- XLLIQLLCWZCATF-UHFFFAOYSA-N ethylene glycol monomethyl ether acetate Natural products COCCOC(C)=O XLLIQLLCWZCATF-UHFFFAOYSA-N 0.000 description 2
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- GOQYKNQRPGWPLP-UHFFFAOYSA-N heptadecan-1-ol Chemical compound CCCCCCCCCCCCCCCCCO GOQYKNQRPGWPLP-UHFFFAOYSA-N 0.000 description 2
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- 238000000034 method Methods 0.000 description 2
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- OMJRVNYAQYMXFR-UHFFFAOYSA-N octan-2-yl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OC(C)CCCCCC OMJRVNYAQYMXFR-UHFFFAOYSA-N 0.000 description 2
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- CHHHXKFHOYLYRE-UHFFFAOYSA-M 2,4-Hexadienoic acid, potassium salt (1:1), (2E,4E)- Chemical compound [K+].CC=CC=CC([O-])=O CHHHXKFHOYLYRE-UHFFFAOYSA-M 0.000 description 1
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- CYEJMVLDXAUOPN-UHFFFAOYSA-N 2-dodecylphenol Chemical compound CCCCCCCCCCCCC1=CC=CC=C1O CYEJMVLDXAUOPN-UHFFFAOYSA-N 0.000 description 1
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- UFVKGYZPFZQRLF-UHFFFAOYSA-N hydroxypropyl methyl cellulose Chemical compound OC1C(O)C(OC)OC(CO)C1OC1C(O)C(O)C(OC2C(C(O)C(OC3C(C(O)C(O)C(CO)O3)O)C(CO)O2)O)C(CO)O1 UFVKGYZPFZQRLF-UHFFFAOYSA-N 0.000 description 1
- 238000010191 image analysis Methods 0.000 description 1
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- 150000002576 ketones Chemical class 0.000 description 1
- 239000007788 liquid Substances 0.000 description 1
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- 239000000711 locust bean gum Substances 0.000 description 1
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- 150000002772 monosaccharides Chemical class 0.000 description 1
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- DALSJXSLCSAJND-UHFFFAOYSA-N n,n-diethyl-4-(4-methylquinazolin-2-yl)aniline Chemical compound C1=CC(N(CC)CC)=CC=C1C1=NC(C)=C(C=CC=C2)C2=N1 DALSJXSLCSAJND-UHFFFAOYSA-N 0.000 description 1
- UPJHNYBDPXOYTC-UHFFFAOYSA-N n,n-diethyl-4-(4-phenylquinazolin-2-yl)aniline Chemical compound C1=CC(N(CC)CC)=CC=C1C1=NC(C=2C=CC=CC=2)=C(C=CC=C2)C2=N1 UPJHNYBDPXOYTC-UHFFFAOYSA-N 0.000 description 1
- KFIUKWSBXNVCHI-UHFFFAOYSA-N n,n-dimethyl-4-(4-morpholin-4-ylquinazolin-2-yl)aniline Chemical compound C1=CC(N(C)C)=CC=C1C1=NC(N2CCOCC2)=C(C=CC=C2)C2=N1 KFIUKWSBXNVCHI-UHFFFAOYSA-N 0.000 description 1
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- GOCLJAKNIYYTMF-UHFFFAOYSA-N n,n-dimethyl-4-[2-(2-octoxyphenyl)-6-phenylpyridin-4-yl]aniline Chemical compound CCCCCCCCOC1=CC=CC=C1C1=CC(C=2C=CC(=CC=2)N(C)C)=CC(C=2C=CC=CC=2)=N1 GOCLJAKNIYYTMF-UHFFFAOYSA-N 0.000 description 1
- WQEPLUUGTLDZJY-UHFFFAOYSA-N n-Pentadecanoic acid Natural products CCCCCCCCCCCCCCC(O)=O WQEPLUUGTLDZJY-UHFFFAOYSA-N 0.000 description 1
- XGXKNJKGLCFDGK-UHFFFAOYSA-N n-[(4-methylphenyl)methyl]-2-pyridin-4-ylaniline Chemical compound C1=CC(C)=CC=C1CNC1=CC=CC=C1C1=CC=NC=C1 XGXKNJKGLCFDGK-UHFFFAOYSA-N 0.000 description 1
- IPCSVZSSVZVIGE-UHFFFAOYSA-N n-hexadecanoic acid Natural products CCCCCCCCCCCCCCCC(O)=O IPCSVZSSVZVIGE-UHFFFAOYSA-N 0.000 description 1
- FUZZWVXGSFPDMH-UHFFFAOYSA-N n-hexanoic acid Natural products CCCCCC(O)=O FUZZWVXGSFPDMH-UHFFFAOYSA-N 0.000 description 1
- PDDANVVLWYOEPS-UHFFFAOYSA-N nitrous acid;n-propan-2-ylpropan-2-amine Chemical compound [O-]N=O.CC(C)[NH2+]C(C)C PDDANVVLWYOEPS-UHFFFAOYSA-N 0.000 description 1
- JXOZTDCDOAVPBQ-UHFFFAOYSA-N nonan-2-yl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OC(C)CCCCCCC JXOZTDCDOAVPBQ-UHFFFAOYSA-N 0.000 description 1
- SDPZWRKQPQDSQW-UHFFFAOYSA-N nonyl palmitate Chemical compound CCCCCCCCCCCCCCCC(=O)OCCCCCCCCC SDPZWRKQPQDSQW-UHFFFAOYSA-N 0.000 description 1
- SNQQPOLDUKLAAF-UHFFFAOYSA-N nonylphenol Chemical compound CCCCCCCCCC1=CC=CC=C1O SNQQPOLDUKLAAF-UHFFFAOYSA-N 0.000 description 1
- 125000003261 o-tolyl group Chemical group [H]C1=C([H])C(*)=C(C([H])=C1[H])C([H])([H])[H] 0.000 description 1
- WRPMUZXHQKAAIC-CZIZESTLSA-N octadecyl (e)-octadec-9-enoate Chemical compound CCCCCCCCCCCCCCCCCCOC(=O)CCCCCCC\C=C\CCCCCCCC WRPMUZXHQKAAIC-CZIZESTLSA-N 0.000 description 1
- ZFCUBQOYWAZKNO-ZPHPHTNESA-N octadecyl (z)-docos-13-enoate Chemical compound CCCCCCCCCCCCCCCCCCOC(=O)CCCCCCCCCCC\C=C/CCCCCCCC ZFCUBQOYWAZKNO-ZPHPHTNESA-N 0.000 description 1
- LOEGNUHLVGAMMW-UHFFFAOYSA-N octadecyl 4-tert-butylbenzoate Chemical compound CCCCCCCCCCCCCCCCCCOC(=O)C1=CC=C(C(C)(C)C)C=C1 LOEGNUHLVGAMMW-UHFFFAOYSA-N 0.000 description 1
- NKBWPOSQERPBFI-UHFFFAOYSA-N octadecyl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCCOC(=O)CCCCCCCCCCCCCCCCC NKBWPOSQERPBFI-UHFFFAOYSA-N 0.000 description 1
- FSJWPESNOACHDX-UHFFFAOYSA-N octan-2-yl docosanoate Chemical compound CCCCCCCCCCCCCCCCCCCCCC(=O)OC(C)CCCCCC FSJWPESNOACHDX-UHFFFAOYSA-N 0.000 description 1
- RZPJLYNNGLQFSH-UHFFFAOYSA-N octan-3-yl dodecanoate Chemical compound CCCCCCCCCCCC(=O)OC(CC)CCCCC RZPJLYNNGLQFSH-UHFFFAOYSA-N 0.000 description 1
- ZVOOTAVWWKKSMX-UHFFFAOYSA-N octan-3-yl tetradecanoate Chemical compound CCCCCCCCCCCCCC(=O)OC(CC)CCCCC ZVOOTAVWWKKSMX-UHFFFAOYSA-N 0.000 description 1
- YYZUSRORWSJGET-UHFFFAOYSA-N octanoic acid ethyl ester Natural products CCCCCCCC(=O)OCC YYZUSRORWSJGET-UHFFFAOYSA-N 0.000 description 1
- RIKCMEDSBFQFAL-UHFFFAOYSA-N octyl 4-hydroxybenzoate Chemical compound CCCCCCCCOC(=O)C1=CC=C(O)C=C1 RIKCMEDSBFQFAL-UHFFFAOYSA-N 0.000 description 1
- CBFCDTFDPHXCNY-UHFFFAOYSA-N octyldodecane Natural products CCCCCCCCCCCCCCCCCCCC CBFCDTFDPHXCNY-UHFFFAOYSA-N 0.000 description 1
- ZQPPMHVWECSIRJ-KTKRTIGZSA-N oleic acid Chemical compound CCCCCCCC\C=C/CCCCCCCC(O)=O ZQPPMHVWECSIRJ-KTKRTIGZSA-N 0.000 description 1
- 229920001542 oligosaccharide Polymers 0.000 description 1
- 150000002482 oligosaccharides Chemical class 0.000 description 1
- 239000012860 organic pigment Substances 0.000 description 1
- 235000010292 orthophenyl phenol Nutrition 0.000 description 1
- 238000007254 oxidation reaction Methods 0.000 description 1
- JCGNDDUYTRNOFT-UHFFFAOYSA-N oxolane-2,4-dione Chemical compound O=C1COC(=O)C1 JCGNDDUYTRNOFT-UHFFFAOYSA-N 0.000 description 1
- 125000003854 p-chlorophenyl group Chemical group [H]C1=C([H])C(*)=C([H])C([H])=C1Cl 0.000 description 1
- 125000000913 palmityl group Chemical group [H]C([*])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])C([H])([H])[H] 0.000 description 1
- YYYQIRQULKVEKH-UHFFFAOYSA-N pentadecyl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OCCCCCCCCCCCCCCC YYYQIRQULKVEKH-UHFFFAOYSA-N 0.000 description 1
- VIGFCAKEBCTBRO-UHFFFAOYSA-N pentan-3-yl docosanoate Chemical compound CCCCCCCCCCCCCCCCCCCCCC(=O)OC(CC)CC VIGFCAKEBCTBRO-UHFFFAOYSA-N 0.000 description 1
- KGWZZYZGKLHJTL-UHFFFAOYSA-N pentan-3-yl hexadecanoate Chemical compound CCCCCCCCCCCCCCCC(=O)OC(CC)CC KGWZZYZGKLHJTL-UHFFFAOYSA-N 0.000 description 1
- JIMNZICTZXMMIE-UHFFFAOYSA-N pentan-3-yl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OC(CC)CC JIMNZICTZXMMIE-UHFFFAOYSA-N 0.000 description 1
- DGBWPZSGHAXYGK-UHFFFAOYSA-N perinone Chemical compound C12=NC3=CC=CC=C3N2C(=O)C2=CC=C3C4=C2C1=CC=C4C(=O)N1C2=CC=CC=C2N=C13 DGBWPZSGHAXYGK-UHFFFAOYSA-N 0.000 description 1
- 230000002093 peripheral effect Effects 0.000 description 1
- 230000035699 permeability Effects 0.000 description 1
- 125000002080 perylenyl group Chemical group C1(=CC=C2C=CC=C3C4=CC=CC5=CC=CC(C1=C23)=C45)* 0.000 description 1
- CSHWQDPOILHKBI-UHFFFAOYSA-N peryrene Natural products C1=CC(C2=CC=CC=3C2=C2C=CC=3)=C3C2=CC=CC3=C1 CSHWQDPOILHKBI-UHFFFAOYSA-N 0.000 description 1
- IEQIEDJGQAUEQZ-UHFFFAOYSA-N phthalocyanine Chemical compound N1C(N=C2C3=CC=CC=C3C(N=C3C4=CC=CC=C4C(=N4)N3)=N2)=C(C=CC=C2)C2=C1N=C1C2=CC=CC=C2C4=N1 IEQIEDJGQAUEQZ-UHFFFAOYSA-N 0.000 description 1
- 229920003023 plastic Polymers 0.000 description 1
- 239000004033 plastic Substances 0.000 description 1
- 229920000058 polyacrylate Polymers 0.000 description 1
- 229920005668 polycarbonate resin Polymers 0.000 description 1
- 239000004431 polycarbonate resin Substances 0.000 description 1
- 238000006116 polymerization reaction Methods 0.000 description 1
- 150000008442 polyphenolic compounds Chemical class 0.000 description 1
- 229920001451 polypropylene glycol Polymers 0.000 description 1
- 239000004302 potassium sorbate Substances 0.000 description 1
- 235000010241 potassium sorbate Nutrition 0.000 description 1
- 229940069338 potassium sorbate Drugs 0.000 description 1
- 230000003449 preventive effect Effects 0.000 description 1
- 230000008569 process Effects 0.000 description 1
- 238000012545 processing Methods 0.000 description 1
- BDERNNFJNOPAEC-UHFFFAOYSA-N propan-1-ol Chemical compound CCCO BDERNNFJNOPAEC-UHFFFAOYSA-N 0.000 description 1
- IZQHTCYPZWOMFQ-UHFFFAOYSA-N propan-2-yl docosanoate Chemical compound CCCCCCCCCCCCCCCCCCCCCC(=O)OC(C)C IZQHTCYPZWOMFQ-UHFFFAOYSA-N 0.000 description 1
- 125000001436 propyl group Chemical group [H]C([*])([H])C([H])([H])C([H])([H])[H] 0.000 description 1
- 235000019423 pullulan Nutrition 0.000 description 1
- 150000003222 pyridines Chemical class 0.000 description 1
- HNJBEVLQSNELDL-UHFFFAOYSA-N pyrrolidin-2-one Chemical compound O=C1CCCN1 HNJBEVLQSNELDL-UHFFFAOYSA-N 0.000 description 1
- FYNROBRQIVCIQF-UHFFFAOYSA-N pyrrolo[3,2-b]pyrrole-5,6-dione Chemical compound C1=CN=C2C(=O)C(=O)N=C21 FYNROBRQIVCIQF-UHFFFAOYSA-N 0.000 description 1
- 239000001397 quillaja saponaria molina bark Substances 0.000 description 1
- 150000003246 quinazolines Chemical class 0.000 description 1
- 229910052761 rare earth metal Inorganic materials 0.000 description 1
- 230000027756 respiratory electron transport chain Effects 0.000 description 1
- 238000007127 saponification reaction Methods 0.000 description 1
- 229930182490 saponin Natural products 0.000 description 1
- 150000007949 saponins Chemical class 0.000 description 1
- 229920006395 saturated elastomer Polymers 0.000 description 1
- 229910052710 silicon Inorganic materials 0.000 description 1
- 229920002545 silicone oil Polymers 0.000 description 1
- 150000003384 small molecules Chemical class 0.000 description 1
- 210000004894 snout Anatomy 0.000 description 1
- 239000001632 sodium acetate Substances 0.000 description 1
- 235000017281 sodium acetate Nutrition 0.000 description 1
- WXMKPNITSTVMEF-UHFFFAOYSA-M sodium benzoate Chemical compound [Na+].[O-]C(=O)C1=CC=CC=C1 WXMKPNITSTVMEF-UHFFFAOYSA-M 0.000 description 1
- 235000010234 sodium benzoate Nutrition 0.000 description 1
- 239000004299 sodium benzoate Substances 0.000 description 1
- 229960003885 sodium benzoate Drugs 0.000 description 1
- 229910000029 sodium carbonate Inorganic materials 0.000 description 1
- 235000019259 sodium dehydroacetate Nutrition 0.000 description 1
- 229940079839 sodium dehydroacetate Drugs 0.000 description 1
- FQENQNTWSFEDLI-UHFFFAOYSA-J sodium diphosphate Chemical compound [Na+].[Na+].[Na+].[Na+].[O-]P([O-])(=O)OP([O-])([O-])=O FQENQNTWSFEDLI-UHFFFAOYSA-J 0.000 description 1
- 239000001488 sodium phosphate Substances 0.000 description 1
- 229910000162 sodium phosphate Inorganic materials 0.000 description 1
- 229940048086 sodium pyrophosphate Drugs 0.000 description 1
- 159000000000 sodium salts Chemical class 0.000 description 1
- DSOWAKKSGYUMTF-GZOLSCHFSA-M sodium;(1e)-1-(6-methyl-2,4-dioxopyran-3-ylidene)ethanolate Chemical compound [Na+].C\C([O-])=C1/C(=O)OC(C)=CC1=O DSOWAKKSGYUMTF-GZOLSCHFSA-M 0.000 description 1
- 239000002904 solvent Substances 0.000 description 1
- 238000005507 spraying Methods 0.000 description 1
- 239000008107 starch Substances 0.000 description 1
- 235000019698 starch Nutrition 0.000 description 1
- 239000005720 sucrose Substances 0.000 description 1
- 150000005846 sugar alcohols Polymers 0.000 description 1
- HXJUTPCZVOIRIF-UHFFFAOYSA-N sulfolane Chemical compound O=S1(=O)CCCC1 HXJUTPCZVOIRIF-UHFFFAOYSA-N 0.000 description 1
- 230000001629 suppression Effects 0.000 description 1
- 239000000725 suspension Substances 0.000 description 1
- PVJXQWMBHUOOCK-UHFFFAOYSA-N tetradecyl decanoate Chemical compound CCCCCCCCCCCCCCOC(=O)CCCCCCCCC PVJXQWMBHUOOCK-UHFFFAOYSA-N 0.000 description 1
- 235000019818 tetrasodium diphosphate Nutrition 0.000 description 1
- 239000001577 tetrasodium phosphonato phosphate Substances 0.000 description 1
- 229920005992 thermoplastic resin Polymers 0.000 description 1
- 229920001187 thermosetting polymer Polymers 0.000 description 1
- 150000003557 thiazoles Chemical class 0.000 description 1
- 239000002562 thickening agent Substances 0.000 description 1
- YODZTKMDCQEPHD-UHFFFAOYSA-N thiodiglycol Chemical compound OCCSCCO YODZTKMDCQEPHD-UHFFFAOYSA-N 0.000 description 1
- JOUDBUYBGJYFFP-FOCLMDBBSA-N thioindigo Chemical compound S\1C2=CC=CC=C2C(=O)C/1=C1/C(=O)C2=CC=CC=C2S1 JOUDBUYBGJYFFP-FOCLMDBBSA-N 0.000 description 1
- 229910052719 titanium Inorganic materials 0.000 description 1
- 239000010936 titanium Substances 0.000 description 1
- 239000004408 titanium dioxide Substances 0.000 description 1
- OGIDPMRJRNCKJF-UHFFFAOYSA-N titanium oxide Inorganic materials [Ti]=O OGIDPMRJRNCKJF-UHFFFAOYSA-N 0.000 description 1
- 238000006276 transfer reaction Methods 0.000 description 1
- 229940087291 tridecyl alcohol Drugs 0.000 description 1
- RYFMWSXOAZQYPI-UHFFFAOYSA-K trisodium phosphate Chemical compound [Na+].[Na+].[Na+].[O-]P([O-])([O-])=O RYFMWSXOAZQYPI-UHFFFAOYSA-K 0.000 description 1
- 239000006097 ultraviolet radiation absorber Substances 0.000 description 1
- 229940057402 undecyl alcohol Drugs 0.000 description 1
- FOROCIRSIXDJQG-UHFFFAOYSA-N undecyl octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OCCCCCCCCCCC FOROCIRSIXDJQG-UHFFFAOYSA-N 0.000 description 1
- 150000004670 unsaturated fatty acids Chemical class 0.000 description 1
- 235000021122 unsaturated fatty acids Nutrition 0.000 description 1
- 239000004034 viscosity adjusting agent Substances 0.000 description 1
- 239000000080 wetting agent Substances 0.000 description 1
- 229920001285 xanthan gum Polymers 0.000 description 1
- 235000010493 xanthan gum Nutrition 0.000 description 1
- 239000000230 xanthan gum Substances 0.000 description 1
- 229940082509 xanthan gum Drugs 0.000 description 1
- UHVMMEOXYDMDKI-JKYCWFKZSA-L zinc;1-(5-cyanopyridin-2-yl)-3-[(1s,2s)-2-(6-fluoro-2-hydroxy-3-propanoylphenyl)cyclopropyl]urea;diacetate Chemical compound [Zn+2].CC([O-])=O.CC([O-])=O.CCC(=O)C1=CC=C(F)C([C@H]2[C@H](C2)NC(=O)NC=2N=CC(=CC=2)C#N)=C1O UHVMMEOXYDMDKI-JKYCWFKZSA-L 0.000 description 1
- 229910052726 zirconium Inorganic materials 0.000 description 1
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Description
前記電子供与性呈色性有機化合物としては、フタリド化合物、フルオラン化合物、スチリノキノリン化合物、ピリジン化合物、キナゾリン化合物、ビスキナゾリン化合物、ジアザローダミンラクトン化合物が挙げられ、そのうち、発色時に蛍光性を有するためには、ピリジン化合物、キナゾリン化合物、ビスキナゾリン化合物、ジアザローダミンラクトン系化合物が用いられ、ピリジン化合物が好適に用いられる。
前記ピリジン系化合物としては、
4-(4′-メチルベンジルアミノフェニル)-ピリジン、
2,6-ジフェニル-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ジフェニル-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-プロピルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ペンチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘプチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-プロピルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ペンチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘプチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-N-フェニル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-N-クロロエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-N-クロロエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-N-クロロエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-N-クロロエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-N-クロロエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-N-エチルオキシエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-N-エチルオキシエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-N-エチルオキシエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-N-エチルオキシエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-N-エチルオキシエチル-N-メチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′-メチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-エチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-プロピルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ブチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ペンチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘキシルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-ヘプチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2′-オクチルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(2´-ノニルオキシフェニル)-4-(4′-N-イソブチル-N-エチルアミノフェニル)-ピリジン、
2,6-ビス(4′-メチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ジメチル-3,5-ビスカルボエトキシ-4-(4′-ジメチルアミノフェニル)-ピリジン、
2-(2′-オクチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-6-フェニル-ピリジン、
2,6-ジエチルオキシ-4-(4′-ジエチルアミノフェニル)-ピリジン 4-(4-メチルオキシフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-フェニル-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-メチルフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
2,4,6-トリス(4-ジメチルアミノフェニル)-ピリジン、
4-(2-クロロ-4-ジメチルアミノフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(3-ニトロフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-メチルオキシカルボニルフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-ジメチルアミノフェニル)-2,6-ビス(2-チエニル)-ピリジン、
4-(4-ジメチルアミノフェニル)-2,6-ビス(2-フリル)-ピリジン、
4-(2-クロロ-4-ジメチルアミノフェニル)-2,6-ビス(2-チエニル)-ピリジン、
4-〔4-(1-ピペリジニル)フェニル〕-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-モルホリノフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(9-ジュロリジニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-メチルフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-メチルオキシフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-メチルオキシフェニル)-2,6-ビス(4-モルホリノフェニル)-ピリジン、
4-(4-フルオロフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-N-オクチルオキシフェニル-N-メチルアミノ)-2,6-ジフェニルピリジン、
4-(4-クロロフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-ニトロフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-N-2-シアノエチル-N-メチルアミノフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(2,5-ジメチルオキシフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-ジエチルアミノフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-ビフェニルイル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-ピロリジニルフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-イソインドリニルフェニル)-2,6-ビス(4-ジメチルアミノフェニル)-ピリジン、
4-(4-N-2-シアノエチル-N-メチルアミノフェニル)-2,6-ジフェニルピリジン、
4-(4-N-メチル-N-フェニルアミノフェニル)-2,6-ジフェニルピリジン、
4-(4-N-クロロエチル-N-メチルアミノフェニル)-2,6-ジフェニルピリジン、
4-(4-N-エチルオキシエチル-N-メチルアミノフェニル)-2,6-ジフェニルピリジン、
2,6-ビス(2′,4′-ジメチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジエチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジプロピルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジブチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジペンチルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジヘキシルオキシフェニル)-4-(4′-ジメチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジメチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジエチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジプロピルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジブチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジペンチルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジヘキシルオキシフェニル)-4-(4′-ジエチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジメチルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジエチルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジプロピルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジブチルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジペンチルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジヘキシルオキシフェニル)-4-(4′-ジプロピルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジメチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジエチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジプロピルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジブチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジペンチルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
2,6-ビス(2′,4′-ジヘキシルオキシフェニル)-4-(4′-ジブチルアミノフェニル)-ピリジン、
等が挙げられる。
2-(4′-ジメチルアミノフェニル)-4-メチルオキシ-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-フェニルオキシ-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-(4′′-ニトロフェニルオキシ)-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-フェニルチオ-キナゾリン、
2-(4′-N-フェニル-N-メチルアミノフェニル)-4-フェニルオキシ-キナゾリン、
2-(4′-ピペリジノフェニル)-4-フェノキシ-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-(4′′-クロロフェニルオキシ)-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-(4′′-メチルオキシフェニルオキシ)-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-(N-フェニル-N-メチルアミノ)-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-モルホリノ-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-フェニル-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-メチル-キナゾリン、
2-(1′-エチル-2′,2′,4′-トリメチル-テトラヒドロキノリン-6′-イル)-4-フェニルオキシ-キナゾリン、
2-(1′-エチル-2′,2′,4′-トリメチル-テトラヒドロキノリン-6′-イル)-4-メチルオキシ-キナゾリン、
2-(1′,2′,2′,4′-テトラメチル-テトラヒドロキノリン-6′-イル)-4-フェニルオキシ-キナゾリン、
2-(1′-エチル-2′-メチル-テトラヒドロキノリン-6′-イル)-4-フェニルオキシ-キナゾリン、
2-(1′,3′-ジメチルインドリン-5′-イル)-4-フェニルオキシ-キナゾリン、
2-(3′,4′-ジメチルベンゾモルホリン-7′-イル)-4-フェニルオキシ-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-(2′′-フェニルオキシエチルオキシ)-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-(2′′-N-フェニル-N-エチルアミノエチルオキシ)-キナゾリン、
2-(4′-ジメチルアミノフェニル)-4-(2′′-モルホリノエチルオキシ)-キナゾリン、
2-(4′-ジベンジルアミノフェニル)-4-(2′′-フェニルオキシエチルオキシ)-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-(2′′-フェニルオキシエチルチオ)-キナゾリン、
2-(4′-ジエチルアミノフェニル)-4-〔2′′-(1-ナフチルオキシ)エチルオキシ〕-キナゾリン、
2-(3′,4′-ジメチルベンゾモルホリン-7′-イル)-(2′′-フェニルオキシエチルオキシ)-キナゾリン、
等が挙げられる。
前記ビスキナゾリン系化合物としては、
4,4′-(エチレンジオキシ)-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
4,4′-〔プロピレンジオキシ(1,3)〕-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
4,4′-〔ブチレンジオキシ(1,3)〕-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
4,4′-〔ブチレンジオキシ(1,4)〕-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
4,4′-(オキシジエチレン)-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
4,4′-エチレン-ビス〔2-(4-ピペリジノフェニル)-キナゾリン〕、
4,4′-エチレン-ビス〔2-(4-ジ-n-プロピルアミノフェニル)-キナゾリン〕、
4,4′-(エチレンジオキシ)-ビス〔2-(4-ジ-n-ブチルアミノフェニル)-キナゾリン〕、
4,4′-シクロヘキシレン-ビス〔2-(4-ジエチルアミノフェニル)-キナゾリン〕、
等が挙げられる。
前記ジアザローダミンラクトン系化合物としては、
2-(ジメチルアミノ)-8-(ジメチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジエチルアミノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-プロピルアミノ)-8-(ジ-n-プロピルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジ-n-ブチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジメチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(N-エチル-N-i-ブチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(N-エチル-N-i-アミルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(N-エチル-N-n-ヘキシルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジ-n-アミルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(n-オクチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジメチルアミノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジエチルアミノ)-8-(ジメチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(モルホリノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ピペリジノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(N-メチルピペラジノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ピロリジノ)-8-(ジエチルアミノ)-4-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジエチルアミノ)-8-(ジエチルアミノ)-4-メチル-4′,5′,6′,7′-テトラクロロ-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジエチルアミノ)-8-(ジエチルアミノ)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジ-n-ブチルアミノ)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(N-エチル-N-i-アミルアミノ)-8-(N-エチル-N-i-アミルアミノ)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(N-エチル-N-i-アミルアミノ)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ピペリジノ)-8-(エチルアミノ)-4-メチル-7-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-メチル-7-メチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-メチル-7-エチル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジ-n-ブチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(N-エチル-N-i-アミルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ピペリジノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(N-メチル-N-シクロヘキシルアミノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジメチルアミノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(i-アミルアミノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ピロリジノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(N-メチルピペラジノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(モルホリノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(N-メチル-N-ベンジルアミノ)-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-[ジ(2-メトキシエチル)アミノ]-8-(ジエチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-(4-メトキシフェニル)-スピロ[5H-[1]ベンゾピラノ(2,3-d)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-(4-クロロフェニル)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジ-n-ブチルアミノ)-8-(ジエチルアミノ)-4-(4-メチルフェニル)-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-[ジ(2-エトキシエチル)アミノ]-8-(ジメチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジエチルアミノ)-8-[(2-メチルフェニル)アミノ]-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(2,6-ジメチルモルホリノ)-8-(ジエチアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジシクロヘキシルアミノ)-8-(ジメチルアミノ)-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
2-(ジブチルアミノ)-8-[(4-クロロフェニル)アミノ]-4-フェニル-スピロ[5H-[1]ベンゾピラノ(2,3-g)ピリミジン-5,1′(3′H)-イソベンゾフラン]-3′-オン、
等が挙げられる。
アルコール類としては、炭素数10以上の脂肪族一価の飽和アルコールが有効であり、具体的にはデシルアルコール、ウンデシルアルコール、ドデシルアルコール、トリデシルアルコール、テトラデシルアルコール、ペンタデシルアルコール、ヘキサデシルアルコール、ヘプタデシルアルコール、オクタデシルアルコール、エイコシルアルコール、ドコシルアルコール等が挙げられる。
エステル類としては、炭素数10以上のエステル類が有効であり、脂肪族及び脂環或いは芳香環を有する一価カルボン酸と、脂肪族及び脂環或いは芳香環を有する一価アルコールの任意の組み合わせから得られるエステル類、脂肪族及び脂環或いは芳香環を有する多価カルボン酸と、脂肪族及び脂環或いは芳香環を有する一価アルコールの任意の組み合わせから得られるエステル類、脂肪族及び脂環或いは芳香環を有する一価カルボン酸と、脂肪族及び脂環或いは芳香環を有する多価アルコールの任意の組み合わせから得られるエステル類が挙げられ、具体的にはカプリル酸エチル、カプリル酸オクチル、カプリル酸ステアリル、カプリン酸ミリスチル、カプリン酸ドコシル、ラウリン酸2-エチルヘキシル、ラウリン酸n-デシル、ミリスチン酸3-メチルブチル、ミリスチン酸セチル、パルミチン酸イソプロピル、パルミチン酸ネオペンチル、パルミチン酸ノニル、パルミチン酸シクロヘキシル、ステアリン酸n-ブチル、ステアリン酸2-メチルブチル、ステアリン酸3,5,5-トリメチルヘキシル、ステアリン酸n-ウンデシル、ステアリン酸ペンタデシル、ステアリン酸ステアリル、ステアリン酸シクロヘキシルメチル、ベヘン酸イソプロピル、ベヘン酸ヘキシル、ベヘン酸ラウリル、ベヘン酸ベヘニル、安息香酸セチル、p-tert-ブチル安息香酸ステアリル、フタル酸ジミリスチル、フタル酸ジステアリル、シュウ酸ジミリスチル、シュウ酸ジセチル、マロン酸ジセチル、コハク酸ジラウリル、グルタル酸ジラウリル、アジピン酸ジウンデシル、アゼライン酸ジラウリル、セバシン酸ジ-(n-ノニル)、1,18-オクタデシルメチレンジカルボン酸ジネオペンチル、エチレングリコールジミリステート、プロピレングリコールジラウレート、プロピレングリコールジステアレート、ヘキシレングリコールジパルミテート、1,5-ペンタンジオールジステアレート、1,2,6-ヘキサントリオールトリミリステート、1,4-シクロヘキサンジオールジデシル、1,4-シクロヘキサンジメタノールジミリステート、キシレングリコールジカプリネート、キシレングリコールジステアレート等が挙げられる。
又、飽和脂肪酸と分枝脂肪族アルコールのエステル、不飽和脂肪酸又は分枝もしくは置換基を有する飽和脂肪酸と分岐状であるか又は炭素数16以上の脂肪族アルコールのエステル、酪酸セチル、酪酸ステアリル及び酪酸ベヘニルから選ばれるエステル化合物も有効である。具体的には、酪酸2-エチルヘキシル、ベヘン酸2-エチルヘキシル、ミリスチン酸2-エチルヘキシル、カプリン酸2-エチルヘキシル、ラウリン酸3,5,5-トリメチルヘキシル、パルミチン酸3,5,5-トリメチルヘキシル、ステアリン酸3,5,5-トリメチルヘキシル、カプロン酸2-メチルブチル、カプリル酸2-メチルブチル、カプリン酸2-メチルブチル、パルミチン酸1-エチルプロピル、ステアリン酸1-エチルプロピル、ベヘン酸1-エチルプロピル、ラウリン酸1-エチルヘキシル、ミリスチン酸1-エチルヘキシル、パルミチン酸1-エチルヘキシル、カプロン酸2-メチルペンチル、カプリル酸2-メチルペンチル、カプリン酸2-メチルペンチル、ラウリン酸2-メチルペンチル、ステアリン酸2-メチルブチル、ステアリン酸2-メチルブチル、ステアリン酸3-メチルブチル、ステアリン酸1-メチルヘプチル、ベヘン酸2-メチルブチル、ベヘン酸3-メチルブチル、ステアリン酸1-メチルヘプチル、ベヘン酸1-メチルヘプチル、カプロン酸1-エチルペンチル、パルミチン酸1-エチルペンチル、ステアリン酸1-メチルプロピル、ステアリン酸1-メチルオクチル、ステアリン酸1-メチルヘキシル、ラウリン酸1,1-ジメチルプロピル、カプリン酸1-メチルペンチル、パルミチン酸2-メチルヘキシル、ステアリン酸2-メチルヘキシル、ベヘン酸2-メチルヘキシル、ラウリン酸3,7-ジメチルオクチル、ミリスチン酸3,7-ジメチルオクチル、パルミチン酸3,7-ジメチルオクチル、ステアリン酸3,7-ジメチルオクチル、ベヘン酸3,7-ジメチルオクチル、オレイン酸ステアリル、オレイン酸ベヘニル、リノール酸ステアリル、リノール酸ベヘニル、エルカ酸3,7-ジメチルオクチル、エルカ酸ステアリル、エルカ酸イソステアリル、イソステアリン酸セチル、イソステアリン酸ステアリル、12-ヒドロキシステアリン酸2-メチルペンチル、18-ブロモステアリン酸2-エチルヘキシル、2-ケトミリスチン酸イソステアリル、2-フルオロミリスチン酸2-エチルヘキシル、酪酸セチル、酪酸ステアリル、酪酸ベヘニル等が挙げられる。
光安定剤は、(イ)、(ロ)、(ハ)成分からなる可逆熱変色性組成物の光劣化を防止するために含有され、(イ)成分1質量%に対して0.3~24質量%、好ましくは0.3~16質量%の割合で含有される。又、前記光安定剤のうち、紫外線吸収剤は、太陽光等に含まれる紫外線を効果的にカットして、(イ)成分の光反応による励起状態によって生ずる光劣化を防止する。又、酸化防止剤、一重項酸素消光剤、スーパーオキシドアニオン消光剤、オゾン消光剤等は光による酸化反応を抑制する。光安定剤は単独で用いてもよいし、2種以上を併用して用いてもよい。
尚、マイクロカプセル化は、界面重合法、in Situ重合法、液中硬化被覆法、水溶液からの相分離法、有機溶媒からの相分離法、融解分散冷却法、気中懸濁被覆法、スプレードライング法等があり、用途に応じて適宜選択される。更にマイクロカプセルの表面には、目的に応じて更に二次的な樹脂皮膜を設けて耐久性を付与させたり、表面特性を改質させて実用に供することもできる。
マイクロカプセル顔料は、内包物/壁膜=7/1~1/1(質量比)の範囲であることが好ましく、壁膜の比率が前記範囲内にあることにより、発色時の色濃度及び鮮明性の低下を防止することができ、より好適には、内包物/壁膜=6/1~1/1(質量比)である。マイクロカプセルに内包させることにより、化学的、物理的に安定な顔料を構成でき、粒子径0.01~50μm、好ましくは0.1~30μm、より好ましくは0.5~20μmの範囲が実用性を満たす。尚、平均粒子径の測定は、マウンテック社製の画像解析式粒度分布測定ソフトウェア「マックビュー」を用いて粒子の領域を判定し、粒子の領域の面積から投影面積円相当径(Heywood径)を算出し、その値による等体積球相当の粒子の平均粒子径として測定した値である。また、全ての粒子或いは大部分の粒子の粒子径が0.2μmを超える場合には、粒度分布測定装置(ベックマン・コールター株式会社製、製品名:Multisizer 4e)を用いてコールター法により等体積球相当の粒子の平均粒子径として測定することも可能である。
前記側鎖にカルボキシル基を有する櫛型高分子分散剤としては、側鎖に複数のカルボキシル基を有する櫛型高分子化合物であれば特に限定されるものではないが、側鎖に複数のカルボキシル基を有するアクリル高分子化合物が好適である。
更に、有機窒素硫黄化合物を含有させることにより、インク組成物を筆記具に充填して実用に供する際、振動による着色剤の沈降をいっそう抑制させることができるため、マイクロカプセル形態である可逆熱変色性顔料の使用時に有利である。
これは、可逆熱変色性顔料のゆるい凝集体を側鎖にカルボキシル基を有する櫛型高分子分散剤によって分散させる分散性をより向上させるものである。前記有機窒素硫黄化合物としては、チアゾール系化合物、イソチアゾール系化合物、ベンゾチアゾール系化合物、ベンゾイソチアゾール系化合物から選ばれる化合物が用いられる。尚、前記側鎖にカルボキシル基を有する櫛型高分子分散剤と、有機窒素硫黄化合物の質量比率は1:1~1:10、好ましくは1:1~1:5であり、前記範囲を満たすことにより、可逆熱変色性顔料のゆるい凝集体の分散性、及び、振動によるマイクロカプセル顔料の沈降抑制を十分に発現させることができる。更に、筆跡の紙面への固着性や粘性を付与するために適用される水溶性樹脂を添加すると、前述の側鎖にカルボキシル基を有する櫛型高分子分散剤と有機窒素硫黄化合物を含むインク中で前記着色剤の安定性を高める機能がいっそう向上する。前記水溶性樹脂としては、アルキッド樹脂、アクリル樹脂、スチレンマレイン酸共重合物、セルロース誘導体、ポリビニルピロリドン、ポリビニルアルコール、デキストリン、ポリビニルアルコール等が挙げられる。特にポリビニルアルコールは、けん化度が70~89モル%の部分けん化度型ポリビニルアルコールはインクが酸性域でも可溶性に富むため、より好適に用いられる。前記水溶性樹脂の添加量としては、インク中に0.3~3.0質量%の範囲で添加される。
2 軸筒(筒状部材)
3 先軸筒
4 後軸筒
5 筆記リフィル
6 クリップ
7 スプリング
8 回転子
9 操作部
Claims (1)
- 略均一の肉厚である筒状部材を具備する筆記具であって、前記筒状部材の表面から内面に貫通する開口部が複数箇所形成されると共に、前記開口部の開口面積がより小さい方が前記筒状部材の前側に配置され、前記開口部の開口面積がより大きい方が前記筒状部材の後側に配置されたことを特徴とする筆記具。
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Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
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JP2005014585A (ja) | 2003-06-05 | 2005-01-20 | Pilot Ink Co Ltd | 感温変色性筆記具用グリップ、それを備えた筆記具、及び筆記具セット |
JP2006289808A (ja) | 2005-04-12 | 2006-10-26 | Pilot Corporation | 筆記具の軸筒 |
JP2007253368A (ja) | 2006-03-21 | 2007-10-04 | Pilot Ink Co Ltd | 筆記具 |
JP2013111920A (ja) | 2011-11-30 | 2013-06-10 | Pentel Corp | 筆記具用部材 |
JP2014004772A (ja) | 2012-06-25 | 2014-01-16 | Pilot Corporation | 筆記具の軸筒 |
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JP2005014585A (ja) | 2003-06-05 | 2005-01-20 | Pilot Ink Co Ltd | 感温変色性筆記具用グリップ、それを備えた筆記具、及び筆記具セット |
JP2006289808A (ja) | 2005-04-12 | 2006-10-26 | Pilot Corporation | 筆記具の軸筒 |
JP2007253368A (ja) | 2006-03-21 | 2007-10-04 | Pilot Ink Co Ltd | 筆記具 |
JP2013111920A (ja) | 2011-11-30 | 2013-06-10 | Pentel Corp | 筆記具用部材 |
JP2014004772A (ja) | 2012-06-25 | 2014-01-16 | Pilot Corporation | 筆記具の軸筒 |
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