CN106252697A - A kind of outflow chamber SOFC pile - Google Patents
A kind of outflow chamber SOFC pile Download PDFInfo
- Publication number
- CN106252697A CN106252697A CN201610631780.9A CN201610631780A CN106252697A CN 106252697 A CN106252697 A CN 106252697A CN 201610631780 A CN201610631780 A CN 201610631780A CN 106252697 A CN106252697 A CN 106252697A
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- CN
- China
- Prior art keywords
- plate
- gas
- gripper shoe
- gas flowfield
- outflow chamber
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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Classifications
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- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0271—Sealing or supporting means around electrodes, matrices or membranes
- H01M8/0276—Sealing means characterised by their form
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
- H01M8/2465—Details of groupings of fuel cells
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
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- Life Sciences & Earth Sciences (AREA)
- Engineering & Computer Science (AREA)
- Manufacturing & Machinery (AREA)
- Sustainable Development (AREA)
- Sustainable Energy (AREA)
- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Fuel Cell (AREA)
Abstract
The invention discloses a kind of outflow chamber SOFC pile, including upper cover plate, battery unit and lower cover, described upper cover plate includes the first gripper shoe and the first gas flowfield plate;The quantity of described battery unit is multiple, and these described battery units are superimposed up and down and are respectively positioned between described upper cover plate and described lower cover;Each described battery unit all includes bipolar plates and flat-plate-type solid-oxide fuel battery;Described lower cover includes that the 3rd gripper shoe and the 3rd gas flowfield plate, the top of described 3rd gripper shoe are provided with the 3rd open slot, and described 3rd gas flowfield plate is arranged at described 3rd open slot.The present invention can guarantee that the uniformity that gas distributes, and improves the efficiency of collected current.
Description
Technical field
The invention belongs to field of batteries, more particularly, to one outflow chamber SOFC pile.
Background technology
SOFC (SOFC) is a kind of generating that the chemical energy of hydrocarbon fuel is converted into electric energy
Device, has energy conversion efficiency advantage high, free of contamination.At present, the SOFC structure of main flow has tubular type and flat two kinds of knots
Structure.Planar SOFC has manufacture and assembles simple, low cost and power density advantages of higher, is increasingly becoming Jiao of research both at home and abroad
Point.Classifying according to supporter, planar SOFC is divided into again electrolyte-supported, cathode support and anode support structure.Electrolyte props up
Support SOFC uses thicker ceramic oxygen ion conductor material to carry out structure support, and overall ohmage is bigger, it is necessary to 1000
Hot operation about DEG C.In this case, the LaCoO using doping more3Pottery is as metallic interconnection materials, and its cost is very
Costliness, generating efficiency is low, is unfavorable for the commercialization of SOFC.The SOFC of cathode support use perovskite ceramic material support,
, easily there is concentration polarization, is also unfavorable for the popularization of SOFC in its poorly conductive.The SOFC of anode-supported is by the Ni/YSZ of high conductivity
Ceramic metal is as support body material, and anode functional layer, electrolyte, negative electrode are by silk screen printing, electrochemical deposition or chemistry gas
The technique such as deposition is sequentially prepared on supporter mutually, the design reduces the concentration polarization of battery, reduces ohm electricity of battery
Resistance, ultra-thin electrolyte design makes SOFC operating temperature be reduced to less than 800 DEG C, metal connector being applied in pile
For possible
What planar SOFC was more conventional has interior stream chamber and the electric pile structure design of two kinds of outflow chamber.Air-flow in the pile of interior stream chamber
Chamber is formed by connector and encapsulant stacking successively, and gas transmission in air flow chamber is oriented parallel to pile stacking direction,
Vertical with airflow direction in battery layers, owing to air flow chamber and bipolar plates are an entirety, therefore bipolar plate structure is complex, difficult processing
Degree is big, and with high costs.In exterior air drain pile, air flow chamber separates with reactor core as gas buffer room, simplifies to a certain extent
The structure of bipolar plates.In above two structure, if bipolar plates uses integrated molding, it is contemplated that the heat change in the course of processing
Shape, it is necessary to use thicker steel plate just can obtain desired structure, this can be greatly increased pile volume, reduce volume energy density.
More easy way is that gripper shoe and gas distributor are processed recombinant respectively, can simplify the preparation work of gas distribution plate
Skill, has also derived the gas distribution plate of various form, includes straight channel, serpentine flow path, branch shape runner, gas flowfield plate shape
Runner etc..
In planar SOFC, connector bipolar plates is made up of gripper shoe and gas distribution plate, and gas distribution plate has concurrently and uniformly divides
Gas distribution and the function collecting battery surface electric current.In general pile, bipolar plate structure is two classes, and a class two-side current collecting device is all adopted
Designing with metal channels, the bipolar plates processing technique of this design is complicated, relatively costly.One class bipolar plate design cathode collector is adopted
Design with metal channels, and anode current collector is frequently with foam Ni or Ni felt, the drawback of this design, nickel foam and metal channels
Different at the deformational behavior of high temperature stress, nickel foam at high temperature intensity is the lowest, and bipolar plates both sides are really asymmetric answering
Power is transmitted, and when pressure transmits from top to bottom, it is possible that the uneven distribution of stress, has influence on the sealing of battery and connects
Touch.Additionally, knowable to the microstructure of nickel foam, its effective area contacted with galvanic anode is the least, electric current collection is imitated
Rate also has the space improved further.
Summary of the invention
For disadvantages described above or the Improvement requirement of prior art, the invention provides a kind of outflow chamber solid oxide fuel
Battery pile, solves bipolar plates complicated process of preparation in prior art, and cost is high, the shortcoming that precision is low, and solve reactor core should simultaneously
Power skewness, the problem that water catchment efficiency is on the low side, simplify the assembly technology of pile, can guarantee that anode and cathode gas distributes uniform
Property, improve the efficiency of collected current.
For achieving the above object, it is proposed, according to the invention, providing a kind of outflow chamber SOFC pile, it is special
Levy and be, including gas buffer cavity, upper cover plate, lower cover and battery unit, wherein,
Described upper cover plate and lower cover are respectively arranged at the top and bottom of described gas buffer cavity;
Described upper cover plate includes the first gripper shoe and the first gas flowfield plate, and the bottom of described first gripper shoe is provided with
One open slot, described first gas flowfield plate is arranged at the first open slot of described first gripper shoe, thus with described first
Gas passage is formed between gripper shoe;
Described battery unit includes N number of bipolar plates and N+1 flat-plate-type solid-oxide fuel battery, these bipolar plates and
Flat-plate-type solid-oxide fuel battery stacked on top, it is crisscross arranged;Adjacent described bipolar plates and described flat-plate-type solid oxygen
Between compound fuel cell, sealing strip is set, leaks for preventing gas;
Each described bipolar plates all includes the second gripper shoe and two the second gas flowfield plates, and wherein, described second supports
The top of plate and bottom are respectively arranged with the second open slot, and each described second gas flowfield plate is respectively arranged at one second opening
At groove, each described second gas flowfield plate respectively and forms gas passage between described second gripper shoe;
Additionally, described upper cover plate and be also equipped with between the flat-plate-type solid-oxide fuel battery of the top for
Prevent the sealing strip that gas leaks;
Described lower cover includes that the 3rd gripper shoe and the 3rd gas flowfield plate, the top of described 3rd gripper shoe are provided with
Three open slots, described 3rd gas flowfield plate is arranged at described 3rd open slot, it addition, described lower cover be positioned at bottom
Flat-plate-type solid-oxide fuel battery between be also equipped with the sealing strip for preventing gas from leaking;
Described first gas flowfield plate, the second gas flowfield plate and the 3rd gas flowfield plate structure are identical.
Preferably, described first gas flowfield plate is made up through pressure forming of corrosion resistant plate, and this corrosion resistant plate
Thickness is 0.1mm~0.3mm.
Preferably, described first gas flowfield plate uses ferrite type stainless steel material to make.
Preferably, the upper and lower surface of described first gas flowfield plate is coated respectively with conductive protection coating.
Preferably, described first gas flowfield plate is welded in described first gripper shoe.
Preferably, each described second gas flowfield plate is all welded in described second gripper shoe.
Preferably, described 3rd gas flowfield plate is welded in described first gripper shoe
Preferably, described sealing strip uses glass-ceramic composite seal.
In general, by the contemplated above technical scheme of the present invention compared with prior art, it is possible to show under acquirement
Benefit effect:
1) in the present invention, bipolar plates ensures the uniformity of anode and cathode gas distribution, improves the efficiency of collected current.
2) in the present invention, bipolar plates can improve the symmetry of electric pile structure, and in reduction pile, stress distribution is uneven
Property, reduce the probability of seal failure.
3) present invention can optimize the assembly technology of pile, simplifies the assemble flow of pile, thus improves the quality of pile
And reliability.
Accompanying drawing explanation
Fig. 1 is the structural representation of the present invention;
Fig. 2 is the decomposing schematic representation of battery unit in the present invention;
Fig. 3 is the structural representation of bipolar plates in the present invention;
Fig. 4 is the partial enlarged drawing of bipolar plates in the present invention.
Detailed description of the invention
In order to make the purpose of the present invention, technical scheme and advantage clearer, below in conjunction with drawings and Examples, right
The present invention is further elaborated.Should be appreciated that specific embodiment described herein only in order to explain the present invention, and
It is not used in the restriction present invention.If additionally, technical characteristic involved in each embodiment of invention described below
The conflict of not constituting each other just can be mutually combined.
With reference to Fig. 1~Fig. 4, a kind of outflow chamber SOFC pile, including gas buffer cavity 1, upper cover
Plate 2, lower cover 4 and battery unit 3, wherein,
Described upper cover plate 2 and lower cover 4 are respectively arranged at the top and bottom of described gas buffer cavity 1;
Described upper cover plate 2 includes the first gripper shoe and the first gas flowfield plate, and the bottom of described first gripper shoe is provided with
First open slot, described first gas flowfield plate is arranged at the first open slot of described first gripper shoe, thus with described
Gas passage is formed between one gripper shoe;
Described battery unit 3 includes N number of bipolar plates 31 and N+1 flat-plate-type solid-oxide fuel battery 32, these pairs
Pole plate 31 and flat-plate-type solid-oxide fuel battery 32 stacked on top, it is crisscross arranged;Adjacent described bipolar plates 31 is with described
Sealing strip 33 is set between flat-plate-type solid-oxide fuel battery 32, leaks for preventing gas;
Each described bipolar plates 31 all includes the second gripper shoe 311 and two the second gas flowfield plates 312, wherein, described
The top of the second gripper shoe 311 and bottom are respectively arranged with the second open slot, and each described second gas flowfield plate 312 sets respectively
Being placed at one second open slot, each described second gas flowfield plate 312 respectively and forms gas between described second gripper shoe 311
Body passage;
Additionally, described upper cover plate 2 and being also equipped with between the flat-plate-type solid-oxide fuel battery 32 of the top
For the sealing strip 33 preventing gas from leaking;
Described lower cover 4 includes that the 3rd gripper shoe and the 3rd gas flowfield plate, the top of described 3rd gripper shoe are provided with
3rd open slot, described 3rd gas flowfield plate is arranged at described 3rd open slot, it addition, described lower cover 4 be positioned at
It is also equipped with the sealing strip 33 for preventing gas from leaking between the flat-plate-type solid-oxide fuel battery 32 of lower section;
Described first gas flowfield plate, the second gas flowfield plate 312 are identical with the 3rd gas flowfield plate structure.
Further, described first gas flowfield plate is made up through pressure forming of corrosion resistant plate, and this corrosion resistant plate
Thickness is 0.1mm~0.3mm, and described first gas flowfield plate uses ferrite type stainless steel material to make, described first gas
The upper and lower surface of flow-field plate is coated respectively with conductive protection coating, and described first gas flowfield plate is welded on described first gripper shoe
On, each described second gas flowfield plate 312 is all welded in described second gripper shoe 311, described 3rd gas flowfield plate weldering
Being connected in described first gripper shoe, described sealing strip 33 uses glass-ceramic composite seal.
The bipolar plates 31 of the present invention may be used for flat-plate-type solid-oxide fuel battery 32 of connecting, it is provided that structure supports,
Distributing gas, separates fuel gas and oxidizing gas, and it is two by the gripper shoe of side trough of belt and the special gas flowfield that is fixed in groove
Plate forms, and wherein both sides groove depth and gas flow-field plate thickness can be processed the most respectively, and gas flowfield board size is slightly less than
The size of groove, slightly larger than the effective affecting acreage of fuel flat-plate-type solid-oxide fuel battery 32, is fixed on groove by spot welding
In road, thickness is slightly above the degree of depth at the edge of groove to realize good contact, realizes air seal with encapsulant thickness matching.
The the first gas flowfield plate used in the present invention preferably employs the gas flowfield plate mentioned in patent CN 104253280A.
Further, described both sides gas flowfield plate is all fixed in gripper shoe by spot welding, for ensureing gas flowfield plate
Contact flexibility, the most what time solder joint chooses surrounding.
Further, gas flowfield plate can be a monoblock, it is possible to several fritters different by whereabouts are spliced, it is achieved gas
The uniformity of stream.
According to another aspect of the present invention, additionally provide the preparation method of SOFC bipolar plates 31,
Its preparation technology is as follows:
S1: select the corrosion resistant plate of desired thickness;
S2: corrosion resistant plate is made through the twin rollers roll forming with particular roller, and waviness width and length can be passed through
Roll die accurately controls, detail referenced patent CN 104253280A.Gas flowfield plate benging after twin rollers processing
Injustice, need to be flattened into desired thickness through precision rollers machine, then through cut to required size.
One piece of corrosion resistant plate of S3: reselection, this corrosion resistant plate, then adds through machinery to definite shape through cut
Work, spot welding, laser welding are prepared as the second gripper shoe 311 with the second open slot.
S4: gas flowfield plate is placed in the second open slot of the second gripper shoe 311, is fixed on through a small amount of spot welding of surrounding and props up
On fagging, complete.
Bipolar plates 31 in the present invention can be used in the outflow chamber SOFC pile of various structure, including
Interior air flue, exterior air drain etc., can be concurrent, cross-current and counter current flow structure, the structure of different simply gripper shoes and processing
Method.Material and the coating of gas flowfield plate adjust also dependent on needs.
As it will be easily appreciated by one skilled in the art that and the foregoing is only presently preferred embodiments of the present invention, not in order to
Limit the present invention, all any amendment, equivalent and improvement etc. made within the spirit and principles in the present invention, all should comprise
Within protection scope of the present invention.
Claims (8)
1. an outflow chamber SOFC pile, it is characterised in that include gas buffer cavity (1), upper cover plate
(2), lower cover (4) and battery unit (3), wherein,
Described upper cover plate (2) and lower cover (4) are respectively arranged at the top and bottom of described gas buffer cavity (1);
Described upper cover plate (2) includes the first gripper shoe and the first gas flowfield plate, and the bottom of described first gripper shoe is provided with
One open slot, described first gas flowfield plate is arranged at the first open slot of described first gripper shoe, thus with described first
Gas passage is formed between gripper shoe;
Described battery unit (3) includes N number of bipolar plates (31) and N+1 flat-plate-type solid-oxide fuel battery (32), these
Bipolar plates (31) and flat-plate-type solid-oxide fuel battery (32) stacked on top, it is crisscross arranged;Adjacent described bipolar plates
(31) and sealing strip (33) is set between described flat-plate-type solid-oxide fuel battery (32), leak for preventing gas;
Each described bipolar plates (31) all includes the second gripper shoe (311) and two the second gas flowfield plates (312), wherein, institute
Top and the bottom of stating the second gripper shoe (311) are respectively arranged with the second open slot, each described second gas flowfield plate (312)
Be respectively arranged at one second open slot, each described second gas flowfield plate (312) respectively with described second gripper shoe (311)
Between formed gas passage;
Additionally, be also equipped with between described upper cover plate (2) and the flat-plate-type solid-oxide fuel battery (32) being positioned at the top
For the sealing strip (33) preventing gas from leaking;
Described lower cover (4) includes that the 3rd gripper shoe and the 3rd gas flowfield plate, the top of described 3rd gripper shoe are provided with
Three open slots, described 3rd gas flowfield plate is arranged at described 3rd open slot, it addition, described lower cover (4) be positioned at
It is also equipped with the sealing strip (33) for preventing gas from leaking between the flat-plate-type solid-oxide fuel battery (32) of lower section;
Described first gas flowfield plate, the second gas flowfield plate (312) are identical with the 3rd gas flowfield plate structure.
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that described first
Gas flowfield plate is made up through pressure forming of corrosion resistant plate, and the thickness of this corrosion resistant plate is 0.1mm~0.3mm.
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that described first
Gas flowfield plate uses ferrite type stainless steel material to make.
A kind of outflow chamber the most according to claim 3 SOFC pile, it is characterised in that described first
The upper and lower surface of gas flowfield plate has been respectively coated with high-temperature electric conduction ceramic layer.
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that described first
Gas flowfield plate is welded in described first gripper shoe.
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that each described
Second gas flowfield plate (312) is all welded on described second gripper shoe (311).
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that the described 3rd
Gas flowfield plate is welded in described 3rd gripper shoe
A kind of outflow chamber the most according to claim 1 SOFC pile, it is characterised in that described sealing
Bar (33) uses glass-ceramic composite seal.
Priority Applications (1)
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CN201610631780.9A CN106252697A (en) | 2016-08-04 | 2016-08-04 | A kind of outflow chamber SOFC pile |
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CN201610631780.9A CN106252697A (en) | 2016-08-04 | 2016-08-04 | A kind of outflow chamber SOFC pile |
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Cited By (6)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN106602119A (en) * | 2016-12-30 | 2017-04-26 | 华中科技大学 | Self-tightening outer flow cavity solid oxide fuel cell stack |
CN106816613A (en) * | 2016-12-30 | 2017-06-09 | 华中科技大学 | A kind of indirect internal reforming SOFC pile |
CN109167084A (en) * | 2018-09-06 | 2019-01-08 | 常州联德电子有限公司 | A kind of solid oxide fuel cell metal connector and its quick molding method |
CN109904465A (en) * | 2019-03-01 | 2019-06-18 | 徐州华清京昆能源有限公司 | A kind of solid oxide fuel cell electrode structure |
CN110600776A (en) * | 2019-09-29 | 2019-12-20 | 武汉华科福赛新能源有限责任公司 | Internal reforming solid oxide fuel cell stack |
CN112928297A (en) * | 2021-01-25 | 2021-06-08 | 中国第一汽车股份有限公司 | Fuel cell flow field plate |
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CN105161743A (en) * | 2015-10-14 | 2015-12-16 | 中国科学院宁波材料技术与工程研究所 | Anode of high-temperature solid-state fuel cell and cell stack unit |
CN105355942A (en) * | 2015-10-29 | 2016-02-24 | 华中科技大学 | Outflow chamber based air-flow chamber sealing device for solid oxide fuel cell |
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US20100019400A1 (en) * | 2008-07-23 | 2010-01-28 | Gm Global Technology Operations, Inc. | Wvt design for reduced mass and improved sealing reliability |
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Publication number | Priority date | Publication date | Assignee | Title |
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CN106602119A (en) * | 2016-12-30 | 2017-04-26 | 华中科技大学 | Self-tightening outer flow cavity solid oxide fuel cell stack |
CN106816613A (en) * | 2016-12-30 | 2017-06-09 | 华中科技大学 | A kind of indirect internal reforming SOFC pile |
CN106602119B (en) * | 2016-12-30 | 2019-05-21 | 华中科技大学 | A kind of self-tightening type outflow chamber solid oxide fuel cell pile |
CN109167084A (en) * | 2018-09-06 | 2019-01-08 | 常州联德电子有限公司 | A kind of solid oxide fuel cell metal connector and its quick molding method |
CN109904465A (en) * | 2019-03-01 | 2019-06-18 | 徐州华清京昆能源有限公司 | A kind of solid oxide fuel cell electrode structure |
CN110600776A (en) * | 2019-09-29 | 2019-12-20 | 武汉华科福赛新能源有限责任公司 | Internal reforming solid oxide fuel cell stack |
CN112928297A (en) * | 2021-01-25 | 2021-06-08 | 中国第一汽车股份有限公司 | Fuel cell flow field plate |
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