CN105753154B - 一种基于海绵铁-氨氧化微生物***同步去除抗炎药与氨氮的方法 - Google Patents
一种基于海绵铁-氨氧化微生物***同步去除抗炎药与氨氮的方法 Download PDFInfo
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- CN105753154B CN105753154B CN201610162396.9A CN201610162396A CN105753154B CN 105753154 B CN105753154 B CN 105753154B CN 201610162396 A CN201610162396 A CN 201610162396A CN 105753154 B CN105753154 B CN 105753154B
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- XKMRRTOUMJRJIA-UHFFFAOYSA-N ammonia nh3 Chemical compound N.N XKMRRTOUMJRJIA-UHFFFAOYSA-N 0.000 title claims abstract description 52
- 230000003647 oxidation Effects 0.000 title claims abstract description 49
- 238000007254 oxidation reaction Methods 0.000 title claims abstract description 49
- 230000002906 microbiologic effect Effects 0.000 title claims abstract description 36
- 239000002260 anti-inflammatory agent Substances 0.000 title claims abstract description 33
- 229940121363 anti-inflammatory agent Drugs 0.000 title claims abstract description 31
- 238000000034 method Methods 0.000 title claims abstract description 23
- QYTBWVFCSVDTEC-UHFFFAOYSA-N azane;iron Chemical compound N.[Fe] QYTBWVFCSVDTEC-UHFFFAOYSA-N 0.000 title claims abstract description 9
- XEEYBQQBJWHFJM-UHFFFAOYSA-N Iron Chemical compound [Fe] XEEYBQQBJWHFJM-UHFFFAOYSA-N 0.000 claims abstract description 101
- QGZKDVFQNNGYKY-UHFFFAOYSA-N Ammonia Chemical compound N QGZKDVFQNNGYKY-UHFFFAOYSA-N 0.000 claims abstract description 88
- 238000006243 chemical reaction Methods 0.000 claims abstract description 88
- 235000015097 nutrients Nutrition 0.000 claims abstract description 58
- 229910052742 iron Inorganic materials 0.000 claims abstract description 46
- 229910021529 ammonia Inorganic materials 0.000 claims abstract description 42
- RZVAJINKPMORJF-UHFFFAOYSA-N Acetaminophen Chemical compound CC(=O)NC1=CC=C(O)C=C1 RZVAJINKPMORJF-UHFFFAOYSA-N 0.000 claims abstract description 33
- 230000015556 catabolic process Effects 0.000 claims abstract description 23
- 229910021536 Zeolite Inorganic materials 0.000 claims abstract description 15
- HNPSIPDUKPIQMN-UHFFFAOYSA-N dioxosilane;oxo(oxoalumanyloxy)alumane Chemical compound O=[Si]=O.O=[Al]O[Al]=O HNPSIPDUKPIQMN-UHFFFAOYSA-N 0.000 claims abstract description 15
- 239000010457 zeolite Substances 0.000 claims abstract description 15
- 230000001360 synchronised effect Effects 0.000 claims abstract description 14
- 229960005489 paracetamol Drugs 0.000 claims abstract description 12
- DCOPUUMXTXDBNB-UHFFFAOYSA-N diclofenac Chemical compound OC(=O)CC1=CC=CC=C1NC1=C(Cl)C=CC=C1Cl DCOPUUMXTXDBNB-UHFFFAOYSA-N 0.000 claims abstract description 11
- 229960001259 diclofenac Drugs 0.000 claims abstract description 11
- 238000003541 multi-stage reaction Methods 0.000 claims abstract description 4
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims description 77
- 239000000243 solution Substances 0.000 claims description 61
- 229910000030 sodium bicarbonate Inorganic materials 0.000 claims description 30
- UIIMBOGNXHQVGW-UHFFFAOYSA-M sodium bicarbonate Substances [Na+].OC([O-])=O UIIMBOGNXHQVGW-UHFFFAOYSA-M 0.000 claims description 30
- 239000010802 sludge Substances 0.000 claims description 23
- IOVCWXUNBOPUCH-UHFFFAOYSA-M Nitrite anion Chemical compound [O-]N=O IOVCWXUNBOPUCH-UHFFFAOYSA-M 0.000 claims description 22
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 claims description 22
- 239000001301 oxygen Substances 0.000 claims description 22
- 229910052760 oxygen Inorganic materials 0.000 claims description 22
- 238000011049 filling Methods 0.000 claims description 16
- 238000004140 cleaning Methods 0.000 claims description 15
- 239000006228 supernatant Substances 0.000 claims description 15
- NLXLAEXVIDQMFP-UHFFFAOYSA-N Ammonia chloride Chemical compound [NH4+].[Cl-] NLXLAEXVIDQMFP-UHFFFAOYSA-N 0.000 claims description 13
- 244000005700 microbiome Species 0.000 claims description 13
- 239000011259 mixed solution Substances 0.000 claims description 11
- 239000010865 sewage Substances 0.000 claims description 11
- 238000009629 microbiological culture Methods 0.000 claims description 10
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 claims description 9
- 230000004913 activation Effects 0.000 claims description 9
- 238000001556 precipitation Methods 0.000 claims description 9
- 238000010790 dilution Methods 0.000 claims description 8
- 239000012895 dilution Substances 0.000 claims description 8
- 239000003814 drug Substances 0.000 claims description 8
- 238000002156 mixing Methods 0.000 claims description 8
- 239000002245 particle Substances 0.000 claims description 7
- 239000008399 tap water Substances 0.000 claims description 7
- 235000020679 tap water Nutrition 0.000 claims description 7
- VEXZGXHMUGYJMC-UHFFFAOYSA-N Hydrochloric acid Chemical compound Cl VEXZGXHMUGYJMC-UHFFFAOYSA-N 0.000 claims description 6
- 239000007788 liquid Substances 0.000 claims description 6
- 239000005416 organic matter Substances 0.000 claims description 6
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- 230000001590 oxidative effect Effects 0.000 claims description 3
- 239000000843 powder Substances 0.000 claims description 3
- 238000004062 sedimentation Methods 0.000 claims description 3
- 238000002791 soaking Methods 0.000 claims description 3
- LPXPTNMVRIOKMN-UHFFFAOYSA-M sodium nitrite Substances [Na+].[O-]N=O LPXPTNMVRIOKMN-UHFFFAOYSA-M 0.000 claims description 3
- 239000013589 supplement Substances 0.000 claims description 2
- 230000001186 cumulative effect Effects 0.000 claims 1
- 238000006731 degradation reaction Methods 0.000 abstract description 20
- 230000000694 effects Effects 0.000 abstract description 8
- 230000035484 reaction time Effects 0.000 abstract description 3
- 239000000203 mixture Substances 0.000 description 7
- 229940021182 non-steroidal anti-inflammatory drug Drugs 0.000 description 7
- 230000008569 process Effects 0.000 description 7
- 238000009825 accumulation Methods 0.000 description 5
- 238000007259 addition reaction Methods 0.000 description 5
- 230000001651 autotrophic effect Effects 0.000 description 5
- 230000008859 change Effects 0.000 description 5
- 230000003110 anti-inflammatory effect Effects 0.000 description 4
- 229940079593 drug Drugs 0.000 description 4
- 239000011159 matrix material Substances 0.000 description 4
- 238000002360 preparation method Methods 0.000 description 4
- 230000001954 sterilising effect Effects 0.000 description 4
- PDNNQADNLPRFPG-UHFFFAOYSA-N N.[O] Chemical compound N.[O] PDNNQADNLPRFPG-UHFFFAOYSA-N 0.000 description 3
- 229920001222 biopolymer Polymers 0.000 description 3
- 238000010828 elution Methods 0.000 description 3
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- HEFNNWSXXWATRW-UHFFFAOYSA-N Ibuprofen Chemical compound CC(C)CC1=CC=C(C(C)C(O)=O)C=C1 HEFNNWSXXWATRW-UHFFFAOYSA-N 0.000 description 2
- 229910002651 NO3 Inorganic materials 0.000 description 2
- NHNBFGGVMKEFGY-UHFFFAOYSA-N Nitrate Chemical compound [O-][N+]([O-])=O NHNBFGGVMKEFGY-UHFFFAOYSA-N 0.000 description 2
- 239000002253 acid Substances 0.000 description 2
- 230000002708 enhancing effect Effects 0.000 description 2
- 239000008239 natural water Substances 0.000 description 2
- 239000000041 non-steroidal anti-inflammatory agent Substances 0.000 description 2
- 239000002574 poison Substances 0.000 description 2
- 239000010801 sewage sludge Substances 0.000 description 2
- 239000000126 substance Substances 0.000 description 2
- 238000012360 testing method Methods 0.000 description 2
- 125000005273 2-acetoxybenzoic acid group Chemical class 0.000 description 1
- QGZKDVFQNNGYKY-UHFFFAOYSA-O Ammonium Chemical compound [NH4+] QGZKDVFQNNGYKY-UHFFFAOYSA-O 0.000 description 1
- VHUUQVKOLVNVRT-UHFFFAOYSA-N Ammonium hydroxide Chemical compound [NH4+].[OH-] VHUUQVKOLVNVRT-UHFFFAOYSA-N 0.000 description 1
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 1
- CWYNVVGOOAEACU-UHFFFAOYSA-N Fe2+ Chemical compound [Fe+2] CWYNVVGOOAEACU-UHFFFAOYSA-N 0.000 description 1
- MQHWFIOJQSCFNM-UHFFFAOYSA-L Magnesium salicylate Chemical compound [Mg+2].OC1=CC=CC=C1C([O-])=O.OC1=CC=CC=C1C([O-])=O MQHWFIOJQSCFNM-UHFFFAOYSA-L 0.000 description 1
- IOVCWXUNBOPUCH-UHFFFAOYSA-N Nitrous acid Chemical compound ON=O IOVCWXUNBOPUCH-UHFFFAOYSA-N 0.000 description 1
- ABBQHOQBGMUPJH-UHFFFAOYSA-M Sodium salicylate Chemical compound [Na+].OC1=CC=CC=C1C([O-])=O ABBQHOQBGMUPJH-UHFFFAOYSA-M 0.000 description 1
- LGBWVEGZBZNNSG-UHFFFAOYSA-N [N].[N].N Chemical compound [N].[N].N LGBWVEGZBZNNSG-UHFFFAOYSA-N 0.000 description 1
- 230000000844 anti-bacterial effect Effects 0.000 description 1
- 229940124599 anti-inflammatory drug Drugs 0.000 description 1
- 230000001741 anti-phlogistic effect Effects 0.000 description 1
- 229940088710 antibiotic agent Drugs 0.000 description 1
- 238000013459 approach Methods 0.000 description 1
- XABJJJZIQNZSIM-UHFFFAOYSA-N azane;phenol Chemical compound [NH4+].[O-]C1=CC=CC=C1 XABJJJZIQNZSIM-UHFFFAOYSA-N 0.000 description 1
- 229940125717 barbiturate Drugs 0.000 description 1
- 230000008901 benefit Effects 0.000 description 1
- 229910052799 carbon Inorganic materials 0.000 description 1
- 150000001875 compounds Chemical class 0.000 description 1
- 238000000205 computational method Methods 0.000 description 1
- 238000012258 culturing Methods 0.000 description 1
- 230000007423 decrease Effects 0.000 description 1
- 238000013461 design Methods 0.000 description 1
- 238000001784 detoxification Methods 0.000 description 1
- 238000011161 development Methods 0.000 description 1
- 238000006073 displacement reaction Methods 0.000 description 1
- 230000007613 environmental effect Effects 0.000 description 1
- 238000002474 experimental method Methods 0.000 description 1
- 210000003608 fece Anatomy 0.000 description 1
- 239000000945 filler Substances 0.000 description 1
- 238000011010 flushing procedure Methods 0.000 description 1
- 239000001257 hydrogen Substances 0.000 description 1
- 229910052739 hydrogen Inorganic materials 0.000 description 1
- 125000004435 hydrogen atom Chemical class [H]* 0.000 description 1
- 238000007654 immersion Methods 0.000 description 1
- 230000000977 initiatory effect Effects 0.000 description 1
- 229940072082 magnesium salicylate Drugs 0.000 description 1
- 230000007246 mechanism Effects 0.000 description 1
- 230000004060 metabolic process Effects 0.000 description 1
- QJGQUHMNIGDVPM-UHFFFAOYSA-N nitrogen group Chemical group [N] QJGQUHMNIGDVPM-UHFFFAOYSA-N 0.000 description 1
- 238000002161 passivation Methods 0.000 description 1
- 230000007096 poisonous effect Effects 0.000 description 1
- 238000012545 processing Methods 0.000 description 1
- 230000002787 reinforcement Effects 0.000 description 1
- 238000011160 research Methods 0.000 description 1
- 229960004025 sodium salicylate Drugs 0.000 description 1
- 230000003637 steroidlike Effects 0.000 description 1
- 239000000758 substrate Substances 0.000 description 1
- 238000012549 training Methods 0.000 description 1
- 238000002604 ultrasonography Methods 0.000 description 1
- 235000021419 vinegar Nutrition 0.000 description 1
- 239000000052 vinegar Substances 0.000 description 1
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Classifications
-
- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F3/00—Biological treatment of water, waste water, or sewage
- C02F3/30—Aerobic and anaerobic processes
-
- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F2101/00—Nature of the contaminant
- C02F2101/10—Inorganic compounds
- C02F2101/16—Nitrogen compounds, e.g. ammonia
-
- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F2101/00—Nature of the contaminant
- C02F2101/30—Organic compounds
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- Life Sciences & Earth Sciences (AREA)
- Biodiversity & Conservation Biology (AREA)
- Microbiology (AREA)
- Hydrology & Water Resources (AREA)
- Engineering & Computer Science (AREA)
- Environmental & Geological Engineering (AREA)
- Water Supply & Treatment (AREA)
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Purification Treatments By Anaerobic Or Anaerobic And Aerobic Bacteria Or Animals (AREA)
Abstract
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CN201610162396.9A CN105753154B (zh) | 2016-03-21 | 2016-03-21 | 一种基于海绵铁-氨氧化微生物***同步去除抗炎药与氨氮的方法 |
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CN201610162396.9A CN105753154B (zh) | 2016-03-21 | 2016-03-21 | 一种基于海绵铁-氨氧化微生物***同步去除抗炎药与氨氮的方法 |
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CN105753154B true CN105753154B (zh) | 2018-05-15 |
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CN106865760A (zh) * | 2017-03-15 | 2017-06-20 | 东北电力大学 | 海绵铁填料强化厌氧氨氧化反应器脱氮效能的工艺 |
CN107973495A (zh) * | 2017-12-29 | 2018-05-01 | 中国科学院南京地理与湖泊研究所 | 多级升流式地表水体氮素和有机质同步去除的装置和方法 |
CN108611276A (zh) * | 2018-04-16 | 2018-10-02 | 仲恺农业工程学院 | 一种利用微藻对酒糟废水进行资源化处理的方法 |
CN109574399B (zh) * | 2018-12-27 | 2021-07-30 | 南京大学 | 一种基于富集硝化细菌强化去除污水中双氯芬酸的方法 |
CN113912179B (zh) * | 2021-10-15 | 2023-09-29 | 北京工业大学 | 一种厌氧铁盐氧化氨氮及同步脱氮污泥的快速培养方法 |
Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP3937664B2 (ja) * | 1999-10-12 | 2007-06-27 | 栗田工業株式会社 | 生物学的窒素除去方法および装置 |
CN101525179A (zh) * | 2009-04-20 | 2009-09-09 | 广东省微生物研究所 | 一种厌氧氨氧化处理低浓度氨氮废水的方法 |
CN101709278A (zh) * | 2009-11-23 | 2010-05-19 | 浙江省环境保护科学设计研究院 | 高浓度亚硝化细菌的规模化培养方法及其用途 |
CN104193002A (zh) * | 2014-09-24 | 2014-12-10 | 山东大学 | 一种基于零价铁耦合厌氧氨氧化高效处理含氮废水的方法 |
CN105347472A (zh) * | 2015-11-15 | 2016-02-24 | 农业部沼气科学研究所 | 高氨氮废水的好氧生物脱氮工艺 |
-
2016
- 2016-03-21 CN CN201610162396.9A patent/CN105753154B/zh active Active
Patent Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP3937664B2 (ja) * | 1999-10-12 | 2007-06-27 | 栗田工業株式会社 | 生物学的窒素除去方法および装置 |
CN101525179A (zh) * | 2009-04-20 | 2009-09-09 | 广东省微生物研究所 | 一种厌氧氨氧化处理低浓度氨氮废水的方法 |
CN101709278A (zh) * | 2009-11-23 | 2010-05-19 | 浙江省环境保护科学设计研究院 | 高浓度亚硝化细菌的规模化培养方法及其用途 |
CN104193002A (zh) * | 2014-09-24 | 2014-12-10 | 山东大学 | 一种基于零价铁耦合厌氧氨氧化高效处理含氮废水的方法 |
CN105347472A (zh) * | 2015-11-15 | 2016-02-24 | 农业部沼气科学研究所 | 高氨氮废水的好氧生物脱氮工艺 |
Non-Patent Citations (1)
Title |
---|
金属离子对厌氧氨氧化反应器效能的影响;彭厦等;《中国给水排水》;20121130;第28卷(第21期);第30-33页 * |
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Application publication date: 20160713 Assignee: Hezhou Tongyun Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045190 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Foshan shangxiaoyun Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045186 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Dongguan Yaluo Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045183 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Dongguan Creative Environmental New Materials Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045170 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: GUANGZHOU DINGRAN MEDICINE TECHNOLOGY Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045223 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Liuzhou Tengtu Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045213 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Liuzhou Renjia Biotechnology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045212 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Beihai anfeigao Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045197 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 Application publication date: 20160713 Assignee: Guangzhou Kelang Medical Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980045194 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231031 |
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Application publication date: 20160713 Assignee: Yantai Oushilan Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980046612 Denomination of invention: A Method for Simultaneous Removal of Anti-inflammatory Drugs and Ammonia Nitrogen Based on Sponge Iron Ammonia Oxidizing Microbial System Granted publication date: 20180515 License type: Common License Record date: 20231109 |
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Application publication date: 20160713 Assignee: Chongqing Longjinsheng Biotechnology Group Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980048318 Denomination of invention: A method for synchronously removing anti-inflammatory drugs and ammonia nitrogen based on sponge iron ammonia oxidizing microbial system Granted publication date: 20180515 License type: Common License Record date: 20231124 Application publication date: 20160713 Assignee: Guangdong Lvyuan Environmental Protection Technology Co.,Ltd. Assignor: Institute of Microbiology, Guangdong Academy of Sciences Contract record no.: X2023980048310 Denomination of invention: A method for synchronously removing anti-inflammatory drugs and ammonia nitrogen based on sponge iron ammonia oxidizing microbial system Granted publication date: 20180515 License type: Common License Record date: 20231124 |
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