CN103804097B - A kind of fertilizer containing Antiphytoviral fertilizer additive - Google Patents
A kind of fertilizer containing Antiphytoviral fertilizer additive Download PDFInfo
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Abstract
The present invention relates to a kind of Antiphytoviral fertilizer additive and the fertilizer containing this additive, the additive of this Antiphytoviral contains containing secondary and micro-element fertilizers, organic acid, anti-plant virus agent and trace mineral supplement; Fertilizer containing this additive is made up of the additive of straight fertilizer or compound manure and Antiphytoviral fertilizer, and the content of additive is the 0.1-5% of fertilizer gross weight.Advantage of the present invention is: when using additive or the fertilizer of this Antiphytoviral, and its obvious effect of increasing production, can prevent and treat some plant viruses in addition.
Description
Technical field
The present invention relates to a kind of additive of using in agroforestry fertilizer and fertilizer thereof, specifically, relate to instant noresidue Antiphytoviral fertilizer additive and the fertilizer containing this additive thereof.
Background technology
Fertilizer is the grain of plant, is one of basic substance improving agriculture production.For a long time, in agriculture production, generally use the fertilizer of a large amount of nitrogenous, phosphorus, potassium, serve negative impact so not only to the band such as agriculture production and environment, and agriculture production cost also constantly increases, thus have impact on agricultural development.
In order to address this problem, in order to improve utilization rate of fertilizer, the research of agricultural science personnel of China have carried out a large amount of research work, achieve some progress.Such as CN1546438A discloses a kind of particulate slow-release fertilizer containing chitin, and this fertilizer is made up of containing the powder of chitin, 5-35 % by weight binding agent, 0-40 % by weight weighting agent, 0-20 % by weight activeconstituents and 0-10 % by weight sealing agent 15-80 % by weight fertilizer components, 10-80 % by weight.This fertilizer has the dual-use function of slowly-releasing and improvement soil.CN1328769A discloses a kind of composition of combining for the chitosan, other composition such as choline chloride 60, trimethyl-glycine, light rare earths, amino acids, vitamins, thanomin, the trace element fertilizer sour with non-toxic organic that are greater than 75% containing water soluble chitosan, particularly lower molecular weight and degree of deacetylation of various farm crop and application thereof.CN1040097C, 1072196C, 1078577C, 1169757C, 1535939A, 1583648A, 1587211A, 1609075A, 1609076A, 1609077A, 1654439A also disclose similar research work result in addition.In addition, many patents or patent application is also had to relate to trace element fertilizer, such as CN1530350A, 1328769A etc.
In addition, plant virus is one of pathogenic agent affecting crop yield and quality, often brings huge disaster to agriculture production.Plant virus major part belongs to single strand RNA virus, and minority is DNA virus.Its grown form have shaft-like, thread and etc. axisymmetric subsphaeroidal icosahedron.Though plant virus is strict cytozoon, specificity is strong, and often a kind of virus can colonize on not of the same race, that genus is even not equal plant.As tobacco mosaic virus (TMV) can infect ten Duo Ge sections, more than 200 kind of draft and xylophyta.In order to eliminate the impact of plant virus on agriculture production, people have also carried out a large amount of research work.Such as CN1042588C discloses a kind of antiviral composition, it contains 0.3-1.0 % by weight ribavirin, 0.5-2.0 % by weight zinc sulfate, 3-30 % by weight soap powder, all the other are copper sulfate, sucrose, yield increasing fungus, trace element and weighting agent, and it can be used for the control of the various viroses of plant.CN1618288A discloses a kind of prevention and cure agent for plant virus diseases, and it is by 35-55 % by weight moroxydine hydrochloride, 35-55 % by weight venus crystals, 7.5-15 % by weight amantadine hydrochloride or chitin.In addition, CN1327740A, 1505932A, 1173631C also disclose agent for preventing and treating plant virus.
But, current Antiphytoviral fertilizer additive, such as CN100463882C, produce many being uniformly mixed for a long time under the high temperature conditions and react, need a large amount of heat energy, production cost is very high, is unfavorable for the energy-saving and emission-reduction work of enterprise; And the production time is generally long, contracting and reaction needed 2 ~ 8 hours, production efficiency is lower, and product competitiveness is low, is unfavorable for market competition.And because it is poorly soluble, specific absorption is low, potential of hydrogen is not suitable for, use after have the problems such as residual, make troubles to agriculture production.
Multiple inorganic chemistry element combines, and easily causes antagonism and precipitation to make line clogging.
Summary of the invention
The object of the invention is to overcome the deficiencies in the prior art part, and provide instant, the fertilizer of additive containing anti-phytopathy of noresidue, the i.e. additive of Antiphytoviral fertilizer and the fertilizer containing this additive thereof.
The object of the invention is to realize in the following way: the described fertilizer containing Antiphytoviral fertilizer additive; this fertilizer is made up of straight fertilizer or compound manure and Antiphytoviral fertilizer additive; the content of additive is the 0.1-5% of fertilizer gross weight; specifically; after straight fertilizer or compound manure fully being mixed with the additive of Antiphytoviral fertilizer, make the fertiliser granulates of diameter 4mm through Squeezinggranulator.
Straight fertilizer refers to single fertilizer, is selected from the fertilizer of nitrogenous, phosphorus or potassium, as urea, ammonium nitrate, potassium primary phosphate or potassium sulfate;
Compound manure refers to the fertilizer at two or more, is selected from the above composite fertilizer of binary compound fertilizer, Nitrogen, Phosphorus and Potassium or ternary, as primary ammonium phosphate or nitrogen-phosphorus-potassium compound fertilizer.
In this fertilizer, contained Antiphytoviral fertilizer additive is made up of following component: with parts by weight
Secondary and micro-element fertilizers 20-70 part
Organic acid 5-15 part
Anti-plant virus agent 1-7 part
Trace mineral supplement 1-10 part
Described secondary and micro-element fertilizers is the mixture of 9 kinds of secondary and micro-element fertilizers of calcareous fertilisers, fertiliser containing magnesium, sulfur fertilizer, boron fertilizer, molydbenum fertilizer, zinc fertilizer, manganese fertilizer, iron fertilizer and copper fertilizer;
The preparation method of Antiphytoviral fertilizer additive: 9 kinds of secondary and micro-element fertilizers mixtures of calcareous fertilisers, fertiliser containing magnesium, sulfur fertilizer, boron fertilizer, molydbenum fertilizer, zinc fertilizer, manganese fertilizer, iron fertilizer and copper fertilizer, content ratio is 10-20: 8-18: 4-10: 2-5: 0.5-1.5: 2-6: 3-8: 6-10: 1-4 by weight respectively, mixture is added in mixing machine, add in mixture and organic acid citric acid, detritus acid or oxalic acid by above-mentioned part by weight, placement 4 hours is released in abundant mixing after 0.5 hour, stand-by, then anti-plant virus agent is added according to the above ratio, be selected from one or more and be selected from ribavirin, triazolone, triadimenol, olefin conversion, moroxydine hydrochloride, triacontanol price quote, polyoxyethylene sorbitol, sodium lauryl sulphate, venus crystals, the anti-plant virus agent of copper sulfate or zinc sulfate, be added in the trace mineral supplement that oneself configures in advance after abundant mixing, wherein, trace mineral supplement specifically consists of, be weight %: urea 28, Sodium hexametaphosphate 99 3, Repone K 7, sodium lignosulfonate 6, sodium polyacrylate 2, Zinc Sulphate Heptahydrate 1.8, tin anhydride 0.7, boric acid 0.4, magnesium sulfate heptahydrate 0.2, cupric sulfate pentahydrate copper 0.06, four water manganous sulfates 0.05, seven water ammonium molybdates 0.01, heptahydrate 0.002, sodium-acetate 1.8 and trimethyl-glycine 0.5, the rest is water.
Described calcareous fertilisers are calcium carbonate, calcium sulfate or calcium phosphate;
Described fertiliser containing magnesium is magnesium sulfate, magnesium chloride or fused(calcium magnesium)phosphate;
Described sulfur fertilizer is ammonium sulfate, sulphur nitric acid or ammonium sulfurous iron ore;
Described boron fertilizer is boric acid or borax;
Described molydbenum fertilizer is ammonium molybdate or Sodium orthomolybdate;
Described zinc fertilizer is Zinc vitriol, zinc chloride or zinc oxide;
Described manganese fertilizer is three anhydrous manganeses or Manganous chloride tetrahydrate;
Described iron fertilizer is seven ferric sulfate hydrates, ferrous ammonium sulphate or iron protoxide;
Described copper fertilizer is Salzburg vitriol or cupric oxide;
Described organic acid is that one or more are selected from organic acid that is natural and/or synthesis, and being selected from is detritus acid, lemon or oxalic acid;
Described anti-plant virus agent is that one or more are selected from the anti-plant virus agent of chemical pesticide or biological pesticide, and one or more are selected from the anti-plant virus agent of ribavirin, triazolone, triadimenol, olefin conversion, moroxydine hydrochloride, triacontanol price quote, polyoxyethylene sorbitol, sodium lauryl sulphate, venus crystals, copper sulfate or zinc sulfate.
Preferably, in this fertilizer, contained Antiphytoviral fertilizer additive is made up of following component: with parts by weight
Secondary and micro-element fertilizers 30-60 part
Organic acid 8-12 part
Anti-plant virus agent 2-5 part
Trace mineral supplement 2-8 part.
More preferably, in this fertilizer, contained Antiphytoviral fertilizer additive is made up of following component: with parts by weight
Secondary and micro-element fertilizers 40-50 part
Organic acid 10-12 part
Anti-plant virus agent 2-4 part
Trace mineral supplement 4-8 part.
Calcium is the constituent of cell walls, the synthesis of protein is had certain effect, also be the cofactor of some enzymatic reaction, and to regulating the physiological equilibrium of medium to have special effect, therefore, during crop calcium deficiency, plant is short and small, root system development is bad, cell walls calcium deficiency, easily by Virus entry, can perish time serious.
Magnesium is chlorophyll constitution element, is the activator of a lot of enzyme, can also promote the synthesis of fat, also participate in the metabolism of nitrogen.During crop magnesium deficiency, blade reticulattion is in yellow or white, and even overstrike is even downright bad.The herbage of magnesium deficiency can cause livestock tic sick.
Sulphur is the component of protein and enzyme, is also present in some physiologically active substance, is also an integral part of nitrogenase system.During crop a lack of sulfur, growth is subject to serious hindrance, blade chlorisis or yellow.
Boron has good effect to the growth of crop, breeding, and during crop boron deficiency, merismatic cell differentiation procedure is hindered, even withered.Boron can also promote the normal development of reproductive organ, has promoter action, can improve the nitrogenase activity of leguminous crop root nodule bacterium, increase amount of nitrogen fixation, can also increase the resistance of crop the synthesis and transport making sugar in object.
Molybdenum can promote the assimilation of nitric nitrogen, has desirable influence to biological nitrogen fixation, can also increase the intensity of photosynthesis of blade.
Zinc can promote that crop carries out photosynthesis, also participates in the synthesis of growth hormone in plant materials, such as, participate in the synthesis of indolylacetic acid, and zinc is the moiety of multiple enzyme, such as, be the moiety of glutamate dehydrogenase, malate dehydrogenase (malic acid dehydrogenase), Phospholipid hydrolase etc.
Manganese participates in the photodissociation of water in photosynthesis directly in plant chloroplast with combined, during crop manganese deficiency, the photodissociation of water is then suppressed, thus affects the photosynthesis of crop.Manganese also has a certain impact to crop respiration, therefore, during crop manganese deficiency, will cause a series of metabolic disorder.Manganese participates in the effect of nitrate-nitrogen reduction ammonification, if crop manganese deficiency, nitric nitrogen can be made at crop cylinder accumulation.Manganese is the promoting agent of ribonucleic acid polymerase, is again the activator of pepx etc., is therefore conducive to protein synthesis.Manganese can also promote seed germination and seeding previous vigor, accelerates pollen germination and pollen tube growth, improves setting percentage.
Iron is indispensable to chlorophyll formation, is the important component part of plant materials internal oxidition albumen, is many oxydase in plant materials, as the integral part of Terminal oxidase, catalase etc., is also the best activator of Chlorophyll.
Copper is the composition of the multiple enzyme such as polyphenoloxidase in plant materials, also relevant with chlorophyll formation, also participates in protein and sugar class metabolism.
In a word, the integral part of trace element enzyme or coenzyme often in plant materials, has very strong specificity, is that crop growth is indispensable and can not mutually replace.
Plant virus is a kind of non-parasitics non cellular organism, after in its invaded plants body, provides genetic information, by the Synthesis replication-competent virus of parasitic cell to parasitic cell.The basic practical measures of current control plant virus is chemical pesticide control, main two classes of medicament of its control plant virus, one class is azole medicament, such as ribavirin, and they can affect viral nucleic acid and the ribosomal combination of host and suppress copying and breeding of virus; Another kind of is moroxydine hydrochloride second copper class medicament, is a kind of wide spectrum, hypovirus control agent, and the synthesis of suppression or break virus nucleic acid and protein, can also combinationally use its two class in addition.
The component of Antiphytoviral agent addition agent of the present invention is mixed according to aforementioned proportion and just can prepare composition of the present invention.Mixing equipment is mixing equipment general in technical field of fertilizers.
The present invention is on Antiphytoviral fertilizer additive basis disclosed in CN100463882C, improve preparation technology further, remove insoluble crustaceans material, add anti-virus formulation and trace element, adjust the ratio of each component, prepare novel instant noresidue Antiphytoviral fertilizer additive, described instant noresidue Antiphytoviral fertilizer additive be a kind of add water to stir need not heat and special fertilizer that rapid solution is made.Its formula and making method are on the bases such as the necessary major element fertilizer nitrogen of farm crop, phosphorus, potassium and trace element fertilizer zinc, iron, calcium, silicon, copper, magnesium, manganese, boron, molybdenum, cobalt, selenium, sulphur, reasonably the outstanding content increasing zinc, selenium element, selects the compound of best constituent content proportioning and component.Namely this compound ensures the content of element, ensures that again speed is water-soluble, does not produce again the material of precipitin reaction to each other.
The present invention compared with prior art, have the following advantages: by constructing the water soluble fertilizer of the present invention that full instant powder macroelement is formed, after using this water-soluble chemical fertilizer, the soil aggregation grain pattern of stability can be formed, to improve the gas permeability of soil, improve the chemical physics environment of various nutritive element in soil, increase the adsorptive capacity on grogs surface, increase the adduction that various nutrition becomes material, nutrition protective belt can be formed rapidly at plant root after using, increase nitrogen, phosphorus, the velocity of diffusion of the nutrients such as potassium in soil and migration distance, promote root system absorbing moisture content and nutrient.Soil water retention, fertilizer-preserving ability can be improved, improve the water ratio of soil, play and suppress evaporation soil moisture conservation effect, improve the replacement receptivity of soil, the breeding of effective microbe in soil can be stimulated to increase, the micro-ecological environment of improvement soil.The synthesis of the nutritive elements such as amino acid, soluble sugar, VITAMIN can be promoted, reduce the harmful substance contents such as nitrate, heavy metal.And additive in the present invention is instant, noresidue, unblocked and can volume increase be increased income when can make drip irrigation.
Embodiment
Embodiment 1
First the fertilizer additive of anti-plant virus is prepared.The method preparing secondary and micro-element fertilizers is: take a certain amount of calcium carbonate, magnesium sulfate, ammonium sulfate, borax, ammonium molybdate, Zinc vitriol, three anhydrous manganeses, seven ferric sulfate hydrates and Salzburg vitriol respectively, trace element fertilizer ratio is 10: 8: 4: 2: 0.5: 2: 3: 6: 1 by weight respectively, at normal temperatures and pressures these raw materials are fully mixed, stand-by, then, taking this mixture 50kg is added in this mixing machine, add 10kg citric acid again, placement 4 hours is discharged in abundant mixing after 0.5 hour, after terminating storage period, add 4kg ribavirin, be added in the trace mineral supplement giving and first preparing after mixing, trace mineral supplement is urea 28, Sodium hexametaphosphate 99 3, Repone K 7, sodium lignosulfonate 6, sodium polyacrylate 2, Zinc Sulphate Heptahydrate 1.8, tin anhydride 0.7, boric acid 0.4, magnesium sulfate heptahydrate 0.2, cupric sulfate pentahydrate copper 0.06, four water manganous sulfates 0.05, seven water ammonium molybdates 0.01, heptahydrate 0.002, sodium-acetate 1.8 and trimethyl-glycine 0.5, the rest is water, stir one hour.
Secondly, in a mixing machine, add commercially available NPK (15-15-15) Nitrogen, Phosphorus and Potassium 100kg, then add the Antiphytoviral fertilizer additive 1kg prepared above, fully after mixing, make the fertiliser granulates of diameter 4mm through Squeezinggranulator.
Then, this fertilizer is used to carry out field test.
Embodiment 2
First the fertilizer additive of Antiphytoviral is prepared.The method preparing secondary and micro-element fertilizers is: take a certain amount of calcium sulfate, magnesium chloride, ammonium sulfate, boric acid, Sodium orthomolybdate, zinc chloride, Manganous chloride tetrahydrate, ferrous ammonium sulphate and Salzburg vitriol respectively, make their nutritive element content ratio by weight, be 10: 8: 5: 2: 1: 2: 4: 8: 2 respectively, these raw materials are fully mixed stand-by.Then, taking this mixture 50kg is added in this mixing machine, add the acid of 10kg detritus again, placement 4 hours is discharged in abundant mixing after 0.5 hour, after terminating storage period, adding after 5kg copper sulfate mixes is added in the trace mineral supplement giving and first preparing, trace mineral supplement is urea 28, Sodium hexametaphosphate 99 3, Repone K 7, sodium lignosulfonate 6, sodium polyacrylate 2, Zinc Sulphate Heptahydrate 1.8, tin anhydride 0.7, boric acid 0.4, magnesium sulfate heptahydrate 0.2, cupric sulfate pentahydrate copper 0.06, four water manganous sulfates 0.05, seven water ammonium molybdates 0.01, heptahydrate 0.002, sodium-acetate 1.8 and trimethyl-glycine 0.5, the rest is water.Stir one hour.
Secondly; in a mixing machine, add selected commercially available NPK (15-15-15) Nitrogen, Phosphorus and Potassium 100kg, then add the Antiphytoviral fertilizer additive 1kg prepared above; after abundant mixing, make the fertiliser granulates of diameter 4mm through Squeezinggranulator.
Then, this fertilizer is used to carry out field test.
Embodiment 3
First the fertilizer additive of preparation control plant virus.The method preparing secondary and micro-element fertilizers is: take 9 kinds of raw materials respectively: calcium phosphate, fused(calcium magnesium)phosphate, sulfurous iron ore, borax, ammonium molybdate, zinc oxide, manganese oxide, iron protoxide and cupric oxide, the content ratio of raw material is made to be 18: 10: 4: 2: 0.5: 5: 5: 8: 2 by weight respectively, these raw materials are fully mixed, stand-by.Then, taking this mixture 50kg is added in this mixing machine, add 10kg oxalic acid again, placement 4 hours is discharged in abundant mixing after 0.5 hour, after terminating storage period, add after 5kg moroxydine hydrochloride mixes, toward the trace mineral supplement configured before this mixture adds 8kg, specifically consist of, be weight %, urea 28, Sodium hexametaphosphate 99 3, Repone K 7, sodium lignosulfonate 6, sodium polyacrylate 2, Zinc Sulphate Heptahydrate 1.8, tin anhydride 0.7, boric acid 0.4, magnesium sulfate heptahydrate 0.2, cupric sulfate pentahydrate copper 0.06, four water manganous sulfates 0.05, seven water ammonium molybdates 0.01, heptahydrate 0.002, sodium-acetate 1.8 and trimethyl-glycine 0.5, the rest is water.Stir one hour.
Secondly, commercially available urea is selected.In an agitator, add selected straight fertilizer urea 100kg, then add the control plant virus fertilizer additive 1.5kg prepared above, fully after mixing, make the fertiliser granulates of diameter 4mm through Squeezinggranulator.
Then, this fertilizer is used to carry out field test.
Comparative example 1-3
Comparative example 1-3 is have accordingly been according to the mode of embodiment 1-3, what just use in comparative example 1-3 contains the fertilizer additive of chitin without trace mineral supplement for what prepare according to CN100463882C method, establish negative control simultaneously, only use base manure, each embodiment is listed in the table below 1 compared with the concrete data of the volume increase ratio of negative control.
Experiment soil is brown earth great soil group, and fertility is even, and irrigation condition is good, extracts 0 ~ 20cm soil sample and chemically examine before experiment, wherein, and organic 0.85%, alkali-hydrolyzable nitrogen 44.0mg/kg, available phosphorus (P
2o
5) 49.0mg/kg, available potassium (K
2o) 82.5mg/kg, Ph value 6.1.
Enforcement crop is corn, rape, apple, and it be line-spacing is 10cm that trench digging is sowed seeds.
Experimental design is that three process are established in experiment, and repeat for four times, plot area is 20m
2, random alignment.
In experimentation, each community is except experiment fertilizer difference, and other field management, agronomic measures are all consistent.
Experimental result and analysis
According to table 1, prepared by the inventive method comparatively not contrasting containing the soil fertility quality of trace mineral supplement containing chitin is all significantly increased; Analysis of variance, F=21.747 > F0.01=8.02, reaches pole conspicuous level.By multiple comparisons, process 1 and process 3 differences reach pole conspicuous level, and therefore water-soluble chemical fertilizer of the present invention has comparatively contrasted extremely significant production-increasing function.
The foregoing is only preferred embodiment of the present invention, not in order to limit the present invention, all any amendments done within the spirit and principles in the present invention, equivalent replacement and improvement etc., all should be included within protection scope of the present invention.
Claims (4)
1. containing the fertilizer of Antiphytoviral fertilizer additive, it is characterized in that: this fertilizer is made up of straight fertilizer or compound manure and Antiphytoviral fertilizer additive, and the content of additive is the 0.1-5% of fertilizer gross weight;
Straight fertilizer is selected from urea, ammonium nitrate or potassium sulfate;
Compound manure is selected from primary ammonium phosphate or nitrogen-phosphorus-potassium compound fertilizer; Wherein,
Described Antiphytoviral fertilizer additive is made up of following component: with parts by weight
Described secondary and micro-element fertilizers is the mixture of 9 kinds of secondary and micro-element fertilizers of calcareous fertilisers, fertiliser containing magnesium, sulfur fertilizer, boron fertilizer, molydbenum fertilizer, zinc fertilizer, manganese fertilizer, iron fertilizer and copper fertilizer;
Described trace mineral supplement, specifically consist of, be weight %: urea 28, Sodium hexametaphosphate 99 3, Repone K 7, sodium lignosulfonate 6, sodium polyacrylate 2, Zinc Sulphate Heptahydrate 1.8, tin anhydride 0.7, boric acid 0.4, magnesium sulfate heptahydrate 0.2, cupric sulfate pentahydrate 0.06, four water manganous sulfate 0.05, seven water ammonium molybdate 0.01, heptahydrate 0.002, sodium-acetate 1.8 and trimethyl-glycine 0.5, the rest is water;
Described calcareous fertilisers are calcium carbonate, calcium sulfate or calcium phosphate;
Described fertiliser containing magnesium is magnesium sulfate, magnesium chloride or fused(calcium magnesium)phosphate;
Described sulfur fertilizer is ammonium sulfate;
Described boron fertilizer is boric acid or borax;
Described molydbenum fertilizer is ammonium molybdate or Sodium orthomolybdate;
Described zinc fertilizer is Zinc vitriol, zinc chloride or zinc oxide;
Described manganese fertilizer is three anhydrous manganeses or Manganous chloride tetrahydrate;
Described iron fertilizer is ferrous ammonium sulphate or iron protoxide;
Described copper fertilizer is Salzburg vitriol or cupric oxide;
Described organic acid is that one or more are selected from organic acid that is natural and/or synthesis, is selected from humic acid, citric acid or oxalic acid;
Described anti-plant virus agent is that one or more are selected from the anti-plant virus agent of chemical pesticide or biological pesticide, is selected from the anti-plant virus agent that one or more are selected from ribavirin, triazolone, triadimenol, olefin conversion, moroxydine hydrochloride, triacontanol price quote, polyoxyethylene sorbitol, sodium lauryl sulphate, venus crystals, copper sulfate or zinc sulfate.
2. fertilizer according to claim 1, is characterized in that: described Antiphytoviral fertilizer additive is made up of following component: with parts by weight
3. fertilizer according to claim 1, is characterized in that: described Antiphytoviral fertilizer additive is made up of following component: with parts by weight
4. the preparation method of the fertilizer described in claim 1-3, after described straight fertilizer or compound manure fully being mixed with described Antiphytoviral fertilizer additive, makes the fertiliser granulates of diameter 4mm through Squeezinggranulator.
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| CN101591205A (en) * | 2009-07-02 | 2009-12-02 | 郭红甫 | A kind of medicament-fertilizer mixture of preventing and treating crop virosis |
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| CN103804097A (en) | 2014-05-21 |
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