AR098484A1 - Insecticidas de 1-aril-3-alquilpirazol - Google Patents
Insecticidas de 1-aril-3-alquilpirazolInfo
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- AR098484A1 AR098484A1 ARP140104359A ARP140104359A AR098484A1 AR 098484 A1 AR098484 A1 AR 098484A1 AR P140104359 A ARP140104359 A AR P140104359A AR P140104359 A ARP140104359 A AR P140104359A AR 098484 A1 AR098484 A1 AR 098484A1
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- alkyl
- ring
- substituted
- unsubstituted
- cyano
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- C07D231/02—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings
- C07D231/10—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings having two or three double bonds between ring members or between ring members and non-ring members
- C07D231/12—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings having two or three double bonds between ring members or between ring members and non-ring members with only hydrogen atoms, hydrocarbon or substituted hydrocarbon radicals, directly attached to ring carbon atoms
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- A01N25/00—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests
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- A01N25/00—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests
- A01N25/08—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests containing solids as carriers or diluents
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- A—HUMAN NECESSITIES
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- A01N25/00—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests
- A01N25/30—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests characterised by the surfactants
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- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
- A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
- A01N43/48—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with two nitrogen atoms as the only ring hetero atoms
- A01N43/50—1,3-Diazoles; Hydrogenated 1,3-diazoles
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- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
- A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
- A01N43/48—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with two nitrogen atoms as the only ring hetero atoms
- A01N43/56—1,2-Diazoles; Hydrogenated 1,2-diazoles
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- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
- A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
- A01N43/48—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with two nitrogen atoms as the only ring hetero atoms
- A01N43/58—1,2-Diazines; Hydrogenated 1,2-diazines
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- A—HUMAN NECESSITIES
- A61—MEDICAL OR VETERINARY SCIENCE; HYGIENE
- A61P—SPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
- A61P33/00—Antiparasitic agents
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- C07D401/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
- C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
- C07D401/04—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings directly linked by a ring-member-to-ring-member bond
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- C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
- C07D401/06—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
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- C07D403/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings
- C07D403/06—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
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- C07D417/06—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
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Abstract
También se describen las composiciones que contienen los compuestos y los métodos para controlar una plaga invertebrada; el método comprende la etapa de poner la plaga invertebrada o su ambiente en contacto con cantidad biológicamente eficaz de un compuesto o una composición de la presente. Reivindicación 1: Un compuesto seleccionado de la fórmula (1), un N-óxido o una sal del estos, caracterizado porque Q es un resto de fórmula (2); R¹ es alquilo C₁₋₆, alquenilo C₂₋₆ o alquinilo C₂₋₆, cada uno insustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, C(X)R⁵ᵃ, C(O)OR⁶ᵃ, C(X)NR⁷ᵃR⁸ᵃ, NR⁹ᵃR¹⁰ᵃ, OR¹²ᵃ, S(O)ₙR¹¹ᵃ, SO₂NR⁹ᵃR¹⁰ᵃ, Si(R¹⁴)₃ y Z¹; o R¹ es un anillo de 3 a 10 miembros totalmente o parcialmente saturado o un sistema anular de 7 a 11 miembros totalmente o parcialmente saturado, cada anillo o sistema anular contiene miembros anulares seleccionados de átomos de carbono y hasta 4 heteroátomos independientemente seleccionados de hasta 2 O, hasta 2 S, y hasta 4 N, en donde hasta 3 miembros anulares de los átomos de carbono son independientemente seleccionados C(=O) y C(=S) y los miembros anulares de los átomos de azufre son independientemente seleccionados de S, S(O) o S(O)₂, cada anillo o sistema anular insustituido o sustituido con 1 a 4 R⁴; Z es fenilo sustituido con 1 a 3 R⁴; o Z es un anillo heteroaromático de 5 ó 6 miembros o un sistema anular bicíclico heteroaromático de 8 a 10 miembros, cada anillo o sistema anular no sustituido o sustituido con 1 a 3 R⁴; Z¹ es un anillo de 3 a 10 miembros o un sistema anular de 7 a 11 miembros, cada anillo o sistema anular contiene miembros anulares seleccionados de átomos de carbono y hasta 4 heteroátomos independientemente seleccionados de hasta 2 O, hasta 2 S, y hasta 4 N, en donde hasta 3 miembros anulares de los átomos de carbono son independientemente seleccionados C(=O) y C(=S) y los miembros anulares de los átomos de azufre son independientemente seleccionados de S, S(O) o S(O)₂, cada anillo o sistema anular insustituido o sustituido con 1 a 4 R⁴; R²ᵃ y R²ᶜ son, independientemente, cada uno, H, halógeno, ciano, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, OR¹² o S(O)ₙR¹¹; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con por lo menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; R²ᵇ y R²ᵈ son, independientemente cada uno, H, halógeno, ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, OR¹², S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con por lo menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R⁴; J¹ es un enlace directo, -C(R³ᵃR³ᵇ)- o -C(R³ᵃR³ᵇ)C(R³ᵃR³ᵇ)-; J² es un enlace directo o -C(R³ᶜR³ᵈ)-; M es -C(R³ᵉ)(A)-, -N(A¹)-, -O- o -S(O)ₙ-; A es halógeno, ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, alquilo C₁₋₄, haloalquilo C₁₋₄, C₍O₎R⁵ᵃ, C(O)OR⁶ᵃ, C(O)NR⁷ᵃR⁸ᵃ, NR⁹ᵃR¹⁰ᵃ, OR¹²ᵃ y S(O)ₙR¹¹ᵃ; o fenilo, un anillo heteroaromático de 5 ó 6 miembros o un sistema anular heteroaromático de 7 a 11 miembros, cada anillo o sistema anular no sustituido o sustituido con 1 a 3 R⁴; A¹ es ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, alquilo C₁₋₄, haloalquilo C₁₋₄, C₍O₎R⁵ᵃ, C(O)OR⁶ᵃ, C(O)NR⁷ᵃR⁸ᵃ, NR⁹ᵃR¹⁰ᵃ, OR¹²ᵃ y S(O)ₙR¹¹ᵃ; o fenilo, un anillo heteroaromático de 5 ó 6 miembros o un sistema anular heteroaromático de 7 a 11 miembros, cada anillo o sistema anular no sustituido o sustituido con 1 a 3 R⁴; o bencilo no sustituido o sustituido con 1 a 3 R⁴; cada R³ᵃ y cada R³ᶜ son independientemente H, halógeno, ciano, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, OR¹² o S(O)ₙR¹¹; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇,cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con por lo menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; cada R³ᵇ y R³ᵈ son, independientemente cada uno, H, halógeno, ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, OR¹², S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con por lo menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R⁴; R³ᵉ es H, halógeno, ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, OR¹², NR⁹R¹⁰, S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆,alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇, cicloalquilalquilo C₄₋₈ o cicloalquenilo C₃₋₆, cada uno no sustituido o sustituido con por lo menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R⁴; R³ᵉ y A pueden tomarse junto con el átomo de carbono al cual están unidos para formar un anillo de 3 a 7 miembros que contiene miembros anulares seleccionados de átomos de carbono y hasta 2 heteroátomos independientemente seleccionados de un átomo de oxígeno, un átomo de azufre, y hasta 2 átomos de nitrógeno, en donde hasta 2 miembros anulares de los átomos de carbono son independientemente seleccionados C(=O) y C(=S) y el miembro anular del átomo de azufre se selecciona de S, S(O) o S(O)₂, el anillo es insustituido o sustituido con hasta 4 sustituyentes independientemente seleccionados del grupo que consiste en halógeno, ciano, y alquilo C₁₋₄; o cuando dos cualquiera de R²ᵃ, R²ᵇ, R²ᶜ, R²ᵈ, R³ᵃ, R³ᵇ, R³ᶜ, R³ᵈ o R³ᵉ son independientemente alquilo C₁₋₄, entonces los dos R²ᵃ, R²ᵇ, R²ᶜ, R²ᵈ, R³ᵃ, R³ᵇ, R³ᶜ, R³ᵈ o R³ᵉ pueden tomarse juntos para formar un anillo; cada R⁴ es independientemente halógeno, ciano, nitro, C(X)R⁵, C(O)OR⁶, C(X)NR⁷R⁸, NR⁹R¹⁰, OR¹², S(O)ₙR¹¹ o SO₂NR⁹R¹⁰; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; cada R⁵ es independientemente H; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R⁵ᵃ es independientemente alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R⁶ es independientemente alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R⁶ᵃ es independientemente alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R⁷ y cada R⁸ son independientemente H; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R⁷ᵃ y R⁸ᵃ es independientemente H, alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R⁹ y cada R¹⁰ son independientemente H, C(X)R⁵, C(O)OR⁶ o C(X)NR⁷R⁸; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R⁹ᵃ y R¹⁰ᵃ es independientemente H, C(X)R⁵ᵃ, C(O)OR⁶ᵃ, C(X)NR⁷ᵃR⁸ᵃ, alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R¹¹ es independientemente alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6 miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R¹¹ᵃ es independientemente alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R¹² es independientemente H; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; o fenilo o un anillo heteroaromático de 5 ó 6miembros, cada anillo no sustituido o sustituido con 1 a 3 R¹³; cada R¹²ᵃ es independientemente alquilo C₁₋₄ o haloalquilo C₁₋₄; cada R¹³ es independientemente halógeno, ciano, nitro, C(X)R⁵ᵃ, C(O)OR⁶ᵃ, C(X)NR⁷ᵃR⁸ᵃ, NR⁹ᵃR¹⁰ᵃ, OR¹²ᵃ, S(O)ₙR¹¹ᵃ o SO₂NR⁹ᵃR¹⁰ᵃ; o alquilo C₁₋₆, alquenilo C₂₋₆, alquinilo C₂₋₆, cicloalquilo C₃₋₇ o cicloalquilalquilo C₄₋₈, cada uno no sustituido o sustituido con al menos un sustituyente independientemente seleccionado del grupo que consiste en halógeno, ciano, nitro, OR¹²ᵃ, alquilo C₁₋₄, haloalquilo C₁₋₄ y S(O)ₙR¹¹ᵃ; cada R¹⁴ es independientemente alquilo C₁₋₄; cada X es independientemente O ó S; y cada n es, independientemente, 0, 1 ó 2.
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JP7449573B2 (ja) | 2021-02-08 | 2024-03-14 | ロンタイ株式会社 | 植生カプセル及びそれを用いた植生方法と植生体 |
CN112920233A (zh) * | 2021-02-24 | 2021-06-08 | 吴霜 | 一种改善其可加工性的甲维盐的合成方法 |
WO2024005032A1 (ja) * | 2022-06-29 | 2024-01-04 | 株式会社Adeka | アゼパンジオン誘導体又はその塩類及び該化合物を含有する有害生物防除剤並びにその使用方法 |
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CN105745201A (zh) | 2016-07-06 |
CN105745201B (zh) | 2019-08-20 |
KR20160086903A (ko) | 2016-07-20 |
US10112906B2 (en) | 2018-10-30 |
BR112016011346B1 (pt) | 2020-09-01 |
US20160280660A1 (en) | 2016-09-29 |
BR112016011346B8 (pt) | 2020-10-20 |
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JP6456953B2 (ja) | 2019-01-23 |
TW201601632A (zh) | 2016-01-16 |
MX2016006555A (es) | 2016-08-03 |
BR112016011346A2 (pt) | 2017-08-08 |
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